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We demonstrate an all-optical approach for precise characterization of attosecond extreme ultraviolet pulses. Isolated attosecond pulse is produced from high order harmonics using intense driving pulse with proper gating technique. When a…

The measurement of optical ultrafast laser pulses is done indirectly because the required bandwidth to measure these pulses exceeds the bandwidth of current electronics. As a result, this measurement problem is often posed as a 1-D phase…

Optics · Physics 2023-04-28 Daniel J Kane , Andrei B. Vakhtin

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , J. Bowlan , S. A. Trugman , R. Valdes Aguilar , J. Qi , X. Liu , J. Furdyna , M. Dobrowolska , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

The recent introduction of coherent optical communications has created a compelling need for ultra-fast phase-sensitive measurement techniques operating at milliwatt peak power levels and in time scales ranging from sub-picoseconds to…

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…

Chemical Physics · Physics 2019-10-23 Baoning Wang , Lixin He , Yanqing He , Yinfu Zhang , Renzhi Shao , Pengfei Lan , Peixiang Lu

We demonstrate a remarkably effective single-stage compression technique for ultrafast pulses in the visible electromagnetic spectrum using second-harmonic pulses at 515 nmderived from a 1030 nm Yb-based femtosecond regenerative amplifier.…

The growth of ultrafast nanophotonic circuits necessitates the development of energy-efficient on-chip pulse characterization techniques. Nanophotonic realizations of Frequency Resolved Optical Gating, a common pulse characterization…

A Python package for the calculation of spectrograms with optimized time and frequency resolution for application in the analysis of numerical simulations on ultrashort pulse propagation is presented. Gabor's uncertainty principle prevents…

Computational Physics · Physics 2018-09-05 O. Melchert , B. Roth , U. Morgner , A. Demircan

A new approach to all-optical detection and control of the coupling between electric and magnetic order on ultrafast timescales is achieved using time-resolved second harmonic generation (SHG) to study a ferroelectric (FE)/ferromagnet (FM)…

Materials Science · Physics 2015-01-12 Y. M. Sheu , S. A. Trugman , L. Yan , Q. X. Jia , A. J. Taylor , R. P. Prasankumar

Accurate and fast characterization of spatiotemporal information of high-intensity, ultrashort pulses is crucial in the field of strong-field laser science and technology. While conventional self-referenced interferometers were widely used…

Optics · Physics 2023-07-19 Yifei Chen , Zhiyuan Huang , Ding Wang , Yu Zhao , Jianhua Fu , Meng Pang , Yuxin Leng , Zhizhan Xu

Second-harmonic generation (SHG) microscopy provides label-free imaging of biological tissues with unique contrast mechanisms, but its resolution is limited by the diffraction limit. Here, we present the first experimental demonstration of…

Optics · Physics 2023-04-28 Jungho Moon , Sungsam Kang , Jin Hee Hong , Seokchan Yoon , Wonshik Choi

We demonstrate unexpectedly strong second harmonic generation (SHG) in Argon gas by use of spatiotemporally focused (SF) femtosecond laser pulses. The resulting SHG by the SF scheme at a 75 cm distance shows a significantly enhanced…

A compact and broadband polarimetric imaging platform is presented, based on second-harmonic generation (SHG) in nonlinear flat-optics. The system employs periodic all-dielectric AlGaAs gratings to induce polarization-dependent SH emission,…

We present an algorithm based on numerical techniques that have become standard for solving nonlinear integral equations: Newton's method, homotopy continuation, the multilevel method and random projection to solve the inversion problem…

Computational Physics · Physics 2021-05-26 Michael Jasiulek

The commonly used methods to characterize ultrafast laser pulses, such as frequency-resolved optical gating (FROG) and dispersion scan (d-scan), face problems when they are used on pulses with a chirp varying within the laser beam or the…

Optics · Physics 2021-02-19 M. Guesmi , Petra Veselá , Karel žÍidek

Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

Optics · Physics 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

A scheme to encode arbitrarily long integer pairs on degenerate optical parametric oscillations multiplexed in time is proposed. The classical entanglement between the polarization directions and the phases of the oscillating pulses,…

Quantum Physics · Physics 2022-05-25 Minghui Li , Wei Wang , Zikang Tang , Hou Ian

The time-resolved detection of ultrashort pulsed THz-band electric field temporal profiles without an ultrashort laser probe is demonstrated. A non-linear interaction between a narrow-bandwidth optical probe and the THz pulse transposes the…

Optics · Physics 2015-06-11 David A. Walsh , Edward W. Snedden , Steven P. Jamison

Numerical optimal control (GRAPE) can in principle discover pulse shapes that suppress all coherent gate error to machine precision. But when does that capability actually matter? We present a systematic comparison of Gaussian, DRAG, and…

Quantum Physics · Physics 2026-02-16 Rylan Malarchick