English
Related papers

Related papers: Ultrafast intermolecular energy transfer from vibr…

200 papers

In a nanoscale molecular junction at finite bias voltage,the intra-molecular distribution of vibrational energy can strongly deviate from the thermal equilibrium distribution and specific vibrational modes can be selectively excited in a…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Rainer Härtle , Roie Volkovich , Michael Thoss , Uri Peskin

We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…

Atomic Physics · Physics 2008-10-28 Christiane P. Koch , Robert Moszynski

Electron capture by {\it isolated} atoms and ions proceeds by photorecombination. In this process a species captures a free electron by emitting a photon which carries away the excess energy. It is shown here that in the presence of an {\it…

Quantum Physics · Physics 2010-03-18 Kirill Gokhberg , Lorenz S. Cederbaum

We investigate the role of electronic-vibrational coupling in resonant electron transport through single-molecule junctions, taking into account that the corresponding coupling strengths may depend on the charge and excitation state of the…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Andre Erpenbeck , Rainer Härtle , Michel Bockstedte , Michael Thoss

Energy dissipation in water is very fast and more efficient than in many other liquids. This behavior is commonly attributed to the intermolecular interactions associated with hydrogen bonding. Here, we investigate the dynamic energy flow…

The transfer of weakly bound KRb molecules from levels just below the dissociation threshold into the vibrational ground state with shaped laser pulses is studied. Optimal control theory is employed to calculate the pulses. The complexity…

Atomic Physics · Physics 2011-04-15 Mamadou Ndong , Christiane P. Koch

Both classical and quantum electrodynamics predict the existence of dipole-dipole long-range electrodynamic intermolecular forces; however, these have never been hitherto experimentally observed. The discovery of completely new and…

In this paper, we study the role of collective vibrational motion in the phenomenon of electronic energy transfer (EET) along a chain of coupled electronic dipoles with varying excitation frequencies. Previous experimental work on EET in…

Quantum Physics · Physics 2015-03-13 F. L. Semião , K. Furuya , G. J. Milburn

We show how to bridge the divide between atomic systems and electronic devices by engineering a coupling between the motion of a single ion and the quantized electric field of a resonant circuit. Our method can be used to couple the…

Quantum Physics · Physics 2015-06-03 D. Kielpinski , D. Kafri , M. J. Woolley , G. J. Milburn , J. M. Taylor

We describe a model of electron transfer reactions affected by local binding to the donor or acceptor sites of a particle in equilibrium with the solution. The statistics of fluctuations of the donor-acceptor energy gap caused by…

Biological Physics · Physics 2007-10-16 Dmitry V. Matyushov

In the present work, we analyze the influence of the polarization effects taking place during the course of a 2DIR spectroscopy experiment performed on a molecular system undergoing an intermolecular vibrational energy transfer process.…

Chemical Physics · Physics 2017-08-18 Albert A. Villaeys , Mabrouk Zouari , Kuo Kan Liang

Efficient energy transfer from electromagnetic waves to ions has been demanded to control laboratory plasmas for various applications and could be useful to understand the nature of space and astrophysical plasmas. However, there exists a…

Plasma Physics · Physics 2019-12-04 Takayoshi Sano , Masayasu Hata , Daiki Kawahito , Kunioki Mima , Yasuhiko Sentoku

We consider the effective interaction between electrons due to the exchange of virtual acoustic waves in a low temperature plasma. Electrons are supposed to participate in rapid radial oscillations forming a spherically symmetric plasma…

Plasma Physics · Physics 2012-01-04 Maxim Dvornikov

Experiments studying vibrational effects on electronic transport through single molecules have observed several seemingly inconsistent behaviors, ranging from up to 30 harmonics of a vibrational frequency in one experiment, to an absence of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Vivek Aji , J. E. Moore , C. M. Varma

Electron-impact ionization of an atom or ion in the presence of a neighboring atom is studied. The latter is first collisionally excited by the incident electron, whose energy is assumed to be high but nonrelativistic. Afterwards, the…

Atomic Physics · Physics 2019-11-06 F. Grüll , A. B. Voitkiv , C. Müller

Highly energetic, relativistic electrons are commonly present in many astrophysical systems, from solar flares to the intra-cluster medium, as indicated by observed electromagnetic radiation. However, open questions remain about the…

Plasma Physics · Physics 2020-05-27 Domenico Trotta , Luca Franci , David Burgess , Petr Hellinger

We consider trasfer-ionization in collisions of fast (3.6 -- 11 MeV/u) protons, alpha-particles and lithium nuclei with helium atoms. There are just a few basic mechanisms contributing to this process which can be grouped into correlated…

Atomic Physics · Physics 2015-06-05 A. B. Voitkiv , X. Ma

We theoretically analyze correlation effects on the transport properties of a benzene molecule that are mediated by interactions between the motion of the nuclei and the transmitted charge. We focus on the lowest-lying molecular vibrational…

Mesoscale and Nanoscale Physics · Physics 2013-08-09 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

A model based on the strong-field and Born-Oppenheimer approximations qualitatively describes the distribution over vibrational states formed in a diatomic molecular ion following ionization of the neutral molecule by intense laser pulses.…

Atomic Physics · Physics 2007-05-23 Thomas Kim Kjeldsen , Lars Bojer Madsen

A numerical simulation of vibrational excitation of molecules was devised, and used to excite computational models of common molecules into a prescribed, pure, normal vibration mode in the ground electronic state, with varying, controlable…

Astrophysics · Physics 2009-11-11 Renaud Papoular