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We present a computational approach for electronically correlated metallic surfaces and interfaces, which combines Density Functional and Dynamical Mean Field Theory using a multi-orbital perturbative solver for the many-body problem. Our…

Strongly Correlated Electrons · Physics 2022-04-06 Andrea Droghetti , Miloš M. Radonjić , Anita Halder , Ivan Rungger , Liviu Chioncel

We present the combination of Density Functional Theory (DFT) and Dynamical Mean Field Theory (DMFT) for computing the electron transmission through two-terminals nanoscale devices. The method is then applied to metallic junctions…

Strongly Correlated Electrons · Physics 2022-09-14 Andrea Droghetti , Milos M. Radonjić , Liviu Chioncel , Ivan Rungger

We extend the nonequilibrium dynamical mean field (DMFT) formalism to inhomogeneous systems by adapting the "real-space" DMFT method to Keldysh Green's functions. Solving the coupled impurity problems using strong-coupling perturbation…

Strongly Correlated Electrons · Physics 2014-08-15 Martin Eckstein , Philipp Werner

We have performed a systematic study of the emergence of meta-stable states in density functional theory plus Hubbard U (DFT+U ) simulations of NiO, CoO, FeO. Particular attention is given to the spin-polarization of the…

Materials Science · Physics 2018-10-25 Samara Keshavarz , Patrik Thunström

A systematic framework to investigate spin dynamics in non-collinear antiferromagnet is proposed. Taking Mn$_3$Sn as a representative example, we derive an effective low energy model based on the multipole expansion of the magnetic…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Takuya Nomoto , Ryotaro Arita

We demonstrate, based on low-temperature scanning tunneling microscopy (STM) and spectroscopy, a pronounced negative differential resistance (NDR) in spin-crossover (SCO) molecular devices, where a Fe$^{\text{II}}$ SCO molecule is deposited…

To develop new devices based on synthetic ferrimagnetic heterostructures, understanding the material's physical properties is pivotal. Here, the induced magnetic moment (IMM), magnetic exchange coupling, and spin textures are investigated…

Dynamical mean-field theory is used to study the three orbital model of the $d^3$ compound SrRu$_2$O$_6$ both with and without explicitly including the O-$p$ states. Depending on the size of the Hund's coupling $J$, at low to intermediate…

Strongly Correlated Electrons · Physics 2017-11-01 Atsushi Hariki , Andreas Hausoel , Giorgio Sangiovanni , Jan Kuneš

We perform a comprehensive theoretical study of the pressure-induced evolution of the electronic structure, magnetic state, and phase stability of the late transition metal monoxides MnO, FeO, CoO, and NiO using a fully charge…

Strongly Correlated Electrons · Physics 2020-06-22 I. Leonov , A. O. Shorikov , V. I. Anisimov , I. A. Abrikosov

We investigate abilities of various linear response based techniques for extracting parameters of antisymmetric Dzyaloshinskii-Moriya (DM) interactions from the first-principles electronic structure calculations. For these purposes, we…

Materials Science · Physics 2023-03-02 I. V. Solovyev

We propose a fast impurity solver for the general quantum impurity model based on the perturbation theory around the atomic limit, which can be used in combination with the local density approximation (LDA) and the dynamical mean field…

Strongly Correlated Electrons · Physics 2009-11-10 Xi Dai , Kristjan Haule , Gabriel Kotliar

We present a computationally efficient method to obtain the spectral function of bulk systems in the framework of steady-state density functional theory (i-DFT) using an idealized Scanning Tunneling Microscope (STM) setup. We calculate the…

Strongly Correlated Electrons · Physics 2020-11-30 David Jacob , Gianluca Stefanucci , Stefan Kurth

The investigation of magnetic energy landscapes and the search for ground states of magnetic materials using ab initio methods like density functional theory (DFT) is a challenging task. Complex interactions, such as superexchange and…

Materials Science · Physics 2024-12-24 Jakob Baumsteiger , Lorenzo Celiberti , Patrick Rinke , Milica Todorović , Cesare Franchini

It is proposed a novel method of the spectrally selective detection of the short spin waves (or magnons) by means of the transverse magneto-optical (MO) intensity effect in transmission in the magnetoplasmonic nanostructure. The method is…

Optics · Physics 2021-05-07 Olga V. Borovkova , Savelii V. Lutsenko , Andrey N. Kalish

Various methods going beyond density-functional theory (DFT), such as DFT+U, hybrid functionals, meta-GGAs, GW, and DFT-embedded dynamical mean field theory (eDMFT), have been developed to describe the electronic structure of correlated…

Strongly Correlated Electrons · Physics 2020-07-16 Subhasish Mandal , Kristjan Haule , Karin M. Rabe , David Vanderbilt

Multi-center transition metal complexes (MCTMs) with magnetically interacting ions have been proposed as components for information processing devices and storage units. For any practical application of MCTMs as magnetic units, it is…

Chemical Physics · Physics 2023-04-03 Henry C. Fitzhugh , James W. Furness , Mark R. Pederson , Juan E. Peralta , Jianwei Sun

The interaction between electronic and nuclear spins in the presence of external magnetic fields can be described by a spin Hamiltonian, with parameters obtained from first principles, electronic structure calculations. We describe an…

Materials Science · Physics 2019-04-10 Krishnendu Ghosh , He Ma , Vikram Gavini , Giulia Galli

We employ density-functional theory (DFT) in the generalized gradient approximation (GGA) and its extensions GGA+$U$ and GGA+Gutzwiller to calculate the magnetic exchange couplings between pairs of Mn ions substituting Cd in a CdTe crystal…

Strongly Correlated Electrons · Physics 2017-02-01 Thorben Linneweber , Jörg Bünemann , Ute Löw , Florian Gebhard , Frithjof Anders

The combination of density functional theory with dynamical mean-field theory (DFT+DMFT) has become a powerful first-principles approach to tackle strongly correlated materials in condensed matter physics. The wide use of this approach…

Strongly Correlated Electrons · Physics 2022-05-10 Xin Qu , Peng Xu , Rusong Li , Gang Li , Lixin He , Xinguo Ren

Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White