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The crystal structure and magnetic properties of the spin-1 triangular-lattice antiferromagnet Ba$_2$La$_2$NiTe$_2$O$_{12}$ are reported. Its crystal structure is trigonal $R\bar{3}$, which is the same as that of Ba$_2$La$_2$NiW$_2$O$_{12}$…

Strongly Correlated Electrons · Physics 2019-08-28 Mutsuki Saito , Masari Watanabe , Nobuyuki Kurita , Akira Matsuo , Koichi Kindo , Maxim Avdeev , Harald O. Jeschke , Hidekazu Tanaka

Here, we report the synthesis and magnetic properties of a new triangular lattice antiferromagnet Ba$_3$CoTa$_2$O$_9$. The effective spin of Co$^{2+}$ is found to be $J=1/2$ at low temperatures due to the combined effect of crystal field…

Materials Science · Physics 2017-03-08 K. M. Ranjith , K. Brinda , U. Arjun , N. G. Hegde , R. Nath

We report a 139La-NMR study of Ba2La2CoTe2O12, S = 1/2 equilateral triangular-lattice antiferromagnet with easy-plane anisotropy at low temperatures. This compound undergoes a magnetic phase transition at TN = 3.26 K into an ordered state…

We successfully synthesized and characterized the triangular lattice anitferromagnet Ba$_8$MnNb$_6$O$_{24}$, which comprises equilateral spin-5/2 Mn$^{2+}$ triangular layers separated by six non-magnetic Nb$^{5+}$ layers. The detailed…

Materials Science · Physics 2019-06-03 R. Rawl , L. Ge , Z. Lu , Z. Evenson , C. R. Dela Cruz , Q. Huang , M. Lee , E. S. Choi , M. Mourigal , H. D. Zhou , J. Ma

We report the results of low-temperature magnetization and specific heat measurements of Sr$_3$CoTa$_2$O$_9$ powder, in which Co$^{2+}$ ions with effective spin-1/2 form a uniform triangular lattice in the $ab$ plane. It was found that…

Strongly Correlated Electrons · Physics 2023-05-24 Iori Nishizawa , Nobuyuki Kurita , Hidekazu Tanaka , Takayuki Goto

We found new two-dimensional (2D) quantum (S=1/2) antiferromagnetic systems: CuRE2Ge2O8 (RE=Y and La). According to our analysis of high-resolution X-ray and neutron diffraction experiments, the Cu-network of CuRE2Ge2O8 (RE=Y and La)…

We report the synthesis, crystal structure, and magnetic properties of two new quantum antiferromagnets A3ReO5Cl2 (A = Sr and Ba). The crystal structure is isostructural with the mineral pinalite Pb3WO5Cl2, in which the Re6+ ion is…

Strongly Correlated Electrons · Physics 2021-04-06 Daigorou Hirai , Takeshi Yajima , Kazuhiro Nawa , Mitsuaki Kawamura , Zenji Hiroi

The magnetic phases of the ideal spin-1/2 triangular-lattice antiferromagnet Ba$_3$CoSb$_2$O$_9$ are identified and studied using $^{135,137}$Ba nuclear magnetic resonance (NMR) spectroscopy in magnetic fields ranging to 30T, oriented…

Strongly Correlated Electrons · Physics 2015-01-13 G. Koutroulakis , T. Zhou , C. D. Batista , Y. Kamiya , J. D. Thompson , S. E. Brown , H. D. Zhou

Based on density functional theory band structure calculations, quantum Monte-Carlo simulations, and high-field magnetization measurements, we address the microscopic magnetic model of BaAg2Cu[VO4]2 that was recently proposed as a spin-1/2…

Materials Science · Physics 2012-06-19 Alexander A. Tsirlin , Angela Moeller , B. Lorenz , Yu. Skourski , H. Rosner

The geometrically frustrated two dimensional triangular lattice magnets A${_4}$B'B${_2}$O$_{12}$ (A = Ba, Sr, La; B' = Co, Ni, Mn; B = W, Re) have been studied by x-ray diffraction, AC and DC susceptibilities, powder neutron diffraction,…

