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We present a general theory for using an optically pumped diamond nitrogen-vacancy center as a tunable, non-equilibrium bath to control a variety of nuclear spin dynamics (such as dephasing, relaxation, squeezing, polarization, etc.) and…

Quantum Physics · Physics 2019-08-17 Ping Wang , Jiangfeng Du , Wen Yang

Imaging of microwave magnetic fields with nano-scale resolution has interesting applications. Specifically, detecting the orientation of the microwave fields is useful in condensed matter physics and quantum control. However, most of the…

Quantum Physics · Physics 2026-01-13 Akshat Rana , Pooja Lamba , Atanu Ghosh , Siddharth Dhomkar , Rama K. Kamineni

Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Ulf Bissbort , Mikhail D. Lukin , Ronald L. Walsworth , Paola Cappellaro

Sensitive nanoscale magnetic resonance imaging (MRI) of target spins using nitrogen-vacancy (NV) centers in diamond will require a quantitative understanding of dominant noise at the surface. We probe this noise by applying dynamical…

Mesoscale and Nanoscale Physics · Physics 2014-07-11 Bryan A. Myers , Matthieu C. Dartiailh , Kenichi Ohno , Ananda Das , David D. Awschalom , Ania C. Bleszynski Jayich

Surface-functionalized nanomaterials can act as theranostic agents that detect disease and track biological processes using hyperpolarized magnetic resonance imaging (MRI). Candidate materials are sparse however, requiring spinful nuclei…

Nitrogen-vacancy (NV) defect in diamond is a very promising tool for numerous sensing applications like magnetometry or thermometry. In this paper, we demonstrate a compact and convenient device for magnetic field imaging where a commercial…

Mesoscale and Nanoscale Physics · Physics 2016-05-10 Ludovic Mayer , Thierry Debuisschert

Understanding the profile of a qubit's wavefunction is key to its quantum applications. Unlike conducting systems, where a scanning tunneling microscope can be used to probe the electron distribution, there is no direct method for…

The ability to create time-dependent magnetic fields of controlled polarization is essential for many experiments with magnetic resonance. We describe a microstrip circuit that allows us to generate strong magnetic field at microwave…

Atomic Physics · Physics 2015-05-28 Mariusz Mrozek , Janusz Mlynarczyk , Daniel S. Rudnicki , Wojciech Gawlik

We demonstrate preferential orientation of nitrogen-vacancy (NV) color centers along two of four possible crystallographic axes in diamonds grown by chemical vapor deposition on the {100} face. We identify the relevant growth regime and…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 L. M. Pham , N. Bar-Gill , D. Le Sage , A. Stacey , M. Markham , D. J. Twitchen , M. D. Lukin , R. L. Walsworth

Dynamic Nuclear Polarization (DNP) is to date the most effective technique to increase the nuclear polarization up to a factor $100,000$ opening disruptive perspectives for medical applications. In DNP, the nuclear spins are driven to an -…

Strongly Correlated Electrons · Physics 2015-08-26 Andrea De Luca , Alberto Rosso

The decoherence of point defect qubits is often governed by the electron spin-nuclear spin hyperfine interaction that can be parameterized by using ab inito calculations in principle. So far most of the theoretical works have focused on the…

Quantum Physics · Physics 2024-05-10 István Takács , Viktor Ivády

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high…

Quantum Physics · Physics 2024-09-06 Zhiyi Hu , Fengjian Jiang , Jingyan He , Yulin Dai , Ya Wang , Nanyang Xu , Jiangfeng Du

Magnetic spin resonance is a key non-invasive sensing and imaging technique across the life-, material- and fundamental sciences with further medical and commercial applications. Recent advances using paramagnetic color centers enable…

Mesoscale and Nanoscale Physics · Physics 2018-07-24 Florestan Ziem , Marwa Garsi , Helmut Fedder , Jörg Wrachtrup

Nuclear magnetic resonance (NMR) imaging with shallow nitrogen-vacancy (NV) centers in diamond offers an exciting route toward sensitive and localized chemical characterization at the nanoscale. Remarkable progress has been made to combat…

We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…

Optical coupling enables intermediate- and long-range interactions between distant quantum emitters. Such interaction may be the basic element in bottom-up approaches of coupled spin systems or for integrated quantum photonics and quantum…

We discuss the side resonances of optically detected magnetic resonance in diamond crystal and propose the new approach to the calculation of hyperfine interaction in composed system, consisted of negatively charged nitrogen-vacancy NV-…

Mesoscale and Nanoscale Physics · Physics 2017-01-17 Alexander Ivanov , Alexei Ivanov

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

Dynamic nuclear polarization (DNP) is an attractive method for initializing nuclear spins that are strongly coupled to optically active electron spins because it functions at room temperature and does not require strong magnetic fields. In…

We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and…