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Guided by perturbative analysis, we improve the accuracy of Aufbau suppressed coupled cluster theory in simple single excitations, multi-configurational single excitations, and charge transfer excitations while keeping the cost of its…

Chemical Physics · Physics 2025-03-26 Harrison Tuckman , Ziheng Ma , Eric Neuscamman

We report a complete implementation of the coupled-cluster method with single, double, and triple excitations (CCSDT) where tensor decompositions are used to reduce its scaling and overall computational costs. For the decomposition of the…

Chemical Physics · Physics 2020-02-20 Michał Lesiuk

We investigate the ability of Aufbau suppressed coupled cluster theory to act as a post-linear-response correction to widely used linear response methods for electronically excited states. We find that the theory is highly resilient to…

Chemical Physics · Physics 2025-06-23 Trine Kay Quady , Harrison Tuckman , Eric Neuscamman

We present a new linked cluster expansion for calculating properties of multiparticle excitation spectra to high orders. We use it to obtain the two-particle spectra for systems of coupled spin-half dimers. We find that even for weakly…

Strongly Correlated Electrons · Physics 2008-03-26 S. Trebst , H. Monien , C. J. Hamer , Z. Weihong , R. R. P. Singh

In this paper we investigate a particular possibility to extend C(1,3) conformal symmetry using Heisenberg operators, and a related possibility to extend conformal supersymmetry using parabose operators. The symmetry proposed is of a simple…

High Energy Physics - Theory · Physics 2007-05-23 Igor Salom

A strong-coupling expansion for models of correlated electrons in any dimension is presented. The method is applied to the Hubbard model in $d$ dimensions and compared with numerical results in $d=1$. Third order expansion of the Green…

Strongly Correlated Electrons · Physics 2009-10-30 Stéphane Pairault , David Sénéchal , A. -M. S. Tremblay

Computationally efficient and accurate quantum mechanical approximations to solve the many-electron Schr\"odinger equation are at the heart of computational materials science. In that respect the coupled cluster hierarchy of methods plays a…

Materials Science · Physics 2022-01-11 Tina N. Mihm , Tobias Schäfer , Sai Kumar Ramadugu , Andreas Grüneis , James J. Shepherd

We tabulate angularly reduced fourth-order many-body corrections to matrix elements for univalent atoms, derived in [A. Derevianko and E.D. Emmons, Phys. Rev. A 65, 052115 (2002)]. In particular we focused on practically important diagrams…

Atomic Physics · Physics 2007-05-23 Andrei Derevianko

Tensor network contraction on arbitrary graphs is a fundamental computational challenge with applications ranging from quantum simulation to error correction. While belief propagation (BP) provides a powerful approximation algorithm for…

Quantum Physics · Physics 2025-10-28 Siddhant Midha , Yifan F. Zhang

The coupled-cluster method is applied to the spin-1/2 antiferromagnetic XXZ model on a square lattice by employing an approximation which contains two-body long-range correlations and high-order four-body local correlations. Improvement is…

Strongly Correlated Electrons · Physics 2015-05-28 Mohammad Merdan , Y. Xian

Recently, within the context of the phase space coherent state path integral quantisation of constrained systems, John Klauder introduced a reproducing kernel for gauge invariant physical states, which involves a projection operator onto…

High Energy Physics - Theory · Physics 2008-11-26 Jan Govaerts

We suggest a new technique of the asymptotic heat kernel expansion for minimal higher derivative operators of a generic $2M$-th order, $F(\nabla)=(-\Box)^M+\cdots$, in the background field formalism of gauge theories and quantum gravity.…

High Energy Physics - Theory · Physics 2024-12-03 Andrei O. Barvinsky , Alexander V. Kurov , Władysław Wachowski

The most general operator product expansion in conformal field theory is obtained using the embedding space formalism and a new uplift for general quasi-primary operators. The uplift introduced here, based on quasi-primary operators with…

High Energy Physics - Theory · Physics 2020-07-15 Jean-François Fortin , Witold Skiba

We analyze the tensor network loop cluster expansion, introduced in [G. Park, J. Gray, and G. K.-L. Chan, Phys. Rev. B 112, 174310 (2025)] as a systematic correction to belief propagation, in the context of general quantum many-body…

In many instances one has to deal with parametric models. Such models in vector spaces are connected to a linear map. The reproducing kernel Hilbert space and affine- / linear- representations in terms of tensor products are directly…

Numerical Analysis · Mathematics 2018-11-26 Hermann G. Matthies , Roger Ohayon

In this paper, we report on a correctly scaling novel coupled cluster singles and doubles (CCSD) implementation for arbitrary high-spin open-shell states. The chosen cluster operator is completely spin-free, i.e. employs spatial…

Chemical Physics · Physics 2022-02-23 Nils Herrmann , Michael Hanrath

We reveal limitations of several standard coupled-cluster (CC) methods with perturbation-theorybased noniterative or approximate iterative treatments of triple excitations when applied to thedetermination of highly accurate potential energy…

Chemical Physics · Physics 2021-10-04 Jan Schnabel , Lan Cheng , Andreas Köhn

We present an excited-state-specific coupled-cluster approach in which both the molecular orbitals and cluster amplitudes are optimized for an individual excited state. The theory is formulated via a pseudoprojection of the traditional…

Chemical Physics · Physics 2023-11-27 Harrison Tuckman , Eric Neuscamman

While either spin or point-group adaptation is straightforward when considered independently, the standard technique for factoring isotropic spin Hamiltonians by the total spin S and the irreducible representation of the point-group is…

Strongly Correlated Electrons · Physics 2025-06-24 Shadan Ghassemi Tabrizi , Thomas D. Kühne

We show that the Zassenhaus decomposition for the exponential of the sum of two non-commuting operators, simplifies drastically when these operators satisfy a simple condition, called the no-mixed adjoint property. An important application…

Mathematical Physics · Physics 2026-04-08 Louis Jourdan , Patrick Cassam-Chenaï