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Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

Collective electron dynamics in plasmonic nanosystems can unfold on timescales in the attosec- ond regime and the direct measurements of plasmonic near-field oscillations is highly desirable. We report on numerical studies on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Frederik Süßmann , Matthias F. Kling

Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…

Chemical Physics · Physics 2022-11-07 Lorenzo Restaino , Deependra Jadoun , Markus Kowalewski

An all-optical method for directly reconstructing the spectral phase of isolated attosecond pulse (IAP) has been proposed recently [New J. Phys. 25, 083003 (2023)]. This method is based on the high-harmonic generation (HHG) streaking…

First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…

Other Condensed Matter · Physics 2015-05-13 C. Lemell , B. Solleder , K. Tokesi , J. Burgdoerfer

We exploit a slightly noncollinear second-harmonic cross-correlation scheme to map the 3D space-time intensity distribution of an unknown complex-shaped ultrashort optical pulse. We show the capability of the technique to reconstruct both…

X-ray free-electron lasers (XFELs) as the world's brightest light sources provide ultrashort X-ray pulses with a duration typically in the order of femtoseconds. Recently, they have approached and entered the attosecond regime, which holds…

Attosecond streaking camera is an ex situ technique in which a linearly polarized (LP) XUV attopulse produces an electron wavepacket by photoionization in the presence of an IR femtopulse. By moving the two synchronous oppositely circularly…

Atomic Physics · Physics 2025-11-27 M. A. H. B. Md Yusoff , H. B. Ambalampitiya , J. M. Ngoko Djiokap

Laser assisted photoemission by a chirped subfemtosecond extreme ultraviolet (XUV) pulse is considered within an exactly solvable quantum-mechanical model. Special emphasis is given to the energy dependence of photoexcitation cross-section.…

Atomic Physics · Physics 2015-05-13 E. E. Krasovskii , M. Bonitz

We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…

Atomic Physics · Physics 2015-05-13 P. Riviere , O. Uhden , U. Saalmann , J. M. Rost

Attosecond photoelectron spectroscopy is often performed with interferometric experimental setups that require outstanding stability. We demonstrate and characterize in detail an actively stabilized, versatile, high spectral resolution…

Signals comprised of a stream of short pulses appear in many applications including bio-imaging and radar. The recent finite rate of innovation framework, has paved the way to low rate sampling of such pulses by noticing that only a small…

Information Theory · Computer Science 2015-05-18 Ronen Tur , Yonina C. Eldar , Zvi Friedman

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

Atomic Physics · Physics 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

Over the past few decades, following the first demonstration of ultrafast electron microscopy, numerous research groups have focused on achieving attosecond temporal resolution in electron microscopy with the goal of imaging electron and…

Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…

Field-emission of electrons underlies major advances in science and technology, ranging from imaging the atomic-scale structure of matter to signal processing at ever-higher frequencies. The advancement of these applications to their…

Optics · Physics 2023-02-22 H. Y. Kim , M. Garg , S. Mandal , L. Seiffert , T. Fennel , E. Goulielmakis

We propose the scheme of temporal double-slit interferometer to precisely measure the electric field of shaped intense femtosecond laser pulse directly, and apply it to control the electron tunneling wave packets in attosecond precision. By…

Atomic Physics · Physics 2023-11-13 Xiaoyun Zhao , Mingqing Liu , Yizhang Yang , Zhou Chen , Xiaolei Hao , Chuncheng Wang , Weidong Li , Jing Chen

The implementation of attosecond photoelectron-photoion coincidence spectroscopy for the investigation of atomic and molecular dynamics calls for a high-repetition-rate driving source combined with experimental setups characterized by…

A short sample sequence of a finite-length pulse signal allows for its reconstruction only if the signal has a sparse representation in some basis. The recurrence of the pulse allows for a statistical approach to its reconstruction. We…

Signal Processing · Electrical Eng. & Systems 2023-08-15 Marek W. Rupniewski