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We revisit the interaction of a first-quantized atomic system (consisting of two charged quantum particles) with the quantum electromagnetic field, pointing out the subtleties related to the gauge nature of electromagnetism and the effect…

Quantum Physics · Physics 2021-01-13 Richard Lopp , Eduardo Martín-Martínez

The Dicke model, which describes the dipolar coupling between N two-level atoms and a quantized electromagnetic field, seemingly violates gauge invariance in the presence of ultrastrong light-matter coupling, a regime that is now…

Quantum Physics · Physics 2020-09-02 Luigi Garziano , Alessio Settineri , Omar Di Stefano , Salvatore Savasta , Franco Nori

The dipole coupling term between a system of N particles with total charge zero and the electromagnetic field is derived in the presence of a weak gravitational field. It is shown that the form of the coupling remains the same as in flat…

General Relativity and Quantum Cosmology · Physics 2009-10-22 Karl-Peter Marzlin

The loss of gauge invariance in models of light-matter interaction which arises from material and photonic space truncation can pose significant challenges to conventional quantum optical models when matter and light strongly hybridize. In…

Quantum Physics · Physics 2023-01-31 Chris Gustin , Sebastian Franke , Stephen Hughes

In a gauge invariant formulation of the molecular electric dipole-photon interaction, the rigorous coupling is strictly linear in the photon creation and photon annihilation operators. The linear coupling allows for a super-radiant phase…

Statistical Mechanics · Physics 2007-05-23 S. Somu , A. Widom , Y. N. Srivastava

We describe the physical relativity of light and matter quantum subsystems, their correlations, and energy exchanges. We examine the most commonly adopted definitions of atoms and photons, noting the significant difference in their…

Quantum Physics · Physics 2023-11-20 Adam Stokes , Hannah Riley , Ahsan Nazir

Quantum light-matter systems at strong coupling are notoriously challenging to analyze due to the need to include states with many excitations in every coupled mode. We propose a nonperturbative approach to analyze light-matter correlations…

Mesoscale and Nanoscale Physics · Physics 2021-04-15 Yuto Ashida , Atac Imamoglu , Eugene Demler

We study the gauge invariance of laser-matter interaction. The velocity gauge where the vector potential is expanded to the $n$-th order with respect to the spatial coordinate, and the length gauge where the electric and magnetic fields are…

Atomic Physics · Physics 2018-12-19 Ryoji Anzaki , Yasushi Shinohara , Takeshi Sato , Kenichi L. Ishikawa

The dipole approximation is employed to describe interactions between atoms and radiation. It essentially consists of neglecting the spatial variation of the external field over the atom. Heuristically, this is justified by arguing that the…

Mathematical Physics · Physics 2018-04-04 Lea Boßmann , Robert Grummt , Martin Kolb

In a recent work of ours [Phys. Rev. Lett. 112, 073601 (2014)], we generalized the Power-Zineau-Woolley gauge to describe the electrodynamics of atoms in an arbitrary confined geometry. Here we complement the theory by proposing a tractable…

Quantum Physics · Physics 2016-04-13 A. Vukics , T. Grießer , P. Domokos

Gauge invariance was discovered in the development of classical electromagnetism and was required when the latter was formulated in terms of the scalar and vector potentials. It is now considered to be a fundamental principle of nature,…

We discuss the problem of gauge fixing for strongly correlated electrons coupled to quantum light, described by projected low-energy models such as those obtained within tight-binding methods. Drawing from recent results in the field of…

Strongly Correlated Electrons · Physics 2021-03-12 Olesia Dmytruk , Marco Schiró

Time-dependent light-matter interactions are a widespread means by which to describe controllable experimental operations. They can be viewed as an approximation in which a third system - the control system - is treated as external within…

Quantum Physics · Physics 2021-02-11 Adam Stokes , Ahsan Nazir

We present a generalized velocity gauge form of the relativistic laser-matter interaction. In comparison with the (equivalent) regular minimal coupling description, this new form of the light-matter interaction results in superior…

We study the different ways of introducing light-matter interaction in first-principle tight-binding (TB) models. The standard way of describing optical properties is the velocity gauge, defined by linear coupling to the vector potential.…

Materials Science · Physics 2021-04-21 Michael Schüler , Jacob A. Marks , Yuta Murakami , Chunjing Jia , Thomas P. Devereaux

We present three schemes to go beyond the electric-dipole approximation in X-ray absorption spectroscopy calculations within a four-component relativistic framework. The first is based on the full semi-classical light-matter interaction…

Chemical Physics · Physics 2021-07-02 Nanna Holmgaard List , Timothé Romain Léo Melin , Martin van Horn , Trond Saue

In two nearby atoms, the dipole-dipole interaction can couple transitions with orthogonal dipole moments. This orthogonal coupling accounts for a number of interesting effects, but strongly depends on the geometry of the setup. Here, we…

Quantum Physics · Physics 2009-11-13 S. I. Schmid , J. Evers

We study the fundamental limits of the precision of estimating parameters of a quantum matter system when it is probed by a travelling pulse of quantum light. In particular, we focus on the estimation of the interaction strength between the…

Quantum Physics · Physics 2023-06-05 Francesco Albarelli , Evangelia Bisketzi , Aiman Khan , Animesh Datta

In this note we discuss the invariance under general changes of reference frame of all the physical predictions of particle detector models in quantum field theory in general and, in particular, of those used in quantum optics to model…

Quantum Physics · Physics 2018-08-10 Eduardo Martin-Martinez , Pablo Rodriguez-Lopez

When atoms and molecules are ionized by laser pulses of finite duration and increasingly high intensities, the validity of the much used dipole approximation, in which the spatial dependence and magnetic component of the external field are…

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