Related papers: Quantum model for Impulsive Stimulated Raman Scatt…
We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…
The "Impulsive Stimulated Raman Scattering" (ISRS), is generally performed using ultrashort laser pulses. It shifts the frequency of the laser beam without any change of the wave surfaces and any appearance of extra lines. ISRS works with…
The Impulsive Stimulated Raman Scattering (ISRS) is a parametric light-matter interaction which shifts the frequencies of two ultrashort laser light pulses by a non-quantified transfer of energy. As ISRS has no threshold, the laser pulses…
A semiclassical model is used to investigate the possibility of selectively exciting one of two closely spaced, uncoupled Raman transitions. The duration of the intense pump pulse that creates the Raman coherence is shorter than the…
We simulate a third-order nonlinear signal in a pump-probe spectroscopy from the interference between first- and second-order wavepackets (WPs), as well as from a state-to-state transition for Stokes and coherent anti-Stokes pathways in the…
Stimulated Raman scattering (SRS) is a powerful method for label-free imaging and spectroscopy of materials. Recent experiments have shown that quantum-enhanced Raman scattering can surpass the shot noise limit and improve the sensitivity…
We investigated the coherent phonon generation mechanism by irradiation of an ultrashort pulse with a simple two-level model. Our derived formulation shows that both impulsive stimulated Raman scattering (ISRS) and impulsive absorption (IA)…
In the shock-ignition inertial confinement fusion scheme, high-intensity lasers propagate through an inhomogeneous coronal plasma, driving a shock designed to cause fuel ignition. During the high-intensity ignitor laser pulse, SRS…
While complicated, unreliable alternatives to Doppler effect were proposed, an elementary optical light- matter interaction provides one which is commonly observed in the labs, but with a distortion due to the use of short, powerful laser…
Quantum entanglement offers an incredible resource for enhancing the sensing and spectroscopic probes. Here we develop a microscopic theory for the stimulated Raman scattering (SRS) using entangled photons. We demonstrate that the…
Stimulated Raman scattering (SRS) has played an increasingly pivotal role in chemistry and photonics. Recently, understanding of light-molecule interaction during SRS was brought to a new quantitative level through the introduction of…
In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…
Stimulated Raman scattering (SRS) represents a powerful tool for accessing the vibrational properties of molecular compounds or solid state systems. From a spectroscopic perspective, SRS is able to capture Raman spectra free from incoherent…
Interaction of a high intensity short laser pulse with near-critical plasmas allows to achieve extremely high coupling efficiency and transfer laser energy to energetic ions. One dimensional Particle-In-Cell (PIC) simulations are considered…
In the quantum process of stimulated Raman scattering (SRS), a laser photon propagating in a resonance medium undergoes multifold conversions into a Stokes photon and back. The nontrivial ``cooperative'' behavior of the Stokes component of…
To date, two types of coupling between electromagnetic radiation and a crystal lattice have been identified experimentally. One is direct, for infrared (IR)-active vibrations that carry an electric dipole. The second is indirect, it occurs…
We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…
Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by…
We have developed a theory of the one-phonon intraband resonance Raman scattering (IRRS) in anisotropic quantum dots subjected to an arbitrarily directed magnetic field. The differential Raman cross section is obtained. The resonance…