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An efficient broadband sum frequency generation (SFG) technique using the two collinear optical parametric processes \omega 3=\omega 1+\omega 2 and \omega 4=\omega 1+\omega 3 is proposed. The technique uses chirped quasi-phase-matched…

Optics · Physics 2015-06-03 A. A. Rangelov , N. V. Vitanov

Sum frequency generation (SFG) has multiple applications, from optical sources to imaging, where efficient conversion requires either long interaction distances or large field concentrations in a quadratic nonlinear material. Metasurfaces…

Optics · Physics 2024-08-22 Neuton Li , Jihua Zhang , Dragomir N. Neshev , Andrey A. Sukhorukov

We introduce sum-frequency generation (SFG) as an effective physical two-photon detector for high power two-mode squeezed coherent states with arbitrary frequency separation, as produced by parametric oscillators well above the threshold.…

Optics · Physics 2013-10-30 Faina Shikerman , Avi Pe'er

Plasmonic nanostructures that support surface plasmon (SP) resonance potentially provide a route for the development of nanoengineered nonlinear optical devices. In this work, second-order nonlinear light scattering, specifically…

Computational Physics · Physics 2016-12-20 Xiaoyan Y. Z. Xiong , Li Jun Jiang , Wei E. I. Sha , Yat Hei Lo , Weng Cho Chew

The miniaturization of nonlinear light sources is central to the integrated photonic platform, driving a quest for high-efficiency frequency generation and mixing at the nanoscale. In this quest, the high-quality ($Q$) resonant dielectric…

Optics · Physics 2023-11-14 Siqi Feng , Tingting Liu , Wenya Chen , Feng Wu , Shuyuan Xiao

Sum-frequency generation (SFG) is a powerful second-order nonlinear spectroscopic technique that provides detailed insights into molecular structures and absolute orientations at surfaces and interfaces. However, conventional SFG based on…

We propose a computational framework to extract non-linear response functions from real-time simulations in the presence of more than one external field. We apply this approach to the calculation of sum frequency generation (SFG) and…

Materials Science · Physics 2025-11-19 Mike N. Pionteck , Myrta Grüning , Simone Sanna , Claudio Attaccalite

We propose and experimentally demonstrate a scheme allowing to reach noncollinear phase-matching of high harmonic generation in solids, which may potentially lead to an enhancement of the generation efficiency. The principle is based on…

Optics · Physics 2026-02-24 Pavel Peterka , František Trojánek , Petr Malý , Martin Kozák

Vibrational sum frequency generation (SFG) is a nonlinear spectroscopic technique widely used to study the molecular structure and dynamics of surface systems. However, the spatial resolution achieved by far-field observations is…

We investigate the up-conversion process of broadband light from parametric down-conversion (PDC), focusing on the spatio-temporal spectral properties of the sum-frequency generated (SFG) radiation. We demonstrate that the incoherent…

Sum-frequency generation (SFG) is a second-order nonlinear process widely used for characterizing surfaces and interfaces with monolayer sensitivity. Recently, optical field enhancement in plasmonic nanocavities has enabled SFG with…

We report on the experimental observation of non-resonant, second-order optical Sum-Frequency Generation (SFG) in five different atomic and molecular gases. The measured signal is attributed to a SFG process by characterizing its intensity…

Sum-frequency generation (SFG) allows for coherent upconversion of an electromagnetic signal and has applications in mid-infrared vibrational spectroscopy of molecules. Recent experimental and theoretical studies have shown that plasmonic…

We investigate the up-conversion process of broadband light from parametric down-conversion (PDC), focusing on the spatio-temporal spectral properties of the sum-frequency generated (SFG) radiation. We demonstrate that the incoherent…

Quantum Physics · Physics 2013-08-13 E. Brambilla , O. Jedrkiewicz , P. Di Trapani , A. Gatti

Phase-mismatch in nonlinear optical processes can severely limit the propagation and conversion efficiency of light fields. Here, we present an efficient optimal-control strategy to mitigate the detrimental effects of phase-mismatch in an…

Quantum Physics · Physics 2025-09-17 Ning Jia , Hamid R. Hamedi , Jing Qian

Sum-frequency generation (SFG) spectroscopy provides a versatile method for the investigation of non-centrosymmetric media and interfaces. Here, using tunable picosecond infrared (IR) pulses from a free-electron laser, the nonlinear optical…

Materials Science · Physics 2023-08-01 Riko Kiessling , Martin Wolf , Alexander Paarmann

Nonlinear-optical microscopy and spectroscopy provide detailed spatial and spectroscopic contrast, specifically sensitive to structural symmetry and order. Ferroics, in particular, have been widely studied using second harmonic generation…

We demonstrate sum-frequency generation in a nonlinear whispering gallery mode resonator between a telecom wavelength and the Rb D2 line, achieved through natural phase matching. Due to the strong optical field confinement and ultra high Q…

Optics · Physics 2015-06-15 Dmitry V. Strekalov , Abijith S. Kowligy , Yu-Ping Huang , Prem Kumar

Vibrational sum frequency generation (SFG) spectroscopy is a powerful technique for investigating molecular structures, orientations, and dynamics at surfaces. However, its spatial resolution is fundamentally restricted to the micrometer…

Multimode quantum light has promising applications in many areas of physics, such as quantum communications and quantum computing. However, its multimode nature also makes it challenging to measure its properties. Recently [Optica Quantum…

Quantum Physics · Physics 2025-04-29 D. Scharwald , P. R. Sharapova
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