Related papers: Quantum model for Impulsive Stimulated Raman Scatt…
Nonclassicality is studied through a quasidistribution of phases for the Raman process under both weak and strong pump conditions. In the former case, the solution is applicable to both resonant and off-resonant Raman processes, while…
A quasi-classical model (QCM) of molecular dynamics in intense femtosecond laser fields has been developed, and applied to a study of the effect of an ultrashort `control' pulse on the vibrational motion of a deuterium molecular ion in its…
We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…
In this article we present a full description of the quantum Kerr Ising model---a linear optical network of parametrically pumped Kerr non-linearities. We consider the non-dissapative Kerr Ising model and, using variational techniques, show…
Conventional scattering theory is incomplete in that it does not adequately describe the behaviour of the wave function at macroscopic distances from the scattering reaction volume. In scattering experiments particles are incident from…
We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…
A collisionless shock wave is treated as a streaming plasma instability in the interstellar medium (ISM). We assume that in a steady state, this instability propagates through the ISM as a self-driven plasma instability, whereby the…
Effect of the induced Compton and Raman scattering on short, bright radio pulses is investigated. It is shown that when a single pulse propagates through the scattering medium, the effective optical depth is determined by the duration of…
Stimulated Raman backscatter (SRS) is used as a remote sensor to quantify the instantaneous laser power after transfer from outer to inner cones that cross in a National Ignition Facility (NIF) gas-filled hohlraum plasma. By matching SRS…
We calculate the resonance fluorescence signal of a two-level system coupled to a quantized phonon mode. By treating the phonons in the independent boson model and not performing any approximations in their description, we also have access…
We solve for the electronic Raman scattering response functions on an infinite-dimensional hypercubic lattice employing dynamical mean field theory. This contribution extends previous work on the nonresonant response to include the mixed…
We examine SERS from two perspectives: as a phenomenon described by the Laplace Equation (the electrostatic or Rayleigh limit) and by the Helmholtz Equation (electrodynamic or Mie limit). We formulate the problem in terms of the scalar…
We study effective models describing systems of quantum particles interacting with quantized (electromagnetic) fields in the quasi-classical regime, i.e., when the field's state shows a large average number of excitations. Once the field's…
Spin-photon interfaces (SPIs) are key devices of quantum technologies, aimed at coherently transferring quantum information between spin qubits and propagating pulses of polarized light. We study the potential of a SPI for quantum non…
A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…
We study the optical response of a binary system of identical atoms in which one of them is excited by an incoherent pump. %We study the properties of photon scattering, absorption and emission, together with the time evolution of the…
We present a flexible and efficient ultrafast time-resolved spontaneous Raman spectroscopy setup to study collective excitation and quasi-particle dynamics in quantum matter. The setup has a broad energy tuning range extending from the…
We demonstrate and study the enhancement of intermediate-field two-photon absorption by shaped femtosecond pulses having spectral phases of antisymmetric nature. The intermediate-field regime corresponds to pulse intensities, where the…
The low energy physics of interacting quantum systems is typically understood through the identification of the relevant quasiparticles or low energy excitations and their quantum numbers. We present a quantum information framework that…
Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…