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Related papers: Adsorption of CO on the Ca3Ru2O7(001) surface

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Adsorption of CO at the Sr$_3$Ru$_2$O$_7$(001) surface was studied with low-temperature scanning tunneling microscopy (STM) and density functional theory. In situ cleaved single crystals terminate in an almost perfect SrO surface. At 78 K,…

The interaction of CO with the Fe3O4(001)-(rt2xrt2)R45{\deg} surface was studied using temperature programmed desorption (TPD), scanning tunneling microscopy (STM) and x-ray photoelectron spectroscopy (XPS), the latter both under ultrahigh…

Chemisorption of CO on the stepped Cu(211) surface is studied within ab-initio density functional theory (DFT) and scanning tunneling microscopy (STM) imaging as well as manipulation experiments. Theoretically we focus on the experimentally…

Materials Science · Physics 2009-11-10 Marek Gajdos , Andreas Eichler , Jurgen Hafner , Gerhard Meyer , Karl-Heinz Rieder

We characterized CO2 adsorption and diffusion on the missing row reconstructed Cu(100)-O surface using a combination of scanning tunneling microscopy (STM) and density functional theory (DFT) calculations with dispersion. We deposited CO2…

Mesoscale and Nanoscale Physics · Physics 2020-07-14 Steven J. Tjung , Qiang Zhang , Jacob J. Repicky , Simuck F. Yuk , Xiaowa Nie , Nancy M. Santagata , Aravind Asthagiri , Jay A. Gupta

Using first-principles calculations, we systematically study the adsorption behaviors of molecular CO on the Be (0001) surface. By calculating the potential energy surfaces, we find that CO molecularly adsorbs on the Be surface with small…

Materials Science · Physics 2015-05-13 Shuang-Xi Wang , Yu Yang , Bo Sun , Rong-Wu Li , Shao-Jun Liu , Ping Zhang

CO adsorption on Cu(111) and Cu(001) surfaces has been studied within ab-initio density functional theory (DFT). The structural, vibrational and thermodynamic properties of the adsorbate-substrate complex have been calculated. Calculations…

Materials Science · Physics 2009-11-10 M. Gajdos , J. Hafner

Using density functional theory and an exchange-correlationfunctional that includes the van der Waals interaction, we study the coadsorption of CO on Ru(0001) saturated with 0.5 ML of oxygen. Different coexisting CO coverages are considered…

Materials Science · Physics 2021-06-09 Auguste Tetenoire , J. Iñaki Juaristi , Maite Alducin

Knowledge of the atomic geometry of a surface is a prerequisite for any detailed understanding of the surface's electronic structure and chemical properties. Previous studies have convincingly demonstrated that density functional theory…

Materials Science · Physics 2007-05-23 C. Stampfl , M. Scheffler

Our ab initio calculations of CO adsorption on several low and high miller index surfaces of Cu show that the adsorption energy increases as the coordination of the adsorption site decreases from 11 to 6, in qualitative agreement with…

Materials Science · Physics 2013-05-29 Faisal Mehmood , Abdelkader Kara , Talat S. Rahman , Klaus Peter Bohnen

We present and discuss the results of ab initio DFT plane-wave supercell calculations of the atomic and molecular oxygen adsorption and diffusion on the LaMnO3 (001) surface which serves as a model material for a cathode of solid oxide fuel…

Materials Science · Physics 2008-02-04 Eugene A. Kotomin , Yuri A. Mastrikov , Eugene Heifets , Joachim Maier

We investigate the adsorption of cobalt phthalocyanine (CoPc) molecules on a thin layer of cobalt oxide grown on Ir(100). To that end we compare the results of low-temperature scanning tunneling microscopy (STM) with those of ab-initio…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Tobias Schmitt , Pascal Ferstl , Lutz Hammer , M. Alexander Schneider , Josef Redinger

Only recently, the activation of oxygen molecules on clean defect-free transition metal oxide surfaces has been reported, for example on the CaO-terminated surface of the Ruddelsden-Popper perovskite \crosurf. In this work we show that…

Materials Science · Physics 2018-10-10 Wernfried Mayr-Schmölzer , Florian Mittendorfer , Josef Redinger

The adsorption of $CO_2$ on the $Fe_3$$O_4$(001)-($\sqrt{2}$ $\times$ $\sqrt{2}$)R45{\deg} surface was studied experimentally using temperature programmed desorption (TPD), electron spectroscopies (UPS and XPS), and scanning tunneling…

Nowadays, electrochemical reduction of CO$_2$ has been considered as an effective method to solve the problem of global warming. The primary challenge in studying the mechanism is to determine the adsorption states of CO$_2$, since…

Chemical Physics · Physics 2020-07-03 Shuai Guo , Yao Li , Lei Liu , Xiangping Zhang , Suojiang Zhang

Using first-principles calculations, we systematically study the adsorption behavior of a single molecular H$_{2}$O on the Be(0001) surface. We find that the favored molecular adsorption site is the top site with an adsorption energy of…

Materials Science · Physics 2015-05-27 Shuang-Xi Wang , Peng Zhang , Jian Zhao , Shu-Shen Li , Ping Zhang

While the small sticking coefficient for molecular hydrogen on the Si(001) surface apparently requires a large energy barrier of adsorption, no such barrier is observed in desorption experiments. We have calculated the potential-energy…

mtrl-th · Physics 2009-10-28 E. Pehlke , M. Scheffler

In$_2$O$_3$-based catalysts have shown high activity and selectivity for CO$_2$ hydrogenation to methanol, however the origin of the high performance of In$_2$O$_3$ is still unclear. To elucidate the initial steps of CO$_2$ hydrogenation…

Polaron formation plays a major role in determining the structural, electrical and chemical properties of ionic crystals. Using a combination of first principles calculations and scanning tunneling microscpoy/atomic force microscopy…

The structure of CO adsorbates on the Rh(110) surface is studied at full coverage using first-principles techniques. The relative energies of different adsorbate geometries are determined by means of accurate structure optimizations. In…

Materials Science · Physics 2009-10-28 Dario Alfe' , Stefano Baroni

Understanding how the local environment of a single-atom catalyst affects stability and reactivity remains a significant challenge. We present an in-depth study of Cu1, Ag1, Au1, Ni1, Pd1, Pt1, Rh1, and Ir1 species on Fe3O4(001); a model…

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