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We experimentally demonstrate sum-frequency generation (SFG) with entangled photon-pairs, generating as many as 40,000 SFG photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a…

Quantum Physics · Physics 2007-05-23 Barak Dayan , Avi pe'er , Asher A. Friesem , Yaron Silberberg

Tailoring spectral properties of photon pairs is of great importance for optical quantum information and measurement applications. High-resolution spectral measurement is a key technique for engineering spectral properties of photons,…

Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes…

The effects of group and phase velocity mismatch are well-known in optical harmonic generation, but the non-degenerate cases remain unexplored. In this work we develop an analytic model which predicts velocity mismatch effects in…

Optics · Physics 2018-01-03 Darien J. Morrow , Daniel D. Kohler , John C. Wright

We propose cascaded spontaneous four-wave mixing (SFWM) in microring resonators as a scalable and efficient approach for directly generating non-Gaussian states of light. Focusing on the well-understood "low-gain" regime, we demonstrate…

Quantum Physics · Physics 2026-02-27 Samuel E. Fontaine , J. E. Sipe , Marco Liscidini , Milica Banic

Triple sum-frequency (TSF) spectroscopy is a recently-developed methodology that enables collection of multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. This work reports the…

Optics · Physics 2018-08-23 Darien J. Morrow , Daniel D. Kohler , Kyle J. Czech , John C. Wright

Light beams with extraordinary spatial structures, such as the Airy beam (AB), the Bessel-Gaussian beam (BGB) and the Laguerre-Gaussian beam (LGB), are widely studied and applied in many optical scenarios. We report on preparation of light…

High-quality crystals without inversion symmetry are the conventional platform to achieve optical frequency conversion via three wave-mixing. In bulk crystals, efficient wave-mixing relies on phase-matching configurations, while at the…

High harmonic generation is a resource of extremely broad frequency combs of ultrashort light pulses. The non-classical nature of this new quantum source has been recently evidenced in semiconductors by showing that high harmonic generation…

The optical nonlinear effects can provide different advanced electromagnetic functionalities, such as wave mixing and phase conjugation, which can be applied in a variety of new applications. However, these effects usually suffer from…

Optics · Physics 2020-06-29 Boyuan Jin , Christos Argyropoulos

Boosting nonlinear frequency conversion in extremely confined volumes remains a key challenge in nano-optics, nanomedicine, photocatalysis, and background-free biosensing. To this aim, field enhancements in plasmonic nanostructures are…

We demonstrate the double electromagnetically induced transparency (double-EIT) and double four-wave mixing (double-FWM) based on a new scheme of non-degenerate four-wave mixing (FWM) involving five levels of a cold 85Rb atomic ensemble, in…

Optics · Physics 2015-06-05 Yang Liu , Jing-Hui Wu , Dong-Sheng Ding , Bao-Sen Shi , Guang-Can Guo

We demonstrate supermode-based second harmonic generation in an integrated nonlinear interferometer made of linear and nonlinear directional couplers. We use a fully-fibered pump shaper to demonstrate second harmonic generation pumped by…

Exploration of optical non-linear response of graphene predominantly relies on ultra-short time domain measurements. Here we propose an alternate technique that uses frequency modulated continuous wavefront optical fields, thereby probing…

Mesoscale and Nanoscale Physics · Physics 2019-03-18 Ashutosh Singh , Saikat Ghosh , Amit Agarwal

Efficient nonlinear frequency conversion in nanophotonics requires not only strong fundamental field but also precise phase matching among distributed nonlinear sources. Here, we develop the two-dimensional Green's function integral method…

Optics · Physics 2025-12-23 Chengkang Liang , Quanying Li , Jiale Xu , Pingqi Gao , Jiancan Yu

Vibrational sum- and difference-frequency generation (SFG and DFG) spectroscopy probes the nonlinear response of interfaces at mid-infrared (MIR) wavelengths while detecting upconverted signals in the visible. Recent work has moved from…

Nonlinear interferometers are promising tools for quantum metrology, as they are characterized by an improved phase sensitivity scaling compared to linear interferometers operating with classical light. However, the multimodeness of the…

Quantum Physics · Physics 2023-11-28 D. Scharwald , T. Meier , P. R. Sharapova

Much work over the last 25 years has demonstrated that the interface-specific, alloptical technique, vibrational sum frequency generation (v-SFG) spectroscopy, is often uniquely capable of characterizing the structure and dynamics of…

Optics · Physics 2018-11-14 Martin Thämer , R. Kramer Campen , Martin Wolf

Capabilities of quantum optical SFG-gate seeded by squeezed light are investigated in the frame of frequency Schmidt modes. Methods to manage and manipulate extensively the properties and mode content of squeezed light are developed.…

Quantum Physics · Physics 2020-12-30 Vladislav Sukharnikov , Polina Sharapova , Olga Tikhonova

The efficient creation and detection of spatial modes of light has become topical of late, driven by the need to increase photon-bit-rates in classical and quantum communications. Such mode creation/detection is traditionally achieved with…