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Broadband microwave spectroscopy has been performed on single-crystalline GaV$_4$S$_8$, which exhibits a complex magnetic phase diagram including cycloidal, N\'eel-type skyrmion lattice, as well as field-polarized ferromagnetic phases below…

We present the results of a muon-spin spectroscopy investigation of GaV$_4$S$_{8-y}$Se$_{y}$ with $y=0, 2, 4$ and 8. Zero-field measurements suggest that GaV$_{4}$Se$_{8}$ and GaV$_{4}$S$_{8}$ have distinct magnetic ground states, with the…

Following the early prediction of the skyrmion lattice (SkL) - a periodic array of spin vortices - it has been observed recently in various magnetic crystals mostly with chiral structure. Although non-chiral but polar crystals with C$_{nv}$…

We report on the anomalous magnetization dynamics of the cycloidally-modulated spin textures under the influence of uniaxial anisotropy in multiferroic $\mathrm{GaV_4S_8}$. The temperature and field dependence of the linear ac…

Mesoscale and Nanoscale Physics · Physics 2020-03-20 E. M. Clements , R. Das , G. Pokharel , M. H. Phan , A. D. Christianson , D. Mandrus , J. C. Prestigiacomo , M. S. Osofsky , H. Srikanth

Skyrmions are whirl like topological spin objects with high potential for future magnetic data storage. It is a fundamental question, relevant for both basic research and application, if a ferroelectric (FE) polarization can be associated…

Strongly Correlated Electrons · Physics 2015-11-18 E. Ruff , S. Widmann , P. Lunkenheimer , V. Tsurkan , S. Bordács , I. Kézsmárki , A. Loidl

We report small-angle neutron scattering studies of the lacunar spinel GaV$_4$S$_8$, which reveal the long-wavelength magnetic states to be cycloidally modulated. This provides direct support for the formation of N\'eel-type skyrmions…

Strongly Correlated Electrons · Physics 2018-01-10 J. S. White , Á. Butykai , R. Cubitt , D. Honecker , C. D. Dewhurst , L. F. Kiss , V. Tsurkan , S. Bordács

Polar lacunar spinels, such as GaV$_4$S$_8$ and GaV$_4$Se$_8$, were proposed to host skyrmion phases under magnetic field. In this work, we put forward, as a candidate for N\'eel-type skyrmion lattice, the isostructural GaMo$_4$S$_8$, here…

Materials Science · Physics 2019-06-26 Hui-Min Zhang , Jun Chen , Paolo Barone , Kunihiko Yamauchi , Shuai Dong , Silvia Picozzi

In the lacunar spinel GaV4S8, the interplay of spin, charge, and orbital degrees of freedom produces a rich phase diagram that includes an unusual Neel-type skyrmion phase composed of molecular spins. To provide insight into the…

The lacunar spinel GaV4S8 exhibits orbital ordering at 44 K and shows a complex magnetic phase diagram below 12.7 K, which includes ferromagnetic and cycloidal spin order. At low but finite external magnetic fields, N\'eel-type skyrmions…

Strongly Correlated Electrons · Physics 2017-12-14 S. Widmann , E. Ruff , A. Günther , H. -A. Krug von Nidda , P. Lunkenheimer , V. Tsurkan , S. Bordács , I. Kézsmárki , A. Loidl

We report the feasibility of using magnetoentropic mapping for the rapid identification of magnetic cycloid and skyrmion phases in uniaxial systems, based on the GaV4S8 and GaV4Se8 model skyrmion hosts with easy-axis and easy-plane…

We report on the slow magnetization dynamics observed upon the magnetic phase transitions of GaV4S8, a multiferroic compound featuring a long-ranged cycloidal magnetic order and a N\'eel-type skyrmion lattice in a relatively broad…

We present an investigation of the influence of low-levels of chemical substitution on the magnetic ground state and N{\' e}el skyrmion lattice (SkL) state in GaV$_4$S$_{8-y}$Se$_y$, where $y =0, 0.1, 7.9$, and $8$. Muon-spin spectroscopy…

We show how low-energy electronic models derived from the first-principles electronic structure calculations can help to rationalize the magnetic properties of two lacunar spinel compounds GaM4S8 with light (M=V) and heavy (M=Mo)…

Strongly Correlated Electrons · Physics 2020-07-14 S. A. Nikolaev , I. V. Solovyev

We present magnetization and muon-spin spectroscopy measurements of N\'{e}el skyrmion-host GaV$_4$S$_8$ under the application of hydrostatic pressures up to $P=2.29$ GPa. Our results suggest that the magnetic phase diagram is altered with…

Strongly Correlated Electrons · Physics 2022-03-23 T. J. Hicken , M. N. Wilson , S. J. R. Holt , R. Khassanov , M. R. Lees , R. Gupta , D. Das , G. Balakrishnan , T. Lancaster

The orientation of N\'eel-type skyrmions in the lacunar spinels GaV$_4$S$_8$ and GaV$_4$Se$_8$ is tied to the polar axes of their underlying crystal structure through the Dzyaloshinskii-Moriya interaction. In these crystals, the skyrmion…

Strongly Correlated Electrons · Physics 2020-09-04 B. Gross , S. Philipp , K. Geirhos , A. Mehlin , S. Bordács V. Tsurkan , A. Leonov , I. Kézsmárki , M. Poggio

We investigate the microwave spin excitations of the cubic chiral magnet Fe$_{0.75}$Co$_{0.25}$Si as driven by the thermal modulation of magnetic interactions via laser heating and probed by time-resolved measurements of the magneto-optical…

We have used inelastic neutron scattering to measure the magnetic excitation spectrum along the high-symmetry directions of the first Brillouin zone of the magnetic skyrmion hosting compound Cu$_2$OSeO$_3$. The majority of our scattering…

Strongly Correlated Electrons · Physics 2016-08-01 G S Tucker , J S White , J Romhányi , D Szaller , I Kézsmárki , B Roessli , U Stuhr , A Magrez , F Groitl , P Babkevich , P Huang , I Živković , H M Rønnow

Skyrmions are particle-like vortices of magnetization with non-trivial topology, which are usually stabilized by Dzyaloshinskii-Moriya interactions (DMI) in noncentrosymmetric bulk materials. Exceptions are centrosymmetric Gd- and Eu-based…

Magnetic materials hosting correlated electrons play an important role for information technology and signal processing. The currently used ferro-, ferri- and antiferromagnetic materials provide microscopic moments (spins) that are mainly…

Strongly Correlated Electrons · Physics 2017-08-02 Markus Garst , Johannes Waizner , Dirk Grundler

In polar magnets, such as GaV$_4$S$_8$, GaV$_4$Se$_8$ and VOSe$_2$O$_5$, modulated magnetic phases namely the cycloidal and the N\'eel-type skyrmion lattice states were identified over extended temperature ranges, even down to zero Kelvin.…

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