We report the results of low-temperature thermal and magnetic measurements on Ba$_3$CoNb$_2$O$_9$ powder, described as a uniform triangular-lattice antiferromagnet (TLAF) with a fictitious spin-1/2. Ba$_3$CoNb$_2$O$_9$ is found to undergo…

Strongly Correlated Electrons · Physics 2015-06-22 Kazuya Yokota , Nobuyuki Kurita , Hidekazu Tanaka

We report the results of magnetization and specific heat measurements on Ba$_3$CoSb$_2$O$_9$, in which the magnetic Co$^{2+}$ ion has a fictitious spin-1/2, and show evidence that a spin-1/2 Heisenberg antiferromagnet on a regular…

Strongly Correlated Electrons · Physics 2015-05-30 Yutaka Shirata , Hidekazu Tanaka , Akira Matsuo , Koichi Kindo

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

Motivated by the recent observations of various exotic quantum states in the equilateral triangular-lattice phosphates Na$_2$BaCo(PO$_4$)$_2$ with $J\rm_{eff}$ = 1/2 and Na$_2$BaNi(PO$_4$)$_2$ with $S$ = 1, the magnetic properties of…

Strongly Correlated Electrons · Physics 2024-12-05 Chuandi Zhang , Junsen Xiang , Cheng Su , Denis Sheptyakov , Xinyang Liu , Yuan Gao , Peijie Sun , Wei Li , Gang Su , Wentao Jin

We present single-crystal neutron scattering measurements of the spin-1/2 equilateral triangular lattice antiferromagnet Ba$_3$CoSb$_2$O$_9$. Besides confirming that the Co$^{2+}$ magnetic moments lie in the ab plane for zero magnetic…

Strongly Correlated Electrons · Physics 2016-03-02 J. Ma , Y. Kamiya , Tao Hong , H. B. Cao , G. Ehlers , W. Tian , C. D. Batista , Z. L. Dun , H. D. Zhou , M. Matsuda

The magnetic and lattice properties of the $S$=1/2 quantum-spin-chain ferromagnet, CuAs$_2$O$_4$, mineral name trippkeite, were investigated. The crystal structure of CuAs$_2$O$_4$ is characterized by the presence of corrugated CuO$_2$…

Materials Science · Physics 2015-06-18 K. Caslin , R. K. Kremer , F. S. Razavi , A. Schulz , A. Muñoz , F. Pertlik , J. Liu , M. -H. Whangbo , J. M. Law

We report an investigation on structure and magnetic properties of the $S=3/2$ zigzag spin chain compound BaCoTe$_2$O$_7$. Neutron diffraction measurements reveal BaCoTe$_2$O$_7$ crystallizes in the noncentrosymmetric space group $Ama2$…

Strongly Correlated Electrons · Physics 2021-07-06 Lisi Li , Xunwu Hu , Zengjia Liu , Jia Yu , Benyuan Cheng , Sihao Deng , Lunhua He , Kun Cao , Dao-Xin Yao , Meng Wang

Ba$_3$CoSb$_2$O$_9$ approximates the two-dimensional spin-1/2 triangular-lattice Heisenberg antiferromagnet. This compound displays magnetic-field-induced quantum phase transitions, including the 1/3-magnetization-plateau, but its…

Strongly Correlated Electrons · Physics 2023-05-17 Kazuki Okada , Hidekazu Tanaka , Nobuyuki Kurita , Daisuke Yamamoto , Akira Matsuo , Koichi Kindo

We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca$_3$CoNb$_2$O$_9$, in which the effective spin of Co$^{2+}$ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and…

Strongly Correlated Electrons · Physics 2015-12-25 J. Dai , P. Zhou , P. S. Wang , F. Pang , T J. Munsie , G. M. Luke , J. S. Zhang , Weiqiang Yu

We report synthesis and magnetic properties of quasi-one-dimensional spin-$\frac{1}{2}$ Heisenberg antiferromagnetic chain compound BaNa$_2$Cu(VO$_4$)$_2$. This orthovanadate has a centrosymmetric crystal structure, $C2/c$, where the…

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