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We report $\alpha$-Cu$_2$V$_2$O$_7$ to be an improper multiferroic with the simultaneous development of electric polarization and magnetization below $T_C$ = 35 K. The observed spontaneous polarization of magnitude 0.55 $\mu$Ccm$^{-2}$ is…

Strongly Correlated Electrons · Physics 2015-06-26 J. Sannigrahi , S. Bhowal , S. Giri , S. Majumdar , I. Dasgupta

Geometrically frustrated structures combined with competing exchange interactions that have different magnitudes are known ingredients for achieving exotic properties. Herein, we studied detailed structural, magnetic, thermal (specific…

Materials Science · Physics 2023-12-18 P. Mohanty , N. Sharma , D. Singh , Y. Breard , D. Pelloquin , S. Marik , R. P. Singh

In order to explore the effects of structural geometry on properties of correlated metals we investigate the magnetic properties of cubic (3C) and hexagonal (4H) BaRuO$_3$. While the 3C variant of BaRuO$_3$ is ferromagnetic below 60K, the…

Strongly Correlated Electrons · Physics 2022-06-13 Hrishit Banerjee , Hermann Schnait , Markus Aichhorn , Tanusri Saha-Dasgupta

The majority of magnetoelectric crystals show complex temperature-magnetic field or temperature-pressure phase diagrams with alternating antiferromagnetic incommensurate, magnetoelectric, and commensurate phases. Such phase diagrams occur…

Strongly Correlated Electrons · Physics 2013-12-20 N. V. Ter-Oganessian , V. P. Sakhnenko

MnSb$_{2}$O$_{6}$ is based on the structural chiral $P$321 space group #150 where the magnetic Mn$^{2+}$ moments ($S=5/2$, $L\approx 0$) order antiferromagnetically at $T_\mathrm{N}=12$ K. Unlike the related iron based langasite…

A detailed investigation of Ba$_2$MnGe$_2$O$_7$ was performed in its low-temperature magnetoelectric state combining neutron diffraction with magnetization measurements on single crystals. In the paramagnetic state at 10 K, polarized…

Strongly Correlated Electrons · Physics 2023-03-07 A. Sazonov , H. Thoma , R. Dutta , M. Meven , A. Gukasov , R. Fittipaldi , V. Granata , T. Masuda , B. Náfrádi , V. Hutanu

We present a phenomenological model for magnetoelectricity in multiferroic materials. The distinctive feature of the model is a two-component complex order parameter that encodes the electric polarization, along with a direct coupling…

Materials Science · Physics 2024-04-11 Pei Wang , You-Quan Li

We have conducted a comprehensive investigation into the magnetic properties of the chiral multiferroic material CoTeMoO$_6$. In contrast with the previous claim of canted antiferromagnetic order with ferromagnetic components, our…

Composition-driven structural transitions in Bi1-xCaxFe1-xMnxO3 ceramics prepared by the tartaric acid modified sol-gel technique have been studied to analyze its effect on the magnetic properties of bismuth ferrite (BiFeO3). It was…

Materials Science · Physics 2014-01-17 Pawan Kumar , Manoranjan Kar

We present a study of the dielectric, structural, and magnetic properties of the multiferroic or linear magnetoelectric substitution series [(NH$_4$)$_{1-x}$K$_x$]$_2$[FeCl$_5$(H$_2$O)]. Pyroelectric currents, magnetic susceptibilities, and…

Severe plastic deformation using high-pressure torsion of ternary Cu-based materials (CuFeCo and CuFeNi) was used to fabricate bulk samples with a nanocrystalline microstructure. The goal was to produce materials featuring the granular…

Materials Science · Physics 2022-08-26 M. Kasalo , S. Wurster , M. Stückler , M. Zawodzki , L. Weissitsch , R. Pippan , A. Bachmaier

Our results describe an unprecedented example of change in the mechanism of magnetically-induced electric polarization from spin current to spin-dependent p-d hybridization model. We have followed the evolution of the magnetic structures of…

Ba2CoGe2O7, crystallizing in the noncentrosymmetric but nonpolar structure, belongs to a special class of multiferroic materials, whose properties are predetermined by the rotoinversion symmetry. Unlike inversion, the rotoinversion symmetry…

Materials Science · Physics 2015-06-23 I. V. Solovyev

This paper presents structural, detailed magnetic, and exchange bias studies in polycrystalline Ba$_{2}$ScRuO$_{6}$ synthesized at ambient pressure. In contrast to its strontium analogue, this material crystallizes in a 6L hexagonal…

Materials Science · Physics 2023-04-28 Prachi Mohanty , Sourav Marik , R. P. Singh

The structural and magnetic properties of spinel compounds $CoB_2O_4$ (B=Cr,Mn and Fe) are studied using the DFT+U method and generalized gradient approximation (GGA). We concentrate on understanding the trends in the properties of these…

Strongly Correlated Electrons · Physics 2016-09-21 Debashish Das , Rajkumar Biswas , Subhradip Ghosh

We present a detailed study of complex dielectric constant and ferroelectric polarization in multiferroic LiCuVO4 as function of temperature and external magnetic field. In zero external magnetic field, spiral spin order with an ab helix…

Strongly Correlated Electrons · Physics 2008-04-15 F. Schrettle , S. Krohns , P. Lunkenheimer , J. Hemberger , N. Büttgen , H. -A. Krug von Nidda , A. V. Prokofiev , A. Loidl

Magnetoelectric effect is a fundamental physics phenomenon that synergizes electric and magnetic degrees of freedom to generate distinct material responses like electrically tuned magnetism, which serves as a key foundation of the emerging…

Transition metal dichalcogenides (TMDC) stand out with their high chemical stability and the possibility to incorporate a wide range of magnetic species between the layers. The behavior of conduction electrons in such materials intercalated…

The olivine compound Mn2GeO4 is shown to feature both a ferroelectric polarization and a ferromagnetic magnetization that are directly coupled and point along the same direction. We show that a spin spiral generates ferroelectricity (FE),…

Materials Science · Physics 2012-08-07 J. S. White , T. Honda , K. Kimura , T. Kimura , Ch. Niedermayer , O. Zaharko , A. Poole , B. Roessli , M. Kenzelmann

The magnetoelectric behavior of BiFeO$_3$ has been explored on the basis of accurate density functional calculations. The structural, electronic, magnetic, and ferroelectric properties of BiFeO$_3$ are predicted correctly without including…

Materials Science · Physics 2007-05-23 P. Ravindran , R. Vidya , A. Kjekshus , H. Fjellvåg , O. Eriksson