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The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we…

Superconductivity · Physics 2021-07-28 Da-Wei Yao , Tao Li

X-ray magnetic circular dichroism spectroscopy has been used to characterize the electronic structure and magnetic moment of Cr$_2^+$. Our results indicate that the removal of a single electron from the $4s\sigma_g$ bonding orbital of…

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

Although orbital degrees of freedom are a factor of fundamental importance in strongly correlated transition metal compounds, orbital correlations and dynamics remain very difficult to access, in particular by neutron scattering. Via a…

Strongly Correlated Electrons · Physics 2015-03-20 Pasquale Marra , Krzysztof Wohlfeld , Jeroen van den Brink

The electronic properties of the polar interface between insulating oxides is a subject of great current interest. An exciting new development is the observation of robust magnetism at the interface of two non-magnetic materials LaAlO_3…

Strongly Correlated Electrons · Physics 2013-10-03 Sumilan Banerjee , Onur Erten , Mohit Randeria

We report on investigations of the complex magnetostructural and spin-state transitions in the breathing pyrochlore LiFeCr$_{4}$O$_{8}$ by means of magnetization, M\"ossbauer spectroscopy, and density functional theory (DFT) calculations.…

Strongly Correlated Electrons · Physics 2023-12-05 Bo Zhang , Wei Ren , Shengyu Yang , Qifeng Kuang , Da Li , Xin Liu , Anmin Zhang , Hua Pang , Liyun Tang , Liang Qiao , Fashen Li , Zhiwei Li

We present a detailed account of the physics of Vanadium sesquioxide (${\rm V_2O_3}$), a benchmark system for studying correlation induced metal-insulator transition(s). Based on a detailed perusal of a wide range of experimental data, we…

Strongly Correlated Electrons · Physics 2009-11-11 M. S. Laad , L. Craco , E. Müller-Hartmann

Due to the strong coupling between magnetism and ferroelectricity, $(\mathrm{ND}_4)_2\mathrm{FeCl}_5\cdot\mathrm{D}_2\mathrm{O}$ exhibits several intriguing magnetic and electric phases. In this letter, we include high-order onsite spin…

Materials Science · Physics 2021-08-25 Shaozhi Li , Randy S. Fishman

We study the spin-dependent electronic structure of UTe and UT_{2}Si_{2} (T=Cu and Mn) compounds with a combination of x-ray magnetic circular dichroism measurements and first principle calculations. By exploiting the presence of sizable…

Strongly Correlated Electrons · Physics 2016-01-12 R. D. dos Reis , L. S. I. Veiga , D. Haskel , J. C. Lang , Y. Joly , F. G. Gandra , N. M. Souza-Neto

Nonresonant inelastic x-ray scattering (NIXS) is a possible tool to detect charge excitations in electron systems. In addition, multipole transitions at high-momentum-transfer region open a new possibility to determine orbital-selective…

Strongly Correlated Electrons · Physics 2015-11-11 Kenji Tsutsui , Eiji Kaneshita , Takami Tohyama

The present paper demonstrates the feasibility of X-ray Absorption Spectroscopy (XAS) and X-ray Magnetic Circular Dichroism (XMCD) at high pressure at the Fe-K edge on the ID24 energy dispersive beamline of the ESRF. In 3d transition…

Instrumentation and Detectors · Physics 2007-05-23 Olivier Mathon , Francois Baudelet , Jean-Paul Itie , Sebastien Pasternak , Alain Polian , Sakura Pascarelli

In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter,…

Proximity effects allow for the adjustment of magnetic properties in a physically elegant way. If two thin ferromagnetic (FM) films are brought into contact, electronic coupling alters their magnetic exchange interaction at their interface.…

The present article reports the governing influence of substituting the M2 site in nanoscale MFe2O4 spinel ferrites by different magnetic metals Fe,Mn,Co,Ni on magnetorheological and magneto elastoviscous behaviors of the corresponding…

Soft Condensed Matter · Physics 2020-03-18 Ankur Chattopadhyay , Subhajyoti Samanta , Rajendra Srivastava , Rajib Mondal , Purbarun Dhar

By performing accurate ab-initio density functional theory calculations, we study the role of $4f$ electrons in stabilizing the magnetic-field-induced ferroelectric state of DyFeO$_{3}$. We confirm that the ferroelectric polarization is…

Materials Science · Physics 2015-05-14 Alessandro Stroppa , Martijn Marsman , Georg Kresse , Silvia Picozzi

Thermally induced spin control is one of the main directions for future spin devices. In this study, we synthesized single-phase polycrystalline ErFe1-xCrxO3 and combined the magnetization curves and M\"ossbauer spectra to determine the…

Materials Science · Physics 2022-07-11 Jiyu Shen , Jiajun Mo , Zeyi Lu , Zhongjin Wu , Chenying Gong , Kaiyang Gao , Pinglu Zheng , Min Liu , Yanfang Xia

The orbitally degenerate A-site spinel compound FeSc2S4 has been experimentally identified as a ``spin-orbital liquid'', with strong fluctuations of both spins and orbitals. Assuming that the second neighbor spin exchange J2 is the dominant…

Strongly Correlated Electrons · Physics 2009-12-14 Gang Chen , Andreas P. Schnyder , Leon Balents

Iron pnictides and selenides display a variety of unusual magnetic phases originating from the interplay between electronic, orbital, and lattice degrees of freedom. Using powder inelastic neutron scattering on the two-leg ladder BaFe2Se3,…

Strongly Correlated Electrons · Physics 2015-07-24 M. Mourigal , Shan Wu , M. B. Stone , J. R. Neilson , J. M. Caron , T. M. McQueen , C. L. Broholm

We study the magnetic, structural, and electronic properties of the recently discovered iron- based superconductor BaFe2S3 based on density functional theory with the generalized gradient approximation. The calculations show that the…

Strongly Correlated Electrons · Physics 2015-08-19 Michi-To Suzuki , Ryotaro Arita , Hiroaki Ikeda

We present a detailed first principles study on the magnetic structure of an Fe monolayer on different surfaces of 5d transition metals. We use the spin-cluster expansion technique to obtain parameters of a spin model, and predict the…

Materials Science · Physics 2014-05-06 E. Simon , K. Palotás , B. Ujfalussy , A. Deák , G. M. Stocks , L. Szunyogh
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