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The importance of many-body effects on electronic and magnetic properties and stability of different structural phases was studied in novel iron oxide - Fe$_2$O. It was found that while Hubbard repulsion hardly affects the electronic…

Strongly Correlated Electrons · Physics 2022-06-08 Alexey O. Shorikov , Sergey V. Streltsov

Rapidly developing science and technology demand new materials with versatile and promising properties for practical applications. In this context, pseudo-octahedral iron(II) spin crossover (SCO) complexes are particularly appealing - not…

In this paper we study, both with theoretical and experimental approach, the effect of iron doping in zirconia. Combining density functional theory (DFT) simulations with the experimental characterization of thin films, we show that iron is…

The electronic and magnetic properties of Fe atoms in the ferromagnetic semiconductor (In,Fe)As codoped with Be have been studied by x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD) at the Fe $L_{2,3}$ edge.…

Transition-metal ions with $5d^2$ electronic configuration in a cubic crystal field are prone to have a vanishing dipolar magnetic moment but finite higher-order multipolar moments, and they are expected to exhibit exotic physical…

Strongly Correlated Electrons · Physics 2025-07-16 J. Okamoto , G. Shibata , Yu. S. Posonov , H. Hayashi , K. Yamaura , H. Y. Huang , A. Singh , C. T. Chen , A. Tanaka , S. V. Streltsov , D. J. Huang , A. Fujimori

We report a Fe K\beta x-ray emission spectroscopy study of local magnetic moments in the rare-earth doped iron pnictide Ca_{1-x}RE_xFe_2As_2 (RE=La, Pr, and Nd). In all samples studied the size of the Fe local moment is found to decrease…

Superconductivity · Physics 2013-01-28 H. Gretarsson , S. R. Saha , T. Drye , J. Paglione , Jungho Kim , D. Casa , T. Gog , W. Wu , S. R. Julian , Young-June Kim

The insulating iron compounds Eu$_2$SrFe$_2$O$_6$ and Sr$_3$Fe$_2$O$_4$Cl$_2$ have high-temperature antiferromagnetic (AF) order despite their different layered structures. Here we carry out density functional calculations and Monte Carlo…

Strongly Correlated Electrons · Physics 2022-08-18 Di Lu , Ke Yang , Lu Liu , Guangyu Wang , Hua Wu

One of the key factors behind the rapid evolution of molecular spintronics is the efficient realization of spin manipulation of organic molecules with a magnetic center. The spin state of such molecules may depend crucially on the…

The spin-orbit entangled (SOE) Jeff-state has been a fertile ground to study novel quantum phenomena. Contrary to the conventional weakly correlated Jeff=1/2 state of 4d and 5d transition metal compounds, the ground state of CuAl2O4 hosts a…

There has been a longstanding debate whether the pyrite CoS$_2$ or its alloys with FeS$_2$ are half metallic. We argue using first principles calculations that there is a finite occupation of minority-spin states at the Fermi level…

Materials Science · Physics 2025-10-17 Anustup Mukherjee , Alaska Subedi

Resistivity and dc magnetization measurements were performed for the polycrystalline Pr$_{0.5}$Ca$_{0.5}$Co$_{1-x}$Fe$_{x}$O$_{3-\delta}$ ($x$ = 0, 0.05, 0.10 and 0.15) samples. The as-fabricated samples exhibit ferromagnetic (FM)…

Strongly Correlated Electrons · Physics 2009-11-11 X. G. Luo , X. Li , G. Y. Wang , G. Wu , X. H. Chen

We study the spin-crossover molecule Fe(phen)$_2$(NCS)$_2$ using density functional theory (DFT) plus dynamical mean-field theory, which allows access to observables not attainable with traditional quantum chemical or electronic structure…

Materials Science · Physics 2015-06-30 Jia Chen , Andrew Millis , Chris Marianetti

The structural, electronic and magnetic properties of Fe7S8 material have been studied within the framework of the ab-initio calculations, the mean field approximation (MFA) and Monte Carlo simulation (MCS). Our study shows that two forms…

Materials Science · Physics 2020-12-09 S. Benyoussef , Y. EL Amraoui , H. Ez-Zahraouy , D. Mezzane , Z. Kutnjak , I. A. Luk'yanchuk , M. EL Marssi

The mysterious second order quantum phase transition, commonly attributed to the `hidden-order' (HO) state, in heavy-fermion metal URu2Si2 exhibits a number of paradoxical electronic and magnetic properties which cannot be associated with…

Strongly Correlated Electrons · Physics 2014-02-18 Tanmoy Das

We have used muon-spin rotation, heat capacity and x-ray diffraction measurements in combination with density functional theory and dipole field calculations to investigate the crystal and magnetic structure of FeTi$_2$O$_5$. We observe a…

Strongly Correlated Electrons · Physics 2019-09-11 Franz Lang , Lydia Jowitt , Dharmalingam Prabhakaran , Roger D. Johnson , Stephen J. Blundell

Using {\it ab initio} molecular dynamics we investigate the electronic and lattice structure of $A$Fe$_2$As$_2$ ($A$=Ca, Sr, Ba) under pressure. We find that the structural phase transition (orthorhombic to tetragonal symmetry) is always…

Superconductivity · Physics 2009-10-13 Yu-Zhong Zhang , Hem C. Kandpal , Ingo Opahle , Harald O. Jeschke , Roser Valenti

Context. The intensity profiles of iron and oxygen in Solar Energetic Particle (SEP) events often display differences that result in a decreasing Fe/O ratio over time. The physical mechanisms behind this behaviour are not fully understood,…

Solar and Stellar Astrophysics · Physics 2017-02-08 S. Dalla , M. S. Marsh , P. Zelina , T. Laitinen

The doping series Eu1-xCaxCoO3-d provides a rather peculiar way to study the spin-state transition in cobalt-based complex oxides since partial substitution of Eu3+ ions by Ca2+ ions does not increase the mean valence state of cobalt but is…

RuO$_{2}$ has been proposed as the prototypical altermagnetic material. However, several reports have recently questioned its intrinsic magnetic ordering, leading to conflicting findings, especially in thin film heterostructures pointing to…

High entropy oxides (HEOs) can possess long-range ordered magnetic states despite their extreme chemical disorder. Very little is known about how the different chemical constituents in HEOs contribute to the emergence of these magnetic…

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