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Over the last two decades, intensive research efforts have been devoted to the suppressions of photoluminescence (PL) blinking and Auger recombination in metal-chalcogenide nanocrystals (NCs), with significant progresses being made only…

Materials Science · Physics 2016-11-03 Fengrui Hu , Chunyang Yin , Huichao Zhang , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

We investigate the charge re-distribution upon optical excitation of various necked homodimer CQDMs using single particle emission spectroscopy. By tuning the hybridization of the electron wavefunction at a fixed center-to-center distance…

Mesoscale and Nanoscale Physics · Physics 2023-06-27 Somnath Koley , Jiabin Cui , Yossef. E. Panfil , Yonatan Ossia , Adar Levi , Einav Scharf , Lior Verbitsky , Uri Banin

We present detailed theoretical and experimental studies of Auger recombination in narrow-gap mercury cadmium telluride quantum wells (HgCdTe QWs). We calculate the Auger recombination probabilities as functions of non-equilibrium carrier…

Mesoscale and Nanoscale Physics · Physics 2020-10-23 V. Ya. Aleshkin , G. Alymov , A. V. Antonov , A. A. Dubinov , V. V. Rumyantsev , S. V. Morozov

Coherently driven semiconductor quantum dots are one of the most promising platforms for non-classical light sources and quantum logic gates which form the foundation of photonic quantum technologies. However, to date, coherent manipulation…

We review the effects of Coulomb correlation on the linear and non-linear optical properties of semiconductor quantum wires, with emphasis on recent results for the bound excitonic states. Our theoretical approach is based on generalized…

Materials Science · Physics 2009-10-30 G. Goldoni , F. Rossi , E. Molinari

The recombination of electron-hole pairs injected in extended conjugated systems is modeled as a multi-pathway vibron-driven relaxation in monoexcited state-space. The computed triplet-to-singlet ratio of exciton formation times $r =…

Materials Science · Physics 2009-11-07 Stoyan Karabunarliev , Eric. R. Bittner

We calculate the photoluminescence spectrum and lifetime of a biexciton in a semiconductor using Fermi's golden rule. Our biexciton wavefunction is obtained using a Quantum Monte Carlo calculation. We consider a recombination process where…

Strongly Correlated Electrons · Physics 2013-01-15 M. Bauer , J. Keeling , M. M. Parish , P. Lopez Rios , P. B. Littlewood

Using semi-analytical models we calculate the energy, effective Bohr radius and radiative lifetime of neutral excitons confined in CdSe colloidal nanoplatelets (NPLs). The excitonic properties are largely governed by the electron-hole…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Fernando Rajadell , Juan I. Climente , Josep Planelles

A growing interest in colloidal quantum dot (QD) based light-emitting diodes (QD-LEDs) has been motivated by the exceptional color purity and spectral tunability of QD emission as well as the amenability of QD materials to highly scalable…

In this work, we theoretically investigate the optical orientation and alignment of excitons in quantum dots with weak electron-hole exchange interaction and long exciton radiative lifetimes. This particular regime is realized in…

Mesoscale and Nanoscale Physics · Physics 2023-08-30 D. S. Smirnov , E. L. Ivchenko

Modern x-ray sources enable the production of coherent x-ray pulses with a pulse duration in the same order as the characteristic lifetimes of core-hole states of atoms and molecules. These pulses enable the manipulation of the core-hole…

Atomic Physics · Physics 2018-01-11 Raymond Sullivan , Junteng Jia , Alvaro Vazquez-Mayagoitia , Antonio Picón

We simulate the time-dependent coherent dynamics of a spatially indirect exciton (an electron-hole pair with the two particles confined in different layers) in a GaAs coupled quantum well system. We use a unitary wave-packet propagation…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 Federico Grasselli , Andrea Bertoni , Guido Goldoni

A set of electron-correlation energies as large as 10 eV have been measured for a magnetic 2ML Fefilm deposited on Ag(001). By exploiting the spin selectivity in angle-resolved Auger-photoelectroncoincidence spectroscopy and the…

Strongly Correlated Electrons · Physics 2020-08-12 R. Gotter , A. Verna , M. Sbroscia , R. Moroni , F. Bisio , S. Iacobucci , F. Offi , S. R. Vaidya , A. Ruocco , G. Stefani

Auger recombination (AR) of the ground biexciton state in quantum-confined lead salt nanowires (NWs) with a strong coupling between the conduction and the valence bands is shown to be strongly suppressed, and only excited biexciton states…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Valery I. Rupasov

Carrier and spin recombination are investigated in p-type GaAs of acceptor concentration NA = 1.5 x 10^(17) cm^(-3) using time-resolved photoluminescence spectroscopy at 15 K. At low pho- tocarrier concentration, acceptors are mostly…

Materials Science · Physics 2017-04-05 F. Cadiz , D. Lagarde , P. Renucci , D. Paget , T. Amand , H. Carrère , A. C. H. Rowe , S. Arscott

The effect of external electric field on electron-hole correlation in GaAs quantum dots is investigated. The electron-hole Schrodinger equation in the presence of external electric field is solved using explicitly correlated full…

Chemical Physics · Physics 2013-02-06 Christopher J. Blanton , Christopher Brenon , Arindam Chakraborty

We develop a general method to calculate Zeeman splittings of electrons and holes in semiconductor nanostructures within the tight-binding framework. The calculation is carried out in the electron-hole picture and is extensible to the…

Other Condensed Matter · Physics 2007-05-23 Pochung Chen

Cooperative spontaneous recombination (superfluorescence) of electron-hole plasmas in semiconductors has been a challenge to observe due to ultrafast decoherence. We argue that superfluorescence can be achieved in quantum-confined…

Mesoscale and Nanoscale Physics · Physics 2009-07-28 Y. D. Jho , X. Wang , J. Kono , D. H. Reitze , A. A. Belyanin , V. V. Kocharovsky , Vl. V. Kocharovsky , G. S. Solomon

Supercell method is used to study the relaxation and screening effects during the Auger transition in metals. In order to make the interaction between the core-holes sited at different atoms negligible, the real metal is simulated by…

Strongly Correlated Electrons · Physics 2007-05-23 Jianmin Yuan

Angle resolved-Auger-photoelectron coincidence spectroscopy (AR-APECS) has been exploited to investigate the role that electron correlation plays in the exchange-coupling at the ferromagnetic/antiferromagnetic interface of a Fe/CoO bilayer…