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We perform a beat-frequency-resolved analysis for two-dimensional electronic spectroscopy using a high-speed and stable 2D electronic spectrometer and few-cycle visible laser pulses to disentangle the vibrational coherences in an artificial…

Fluorescence imaging is an essential diagnostic tool in many fields, but diffraction-limited optical imaging at depth is limited by scattering. Here, we present a method based on multiple random illuminations, combined with a computational…

Optics · Physics 2026-03-30 Lei Zhu , Tengfei Wu , Bernhard Rauer , Hilton B. de Aguiar , Sylvain Gigan

We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor…

Diffraction of coherent x-ray beams is treated through the Fractionnal Fourier transform. The transformation allow us to deal with coherent diffraction experiments from the Fresnel to the Fraunhofer regime. The analogy with the…

Other Condensed Matter · Physics 2025-01-08 David Le Bolloc'h , Jean-Francois Sadoc

X-ray free-electron lasers (XFELs) utilize high-density and high-energy electron bunches which are well-suited to produce Compton back-scattering radiation. Here we study study interaction of such electron bunches during head-on collision…

Accelerator Physics · Physics 2023-11-16 Svitozar Serkez , Eugene Bulyak , Gianluca Geloni

X-ray free-electron lasers (XFELs) utilize high-density and high-energy electron bunches which are well-suited to produce Compton back-scattering radiation. Here we study back-scattered radiation pulses produced by the interaction of XFEL…

Accelerator Physics · Physics 2023-09-28 Eugene Bulyak , Svitozar Serkez , Gianluca Aldo Geloni

X-ray scattering experiments using Free Electron Lasers (XFELs) are a powerful tool to determine the molecular structure and function of unknown samples (such as COVID-19 viral proteins). XFEL experiments are a challenge to computing in two…

Distributed, Parallel, and Cluster Computing · Computer Science 2024-03-21 Johannes P. Blaschke , Aaron S. Brewster , Daniel W. Paley , Derek Mendez , Asmit Bhowmick , Nicholas K. Sauter , Wilko Kröger , Murali Shankar , Bjoern Enders , Deborah Bard

The Linac Coherent Light Source (LCLS) is an X- ray free electron laser (XFEL) facility enabling the study of the structure and dynamics of single macromolecules. A major upgrade will bring the repetition rate of the X-ray source from 120…

Computational Physics · Physics 2021-09-14 Hsing-Yin Chang , Elliott Slaughter , Seema Mirchandaney , Jeffrey Donatelli , Chun Hong Yoon

X-ray sources are developing rapidly and their coherent output is growing extremely rapidly. The increased coherent flux from modern X-ray sources is being matched with an associated rapid development in experimental methods. This article…

Optics · Physics 2012-08-09 Keith A Nugent

Measurements of the spatial and temporal coherence of single, femtosecond x-ray pulses generated by the first hard x-ray free-electron laser (FEL), the Linac Coherent Light Source (LCLS), are presented. Single shot measurements were…

Modern x-ray free-electron lasers (XFELs) produce x-ray pulses of exceptional transverse coherence. This is due largely to the process of optical guiding by which the radiation is both refractively guided by the bunched electron beam and…

Accelerator Physics · Physics 2021-04-20 River R. Robles , Gabriel Marcus , Zhirong Huang

The evolution from 3rd to 4th generation synchrotron radiation (SR) sources significantly enhanced their coherence, making coherent scattering techniques such as coherent X-ray diffraction imaging (CXDI) and X-ray photon correlation…

Accelerator Physics · Physics 2021-10-20 Han Xu , Zhongzhu Zhu , Peng Liu , Yuhui Dong , Liang Zhou

Compressive spectral imaging enables to reconstruct the entire three-dimensional (3D) spectral cube from a few multiplexed images. Here, we develop a novel compressive spectral imaging technique using diffractive lenses. Our technique uses…

Image and Video Processing · Electrical Eng. & Systems 2019-09-24 Oğuzhan Fatih Kar , Figen S. Oktem

Neutron imaging is an invaluable noninvasive technique for exploring new science and assisting industrial manufacture. However, state-of-the-art neutron facilities are extremely expensive and inconvenient to access, while the flux of…

We study a nonlinear Schr\"odinger equation which arises as an effective single particle model in X-ray Free Electron Lasers (XFEL). This equation appears as a first-principles model for the beam-matter interactions that would take place in…

Numerical Analysis · Mathematics 2014-06-18 Paolo Antonelli , Agissilaos Athanassoulis , Zhongyi Huang , Peter A. Markowich

X-ray fluorescence holography (XFH) is a method for obtaining diffraction-limited images of the local atomic structure around a given type of emitter. The reconstructed wave-field represents a distorted image of the scatterer electron…

Condensed Matter · Physics 2009-09-29 S. Marchesini , C. S. Fadley , F. J. Garcia de Abajo

In coherent X-ray diffraction microscopy the diffraction pattern generated by a sample illuminated with coherent x-rays is recorded, and a computer algorithm recovers the unmeasured phases to synthesize an image. By avoiding the use of a…

The number of photons available by coherent X-ray scattering from a single biomolecule is considerably less because of the extremely small elastic-scattering cross-section and low damage threshold. Even with a high X-ray flux of 3 x 10to 12…

Optics · Physics 2009-11-13 Tsumoru Shintake

Many applications of short-wavelength radiation impose strong requirements on the coherence properties of the source. However, the measurement of such properties poses a challenge, mainly due to the lack of high-quality optics and source…