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We report on the first streaking measurement of water-window attosecond pulses generated via high harmonic generation, driven by sub-2-cycle, CEP-stable, 1850 nm laser pulses. Both the central photon energy and the energy bandwidth far…

Many experiments in attosecond science will benefit from attosecond pulses at high repetition rates with sufficient photon flux for pump-probe experiments. We use 7fs, 800nm pulses from a non-collinear optical parametric chirped pulse…

A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…

Atomic Physics · Physics 2015-04-06 Pengfei Lan , Peixiang Lu , Wei Cao , Yuhua Li , Xinlin Wang

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

Atomic and Molecular Clusters · Physics 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

We report on the global temporal pulse characteristics of individual harmonics in an attosecond pulse train by means of photo-electron streaking in a strong low-frequency transient. The scheme allows direct retrieval of pulse durations and…

We demonstrate a new attosecond pulse reconstruction modality which uses an algorithm that is derived from ptychography. In contrast to other methods, energy and delay sampling are not correlated, and as a result, the number of electron…

Optics · Physics 2015-11-17 M. Lucchini , M. H. Brügmann , A. Ludwig , L. Gallmann , U. Keller , T. Feurer

Achromatic flying-focus enables programmable control of intensity peak velocity, with applications in ultrafast optics. However, spatiotemporal coupling inherently elongates ultrashort pulses by introducing frequency-dependent focusing and…

Optics · Physics 2026-03-27 Jérôme Touguet , Igor A. Andriyash , Lucas Rovige , Cédric Thaury

The waveforms of attosecond pulses produced by high-harmonic generation carry information on the electronic structure and dynamics in atomic and molecular systems. Current methods for the temporal characterization of such pulses have…

Ultra-short laser pulses with femtosecond to attosecond pulse duration are the shortest systematic events humans can create. Characterization (amplitude and phase) of these pulses is a key ingredient in ultrafast science, e.g., exploring…

Optics · Physics 2018-03-19 Tom Zahavy , Alex Dikopoltsev , Oren Cohen , Shie Mannor , Mordechai Segev

Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

An electrical pulse E(t) is completely defined by its time-dependent amplitude and polarisation direction. For optical pulses the manipulation and characterisation of the light polarisation state is fundamental due to its relevance in…

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

A detection scheme for characterizing high-energy $\gamma$-ray pulses down to the zeptosecond timescale is proposed. In contrast to existing attosecond metrology techniques, our method is not limited by atomic shell physics and therefore…

Instrumentation and Detectors · Physics 2011-08-17 Andreas Ipp , jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

A new method for efficiently generating an isolated single-cycle attosecond pulse is proposed. It is shown that the ultraviolet (UV) attosecond pulse can be utilized as a robust tool to control the dynamics of electron wave packets (EWPs).…

Atomic Physics · Physics 2009-11-13 Pengfei Lan , Peixiang Lu , Wei Cao , Xinlin Wang

Typically, in Self-Amplified Spontaneous Emission Free Electron Laser (SASE FEL) based short-pulse schemes, pulse duration is limited by FEL coherence time. For hard X-ray FELs, coherence time is in a few hundred attosecond range while for…

Accelerator Physics · Physics 2022-02-09 E. A. Schneidmiller

We have proposed and developed a method to utilize attosecond pulses in diffraction imaging techniques applied to complex samples. In this study, the effects of the broadband properties of the wavefield owing to attosecond pulses are…

Optics · Physics 2023-12-01 G. N. Tran , Katsumi Midorikawa , Eiji J. Takahashi

Ultrafast experiments require precise temporal characterization of laser pulses, where pulse reconstruction is typically achieved through iterative retrieval algorithms. In this context, the amplitude swing technique has emerged as a robust…

Optics · Physics 2025-06-12 Cristian Barbero , Íñigo J. Sola , Benjamín Alonso

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen
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