Related papers: Quantum model for Impulsive Stimulated Raman Scatt…
Plasmon-enhanced Raman scattering (PERS) becomes nonlinear when phonon pumping and phonon-stimulated scattering come into play. It is fundamental to the understanding of PERS and its photobleaching behavior. By quantization of the molecular…
Surface-Enhanced Raman Scattering (SERS) allows for detection and identification of molecular vibrational fingerprints in minute sample quantities. The SERS process can be also exploited for optical manipulation of molecular vibrations. We…
Ultrafast characterization and control of many-body interactions and elementary excitations are critical to understanding and manipulating emergent phenomena in strongly correlated systems. In particular, spin interaction plays an important…
We consider the coherent stimulated Raman process developing in an optically dense disordered atomic medium, which can also incoherently scatter the light over all outward directions. The Raman process is discussed in the context of a…
Induced Compton scattering (ICS) is a nonlinear interaction between intense electromagnetic radiation and a rarefied plasma. Although the magnetosphere of pulsars is a potential cite at which ICS occurs in nature, the ICS signatures have…
A comprehensive theory is proposed to describe the propagation and absorption of ultra-intense, short laser pulse through the under-dense plasma. The kinetic aspects of plasma are fully incorporated using extensive particle-in-cell (PIC)…
We report a joint experimental and theoretical study of the interference properties of a single photon source based on a In(Ga)As quantum dot embedded in a quasi-planar GaAs-microcavity. Using resonant laser excitation with a pulse…
We theoretically investigate resonant x-ray scattering from two non-interacting Ne+ ions driven by an intense attosecond pulse using a non-relativistic, QED-based time-dependent framework. Our model includes Rabi oscillations,…
Photophysical and photochemical processes are ruled by the interplay between transient vibrational and electronic degrees of freedom, which are ultimately determined by the multidimensional potential energy surfaces (PESs). Differences…
We explore coherent control of stimulated Raman scattering in the nonimpulsive regime. Optical pulse shaping of the coherent pump field leads to control over the stimulated Raman output. A model of the control mechanism is investigated.
Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential…
Coherent Raman scattering spectroscopy is studied purposely, with the Gaussian ultrashort pulses as a hands-on elucidatory extraction tool of the clean coherent Raman resonant spectra from the overall measured data contaminated with the…
Stimulated Raman scattering (SRS) in plasma in the degenerate regime is studied theoretically and numerically. Different from normal SRS with the non-degenerate eigen electrostatic mode excited, the degenerate SRS is developed at plasma…
The classical or quantum nature of optical spectroscopy signals is a topic that has attracted great attention recently. Spectroscopic techniques have been classified as quantum or classical depending on the light-source used in their…
We report results and modelling of an experiment performed at the TAW Vulcan laser facility, aimed at investigating laser-plasma interaction in conditions which are of interest for the Shock Ignition scheme to Inertial Confinement Fusion,…
Spontaneous Raman scattering (SpRS) is a weak non-linear effect, particularly relevant to classical-quantum coexistence transmission and sensing applications. In classical transmission, the relevant Raman effect is stimulated Raman…
We investigate intensity of the parametric down conversion of ultrashort, ultraviolet pulse both in a low- and high-conversion regime. In the first regime, we develop a simple analytical expressions for the photon flux of the fluorescence.…
Nonlinear optical processes are used in biological microscopy to surpass the diffraction limit on resolution, image deeper into brain tissues, and identify biomolecules without exogenous labels. These techniques typically require high…
An accurate, closed-form expression evaluating the nonlinear interference (NLI) power in coherent optical transmission systems in the presence of inter-channel stimulated Raman scattering (ISRS) is derived. The analytical result enables a…
We treat resonant Raman scattering via the multiphonon exciton transitions in cylindrical quantum dots with a parabolic confinement in the lateral direction and with a finite rectangular interface-barrier confinement in the axial direction.…