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A detailed high pressure study is carried out on 1T$^\prime$ MoTe$_{2}$ using X-ray diffraction(XRD) and Raman spectroscopy measurements upto about 30.5 GPa. High pressure XRD measurements show no structural transition. All the lattice…

Materials Science · Physics 2020-01-07 Bishnupada Ghosh , Pinku Saha , Goutam Dev Mukherjee

Layered magnetic transition-metal thiophosphate NiPS3 has unique two-dimensional (2D) magnetic properties and electronic behavior. The electronic band structure and corresponding magnetic state are expected to sensitive to the interlayer…

Strongly Correlated Electrons · Physics 2020-09-30 Xiaoli Ma , Yimeng Wang , Yunyu Yin , Binbin Yue , Jianhong Dai , Jianting Ji , Feng Jin , Fang Hong , Jian-Tao Wang , Qingming Zhang , Xiaohui Yu

We report a polarized Raman scattering study of the lattice dynamics of $\beta$-Li$_2$IrO$_3$ under hydrostatic pressures up to 7.62 GPa. At ambient pressure, $\beta$-Li$_2$IrO$_3$ exhibits the hyperhoneycomb crystal structure and a…

Layered {\alpha}-RuCl3 is a promising material to potentially realize the long-sought Kitaev quantum spin liquid with fractionalized excitations. While evidence of this exotic state has been reported under a modest in-plane magnetic field,…

The structural and vibrational properties of phenanthrene are measured at high pressures up to 30.2 GPa by Raman spectroscopy and synchrotron x-ray diffraction techniques. Two phase transitions are observed in raman spectra under pressures…

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge…

Strongly Correlated Electrons · Physics 2021-11-22 Srishti Pal , Arnab Seth , Piyush Sakrikar , Anzar Ali , Subhro Bhattacharjee , D. V. S. Muthu , Yogesh Singh , A. K. Sood

We suggest, and demonstrate, a systematic approach to the study of cuprate superconductors, namely, progressive change of ion size in order to systematically alter the interaction strength and other key parameters. R(Ba,Sr)$_2$Cu$_3$O$_y$…

Hydrocarbons are of great importance in carbon-bearing fluids in deep Earth and in ice giant planets at extreme pressure (P)-temperature (T) conditions. Raman spectroscopy is a powerful tool to study the chemical speciation of hydrocarbons;…

Computational Physics · Physics 2021-05-18 Rui Hou , Ding Pan

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

Magnetic and vibrational excitations in SrCu$_2$(BO$_3$)$_2$ are studied using Raman spectroscopy at hydrostatic pressures up to 34 kbar and temperatures down to 2.6 K. The frequency of a particular optical phonon, the so-called pantograph…

Strongly Correlated Electrons · Physics 2020-05-06 Simon Bettler , Lena Stoppel , Zewu Yan , Severian Gvasaliya , Andrey Zheludev

We have investigated the magnetic-field- and pressure-induced structural and magnetic phases of the triple-layer ruthenate - Sr$_{4}$Ru$_{3}$O$_{10}$. Magnetic-field-induced changes in the phonon spectra reveal dramatic spin-reorientation…

Strongly Correlated Electrons · Physics 2009-11-11 Rajeev Gupta , M. Kim , H. Barath , S. L. Cooper , G. Cao

We have used a combination of ultrafast coherent phonon spectroscopy, ultrafast thermometry, and time-dependent Landau theory to study the inversion symmetry breaking phase transition at $T_c = 200$ K in the strongly spin-orbit coupled…

Strongly Correlated Electrons · Physics 2018-01-26 J. W. Harter , D. M. Kennes , H. Chu , A. de la Torre , Z. Y. Zhao , J. -Q. Yan , D. G. Mandrus , A. J. Millis , D. Hsieh

In order to investigate the origin of the phase transition observed in NaV$_2$O$_5$, as well as its electronic structure, we have measured Raman intensities as a function of the laser wavelength above and below the phase transition…

Strongly Correlated Electrons · Physics 2015-06-25 M. J. Konstantinovic , Z. V. Popovic , T. Ruf , M. Cardona , A. N. Vasil'ev , M. Isobe , Y. Ueda

Magnetic excitations in layered magnetic materials that can be thinned down the two-dimensional (2D) monolayer limit are of high interest from a fundamental point of view and for applications perspectives. Raman scattering has played a…

Mesoscale and Nanoscale Physics · Physics 2023-02-20 Amit Pawbake , Thomas Pelini , Nathan P. Wilson , Kseniia Mosina , Zdenek Sofer , Rolf Heid , Clement Faugeras

The number of absorption and Raman optical modes for each Wyckoff orbit in the high-temperature tetragonal (I4/mmm) parent lattice of the Ruddlesden-Popper compounds Ca$_3$X$_2$O$_7$, with X=Mn or X=Ti is given. We analyze the effect of…

Materials Science · Physics 2011-01-26 A. B. Harris

Material realization of the non-Abelian Kitaev spin liquid phase - an example of Ising topological order (ITO) - has been the subject of intense research in recent years. The $4d$ honeycomb Mott insulator $\alpha$-RuCl$_3$ has emerged as a…

Strongly Correlated Electrons · Physics 2021-02-26 Jacob S. Gordon , Hae-Young Kee

We report high pressure Raman, synchrotron x-ray diffraction and electrical transport studies on Weyl semimetals NbP and TaP along with first-principles density functional theoretical (DFT) analysis. The frequencies of first-order Raman…

Differently distorted areas on a polycarbonate sample are studied by means of Raman spectroscopy. The various Raman lines, whose energy shifts range between 200 and 3200 cm-1, are compared for different sample positions with respect to…

Materials Science · Physics 2012-03-02 J. Debus , D. Dunker

Near-forward Raman scattering combined with ab initio phonon and bond length calculations is used to study the phonon-polariton transverse optical modes (with mixed electrical and mechanical character) of the II-VI ZnSeS mixed crystal under…

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