Related papers: Ultrafast infrared spectroscopy with single molecu…
We have developed a single-shot imaging technique that can capture ultrafast events occurring on femtosecond to picosecond time scales. The technique is based on an optical pump-probe method, in which multiple time-delayed femtosecond…
A quantum information processor is proposed that combines experimental techniques and technology successfully demonstrated either in nuclear magnetic resonance experiments or with trapped ions. An additional inhomogenenous magnetic field…
We have developed a novel all-optical broadband scheme for exciting, amplifying and measuring the secular motion of ions in a radio frequency trap. Oscillation induced by optical excitation has been coherently amplified to precisely control…
We use quantum-logic spectroscopy (QLS) and interrogate rotational transitions of a single CaH+ ion with a highly coherent frequency comb, achieving a fractional statistical uncertainty for a transition line center of 4 x 10^-13. We also…
We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…
We present a detailed method for accumulating Ca$^{+}$ ions controllably in a linear Paul trap. The ions are generated by pulsed laser ablation and dynamically loaded into the ion trap by switching the trapping potential on and off. The…
Tunnel ionization of room-temperature D$_2$ in an ultrashort (12 femtosecond) near infra-red (800 nm) pump laser pulse excites a vibrational wavepacket in the D2+ ions; a rotational wavepacket is also excited in residual D2 molecules. Both…
A single-ion reservoir has been tested, and characterized in order to be used as a highly sensitive optical detector of electric signals arriving at the trapping electrodes. Our system consists of a single laser-cooled $^{40}$Ca$^+$ ion…
The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…
We trap absorbing micro-particles in air by photophoretic forces generated using a single loosely focused Gaussian trapping beam. We measure a component of the radial Brownian motion of a trapped particle cluster and determine the power…
We consider pump-probe spectroscopy of a single ion with a highly metastable (probe) clock transition which is monitored by using the quantum jump technique. For a weak clock laser we obtain the well known Autler-Townes splitting. For…
Advanced techniques for manipulation of internal states, standard in atomic physics, are demonstrated for a charged molecular species for the first time. We address individual hyperfine states of ro-vibrational levels of a diatomic ion by…
An experimental demonstration of a novel all-optical technique for loading ion traps, that has particular application to microtrap architectures, is presented. The technique is based on photo-ionisation of an atomic beam created by pulsed…
We demonstrate a general method for state detection of trapped ions that can be applied to a large class of atomic and molecular species. We couple a "spectroscopy" ion (Al+) to a "control" ion (Mg+) in the same trap and perform state…
Preparing molecules at rest and in a highly pure quantum state is a long standing dream in chemistry and physics, so far achieved only for a select set of molecules in dedicated experimental setups. Here, a quantum-limited combination of…
We demonstrate the operation of a dual-frequency Paul trap and characterize its performance by storing either electrons or calcium ions while applying two quadrupole fields simultaneously which oscillate at $\Omega_\textrm{fast} = 2\pi…
A mixed-species geometric phase gate has been proposed for implementing quantum logic spectroscopy on trapped ions that combines probe and information transfer from the spectroscopy to the logic ion in a single pulse. We experimentally…
We theoretically analyze the dynamics of an atomic double-well system with a single ion trapped in its center. We find that the atomic tunnelling rate between the wells depends both on the spin of the ion via the short-range spin-dependent…
We propose a detection method for ultracold atoms which allows reconstruction of the full one-particle and two-particle correlation functions from the measurements. The method is based on Fourier sampling of the time-of-flight images…
Tremendous advances in laser pump-probe techniques open the door for the observation in real time of ultrafast \textit{electronic} processes. Particularly attractive is the visualization of interatomic processes where one can follow the…