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Barium zirconate BaZrO3 is one of few perovskites that is claimed to retain an average cubic structure down to 0K at ambient pressure, while being energetically very close to a tetragonal phase obtained by condensation of a soft phonon mode…

Materials Science · Physics 2024-03-22 Erik Fransson , Petter Rosander , Paul Erhart , Göran Wahnström

Density functional perturbation theory calculations of alpha-quartz using extended norm conserving pseudopotentials have been used to study the elastic properties and phonon dispersion relations along various high symmetry directions as a…

Materials Science · Physics 2007-05-23 N. Choudhury , S. L. Chaplot

We compute lattice dynamical properties of iron at the bcc-fcc phase transition using dynamical mean-field theory implemented with the frozen-phonon method. Electronic correlations are found to have a strong effect on the lattice stability…

Materials Science · Physics 2015-05-30 I. Leonov , A. I. Poteryaev , V. I. Anisimov , D. Vollhardt

Problems of heat transport are ubiquitous to various technologies such as power generation, cooling, electronics, and thermoelectrics. In this paper we advocate for the application of the quantum self-consistent reservoir method, which is…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Roya Moghaddasi Fereidani , Dvira Segal

A comprehensive, critical study of the vibrational, thermodynamic and thermoelastic properties of bcc iron is presented, using well established semi-empirical embedded-atom method potentials available in the literature. Classical molecular…

Materials Science · Physics 2018-05-18 Daniele Dragoni , Davide Ceresoli , Nicola Marzari

We measured phonon dispersion in single crystal EuTiO$_3$ using inelastic x-ray scattering. A structural transition to an antiferrodistortive phase was found at a critical temperature $T_0$=287$\pm$1 K using powder and single-crystal x-ray…

Strongly Correlated Electrons · Physics 2015-06-11 David S. Ellis , Hiroshi Uchiyama , Satoshi Tsutsui , Kunihisa Sugimoto , Kenichi Kato , Daisuke Ishikawa , Alfred Q. R. Baron

Experimental phonon imaging in diamond anvils cell is demonstrated to be an adequate tool to extract the complete set of elastic constants of single-crystalline silicon up to the ZB$\rightarrow \beta-$Sn transition (10 GPa). Contrary to…

Materials Science · Physics 2015-05-19 F. Decremps , L. Belliard , M. Gauthier , B. Perrin

On the basis of the self-consistent phonon theory and the special displacement method, we develop an approach for the treatment of anharmonicity in solids. We show that this approach enables the efficient calculation of…

Materials Science · Physics 2023-08-09 Marios Zacharias , George Volonakis , Feliciano Giustino , Jacky Even

An analytical model of high frequency oscillations of the kinetic and potential energies in a one-dimensional harmonic crystal with a substrate potential is obtained by introducing the nonlocal energies [1]. A generalization of the kinetic…

Statistical Mechanics · Physics 2018-02-07 Mikhail B. Babenkov , Anton M. Krivtsov , Denis V. Tsvetkov

We consider two high-frequency thermal processes in uniformly heated harmonic crystals relaxing towards equilibrium: (i) equilibration of kinetic and potential energies and (ii) redistribution of energy among spatial directions. Equation…

Statistical Mechanics · Physics 2017-08-01 Vitaly A. Kuzkin , Anton M. Krivtsov

We report neutron inelastic scattering on single crystal 0.68Pb(Mg1/3Nb2/3O3)-0.32PbTiO3 (PMN-0.32PT), a relaxor ferroelectric material that lies within the compositional range of the morphotropic phase boundary (MPB). Data were obtained…

Materials Science · Physics 2009-11-13 Hu Cao , Chris Stock , Guangyong Xu , Peter M. Gehring , Jiefang Li , Dwight Viehland

In the warm dense regime, where the electron temperature is increased to the same order of the Fermi temperature, the dynamical stability of elemental metals depends on its electronic band structure as well as its crystal structure. It has…

Materials Science · Physics 2021-03-31 Shota Ono , Daigo Kobayashi

Phonon frequency moments and thermodynamic functions (electrostatic and vibrational parts of the free energy, internal energy, and heat capacity) are calculated for bcc and fcc Coulomb crystals in the harmonic approximation with a…

Plasma Physics · Physics 2009-11-07 D. A. Baiko , A. Y. Potekhin , D. G. Yakovlev

The phonon dispersion and the electron-phonon interaction for the $\beta$-Po and the bcc high pressure phases of tellurium are computed with density-functional perturbation theory. Our calculations reproduce and explain the experimentally…

Thermal resonance, in which the temperature amplitude attains a maximum value (peak) in response to an external exciting frequency source, is a phenomenon pertinent to the presence of underdamped thermal oscillations and explicit…

Materials Science · Physics 2024-07-22 Emad Awad , Weizhong Dai , Sergey Sobolev

The lattice thermal conductivity (LTC) of ZrSe$_2$, a typical layered transition metal disulfide, has been calculated using a hybrid approach that combines force field molecular dynamics (MD) simulation and Boltzmann transport equation…

Materials Science · Physics 2025-09-10 Yong Lu , Fawei Zheng

The properties of crystals consisting of several components can be widely tuned. Often solid solutions are produced, where substitutional or interstitional disorder determines the crystal thermodynamic and mechanical properties. The…

Soft Condensed Matter · Physics 2019-10-30 Tadeus Ras , Michael Szafarczyk , Matthias Fuchs

The structural phase behaviors of pure zirconium metal under compressions up to $160$ GPa at room temperature are investigated from the perspective of ensemble theory where the partition function is solved by our recently proposed method…

Materials Science · Physics 2022-10-21 Bo-Yuan Ning

Phonons play a critical role in determining various material properties, but conventional methods for phonon calculations are computationally intensive, limiting their broad applicability. In this study, we present an approach to accelerate…

Materials Science · Physics 2024-07-16 Huiju Lee , Vinay I. Hegde , Chris Wolverton , Yi Xia

Modern advances in generating ultrabright electron beams have unlocked unprecedented experimental advances based on synchrotron radiation. Current challenges lie in improving the quality of electron sources with novel photocathode materials…

Materials Science · Physics 2024-02-27 Julia Santana-Andreo , Holger-Dietrich Saßnick , Caterina Cocchi