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It is shown that the energy absorption of a rare-gas cluster from a vacuum-ultraviolet (VUV) pulse can be traced with time-delayed extreme-ultraviolet (XUV) attosecond probe pulses by measuring the kinetic energy of the electrons detached…

Atomic and Molecular Clusters · Physics 2008-04-07 Ulf Saalmann , Ionuţ Georgescu , Jan M. Rost

Time- and angle-resolved photoelectron spectroscopy (trARPES) is a powerful method to track the ultrafast dynamics of quasiparticles and electronic bands in energy and momentum space. We present a setup for trARPES with 22.3 eV…

Transient grating spectroscopy has become a mainstay among metal and semiconductor characterization techniques. Here we extend the technique towards the shortest achievable timescales by using tabletop high-harmonic generation of attosecond…

We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shake-up of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond…

Atomic Physics · Physics 2013-05-24 Renate Pazourek , Stefan Nagele , Johannes Feist , Joachim Burgdörfer

We demonstrate a novel method to measure the temporal evolution of electric fields with optical frequencies. Our technique is based on the detection of transient currents in air plasma. These directional currents result from sub-cycle…

Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…

Accelerator Physics · Physics 2025-07-01 Andreas Seidel , Carola Zepter , Alexander Sävert , Stephan Kuschel , Matt Zepf

We propose a method for a straightforward characterization of the temporal shape of femtosecond pulses in the extreme-ultraviolet/soft X-ray spectral region. The approach is based on the presence of a significant linear frequency chirp in…

Optics · Physics 2015-06-15 David Gauthier , Benoît Mahieu , Giovanni De Ninno

Attosecond electron pulses enable real-time probing of ultrafast matter dynamics, yet conventional modulation schemes suffer from drastically shortened longitudinal focal lengths when targeting sub-attosecond durations. To address this…

Plasma Physics · Physics 2026-05-15 Qi Huang , Qing Jia , Zhongxuan Wang , Jian Zheng

Spectral Doppler ultrasound imaging allows visualizing blood flow by estimating its velocity distribution over time. Duplex ultrasound is a modality in which an ultrasound system is used for displaying simultaneously both B-mode images and…

Information Theory · Computer Science 2018-08-03 Regev Cohen , Yonina C. Eldar

We propose a simple all-in-line single-shot scheme for diagnostics of ultrashort laser pulses, consisting of a multi-mode fiber, a nonlinear crystal and a CCD camera. The system records a 2D spatial intensity pattern, from which the pulse…

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

We demonstrate that time-domain ptychography, a recently introduced ultrafast pulse reconstruction modality, has properties ideally suited for the temporal characterization of complex light pulses with large time-bandwidth products as it…

The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

Dispersion-based photonics-assisted microwave measurement systems provide immense potential for real-time analysis of wideband and dynamic signals. However, they face two critical challenges: a difficulty in achieving high frequency…

Optics · Physics 2026-02-13 Chi Jiang , Taixia Shi , Hang Yang , Lei Gao , Xianxin Zhang , Yiqing Liu , Yang Chen

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

A novel algorithm for the ultrashort laser pulse characterization method of interferometric frequency-resolved optical gating (iFROG) is presented. Based on a genetic method, namely differential evolution, the algorithm can exploit all…

Optics · Physics 2017-10-25 Janne Hyyti , Esmerando Escoto , Günter Steinmeyer

Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating…

Optics · Physics 2026-04-17 Rocio Borrego Varillas , Pierre Agostini , Fernando Ardana-Lamas , Cord L. Arnold , David Ayuso , Maurizio Reduzzi , Jakub Benda , Jens Biegert , Charles Bourassin-Bouchet , Thomas Brabec , Christian Brahms , Andrew C. Brown , David Busto , Jérémie Caillat , Francesca Calegari , Carlo Callegari , Stefanos Carlström , Zenghu Chang , Ming-Chang Chen , Anna G. Ciriolo , Paul Corkum , Gabriele Crippa , Rafael de Q. Garcia , Louis DiMauro , Nirit Dudovich , Per Eng-Johnsson , Davide Faccialà , Philip Flores , Titouan Gadeyne , Gianluca Aldo Geloni , Chase Geirger , Shima Gholam-Mirzaei , Jimena D. Gorfinkiel , Eleftherios Goulielmakis , Mohammed Hassan , Carlos Hernández-García , Phay Ho , Dandan Hui , Lynda R. Hutcheson , Misha Ivanov , Subhendu Kahaly , Henry Kapteyn , Nicholas Karpowicz , Franz X. Kärtner , Matthias Kling , Omer Kneller , Dong Hyuk Ko , Peter M. Kraus , Maximilian Kubullek , Stephen R. Leone , Franck Lépine , Anne L'Huillier , Chen-Ting Liao , Thomas Linker , Alexander Gabriel Lohr , Matteo Lucchini , Lars Bojer Madsen , Roland E. Mainz , Balázs Major , Jon P. Marangos , David Marco , Hugo Marroux , Sean Marshallsay , Rebeca Martínez Vázquez , Rodrigo Martín-Hernández , Zdeněk Mašín , Michael Meyer , Felipe Morales Moreno , Margaret Murnane , Daniel M. Neumark , Mauro Nisoli , Marcus Ossiander , Sreelakshmi Palakka , Serguei Patchkovskii , Zekun Pi , Luis Plaja , Julita Poborska , Miguel A. Porras , Kevin C. Prince , David N. Purschke , Nicolette G. Puskar , Giulio Maria Rossi , Jérémy R. Rouxel , Thierry Ruchon , Patrick Rupprecht , Pascal Salières , Giuseppe Sansone , Fabian Scheiba , Martin Schultze , Bernd Schütte , Svitozar Serkez , Miguel A. Silva-Toledo , Olga Smirnova , Salvatore Stagira , Andrea Trabattoni , John C. Travers , Igor Tyulnev , Morgane Vacher , Giulio Vampa , Hugo W. van der Hart , Katalin Varjú , Anne-Lise Viotti , Vartika Vishnoi , Marc Vrakking , Vincent Wanie , Stefan Witte , Fei Xu , Vladislav S. Yakovlev , Linda Young , Diling Zhu , Caterina Vozzi

We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…