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Semiconductor surfaces with narrow surface bands provide unique playgrounds to search for Mott-insulating state. Recently, a combined experimental and theoretical study [Phys. Rev. Lett. 114, 247602 (2015)] of the two-dimensional (2D) Sn…

Materials Science · Physics 2016-01-18 Seho Yi , Hunpyo Lee , Jin-Ho Choi , Jun-Hyung Cho

This is a summary of a central argument in recent review articles by the author (cond-mat/0109419, cond-mat/0211005, and cond-mat/0211027). An effective field theory is derived for the low energy spin singlet excitations in a paramagnetic…

Strongly Correlated Electrons · Physics 2009-11-10 Subir Sachdev

It is well-known experimentally that the positively-charged muon and the muonium atom may bind to molecules and solids, and through muon$'$s magnetic interaction with unpaired electrons, valuable information on the local environment…

Chemical Physics · Physics 2022-01-25 Mohammad Goli , Shant Shahbazian

Spin-density-functional theory (SDFT) is the most widely implemented and applied formulation of density-functional theory. However, it is still finding novel applications, and occasionally encounters unexpected problems. In this paper we…

Materials Science · Physics 2015-06-25 K. Capelle , Valter L. Libero

DFT+U is a widely used treatment in the density functional theory (DFT) to deal with correlated materials that contain open-shell elements, whereby the quantitative and sometimes even qualitative failures of local and semilocal…

Computational Physics · Physics 2024-02-09 Zhendong Cao , Guanghui Cai , Fankai Xie , Huaxian Jia , Wei Liu , Yaxian Wang , Feng Liu , Xinguo Ren , Sheng Meng , Miao Liu

According to the Hohenberg-Kohn theorem of density-functional theory (DFT), all observable quantities of systems of interacting electrons can be expressed as functionals of the ground-state density. This includes, in principle, the spin…

Strongly Correlated Electrons · Physics 2019-09-04 Carsten A. Ullrich

We study the nature of spin excitations of individual transition metal atoms (Ti, V, Cr, Mn, Fe, Co and Ni) deposited on a Cu$_2$N/Cu(100) surface using both spin-polarized density functional theory (DFT) and exact diagonalization of an…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Alejandro Ferrón , Jose Luis Lado , Joaquín Fernández-Rossier

Nuclear Magnetic Resonance (NMR) shielding constants of transition metals in solvated complexes are computed at the relativistic density functional theory (DFT) level. The solvent effects evaluated with subsystem-DFT approaches are compared…

Chemical Physics · Physics 2021-08-09 Malgorzata Olejniczak , Andrej Antusek , Michal Jaszunski

We present a first-principles investigation of the structural, electronic, and magnetic properties of pyrolusite ($\beta$-MnO$_2$) using conventional and extended Hubbard-corrected density-functional theory (DFT+$U$ and DFT+$U$+$V$). The…

Materials Science · Physics 2021-10-06 Ruchika Mahajan , Iurii Timrov , Nicola Marzari , Arti Kashyap

We investigate the mechanism behind the breakdown of the compensation of large magnetic moments leading to weak ferromagnetism. For this we use first-principles calculations within density functional theory and we focus on the weak…

Other Condensed Matter · Physics 2007-05-23 Robert Laskowski , Gilles Santi

Dynamical mean-field theory (DMFT) is a non-perturbative technique for the investigation of correlated electron systems. Its combination with the local density approximation (LDA) has recently led to a material-specific computational scheme…

Strongly Correlated Electrons · Physics 2009-11-10 D. Vollhardt , K. Held , G. Keller , R. Bulla , Th. Pruschke , I. A. Nekrasov , V. I. Anisimov

The dynamical and thermodynamic phase stabilities of the stoichiometric compound CrN including different structural and magnetic configurations are comprehensively investigated using a first-principles density-functional-theory (DFT) plus U…

VO2 is renowned for its electric transition from an insulating monoclinic (M1) phase characterized by V-V dimerized structures, to a metallic rutile (R) phase above 340 Kelvin. This transition is accompanied by a magnetic change: the M1…

Materials Science · Physics 2023-10-10 Yubo Zhang , Da Ke , Junxiong Wu , Chutong Zhang , Baichen Lin , Zuhuang Chen , John P. Perdew , Jianwei Sun

The low-energy dynamical optical response of dimerized and undimerized spin liquid states in a one-dimensional charge transfer Mott insulator is theoretically studied. An exact analysis is given for the low-energy asymptotic behavior using…

Strongly Correlated Electrons · Physics 2009-10-23 Hosho Katsura , Masahiro Sato , Takashi Furuta , Naoto Nagaosa

We studied several aspects of the Mott metal-insulator transition in the disordered case. The model on which we based our analysis is the disordered Hubbard model, which is the simplest model capable of capturing the Mott metal-insulator…

Strongly Correlated Electrons · Physics 2020-07-01 M. Y. Suárez-Villagrán , N. Mitsakos , Tsung-Han Lee , V. Dobrosavljević , J. H. Miller, , E. Miranda

A microscopic control over the origin and dynamics of localised spin centres in lower dimensional solids turns out to be a key factor for next generation spintronics and quantum technologies. With the help of low temperature electron…

Materials Science · Physics 2023-12-29 Sudipta Khamrui , Kamini Bharti , Daniella Goldfarb , Tilak Das , Debamalya Banerjee

While density functional theory (DFT) is widely applied for its combination of cost and accuracy, corrections (e.g., DFT+U) that improve it are often needed to tackle correlated transition-metal chemistry. In principle, the functional form…

Chemical Physics · Physics 2021-03-12 Akash Bajaj , Heather J. Kulik

We present an ab initio investigation of magnetic exchange interactions using the spin-spiral method implemented in the VASP code, with a comparative analysis of the self-consistent (SC) and magnetic force theorem (MFT) approaches. Using…

Materials Science · Physics 2025-10-30 Umit Dogan Daglum , Maria Stamenova , Ersoy Sasioglu , Stefano Sanvito

Time-dependent spin density functional theory (TD-SDFT) allows the theoretical description of spin and magnetization dynamics in electronic systems from first quantum mechanical principles. TD-SDFT accounts for electronic interaction…

Materials Science · Physics 2024-10-04 Jenna L. Bologa , Carsten A. Ullrich

We address the nature of the Mott transition in the Hubbard model at half-filling using cluster Dynamical Mean Field Theory (DMFT). We compare cluster DMFT results with those of single site DMFT. We show that inclusion of the short range…

Strongly Correlated Electrons · Physics 2009-11-13 H. Park , K. Haule , G. Kotliar
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