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We report the connection between the stacking order and magnetic properties of bilayer CrI$_3$ using first-principles calculations. We show that the stacking order defines the magnetic ground state. By changing the interlayer stacking order…

Materials Science · Physics 2018-11-19 Nikhil Sivadas , Satoshi Okamoto , Xiaodong Xu , Craig. J. Fennie , Di Xiao

Aiming to clarify the mechanisms governing the interlayer magnetic coupling, we have investigated the stacking energy and interlayer magnetism of bilayer CrBr$_3$ systemically. The magnetic ground states of bilayer CrBr$_3$ with different…

Mesoscale and Nanoscale Physics · Physics 2020-11-06 Jun-Shan Si , Hongxing Li , Bin-Guang He , Zi-Peng Cheng , Wei-Bing Zhang

We use a first-principles calculations approach to reveal the electronic and magnetic properties of chromium diiodide (CrI$_2$) bilayers and establish a hierarchy of magnetic interactions across stable registries. The monolayer presents a…

Materials Science · Physics 2025-12-23 B. Valdés-Toro , I. Ferreira-Araya , R. A. Gallardo , J. W. González

The interlayer magnetic interaction in bilayer CrI$_3$ plays a crucial role for its device applications. In this work, we studied the interlayer magnetic interaction in $\pi/3$-twisted bilayer CrI$_3$ using first-principles calculations.…

Materials Science · Physics 2022-01-11 Haodong Yu , Jize Zhao , Fawei Zheng

Stacking order can significantly influence the physical properties of two-dimensional (2D) van der Waals materials. The recent isolation of atomically thin magnetic materials opens the door for control and design of magnetism via stacking…

In twisted two-dimensional (2D) magnets, the stacking dependence of the magnetic exchange interaction can lead to regions of ferromagnetic and antiferromagnetic interlayer order, separated by non-collinear, skyrmion-like spin textures.…

We address the interplay between stacking and interlayer exchange for ferromagnetically ordered CrI$_3$, both for bilayers and bulk. Whereas bulk CrI$_3$ is ferromagnetic, both magneto-optical and transport experiments show that interlayer…

Mesoscale and Nanoscale Physics · Physics 2019-08-29 D. Soriano , C. Cardoso , J. Fernández-Rossier

The physical properties of two-dimensional van der Waals (2D vdW) crystals depend sensitively on the interlayer coupling, which is intimately connected to the stacking arrangement and the interlayer spacing. For example, simply changing the…

Controlling the crystal structure is a powerful approach for manipulating the fundamental properties of solids. Unique to two-dimensional (2D) van der Waals materials, the control can be achieved by modifying the stacking order through…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Weijong Chen , Zeyuan Sun , Lehua Gu , Xiaodong Xu , Shiwei Wu , Chunlei Gao

Recently intrinsic ferromagnetism in two-dimensional(2D) van der Waals materials was discovered [1, 2, 3]. A monolayer of Chromiun triiodide(CrI3) is ferromagnetic while a bilayer structure was reported to be anti-ferro magnetic, moreover…

Materials Science · Physics 2018-11-30 E. Suarez Morell , Andrea León , R. Hiroki Miwa , P. Vargas

Long-range magnetic orders in atomically thin ferromagnetic CrI3 give rise to new fascinating physics and application perspectives. The physical properties of two-dimensional (2D) ferromagnetism CrI3 are significantly influenced by…

Materials Science · Physics 2019-11-13 Kai Guo , Bowen Deng , Zhongtai Shi , Yue Li , Xin Wang , Lei Bi , Li Zhang , Haipeng Lu , Peiheng Zhou , Linbo Zhang , Yingchun Cheng , Bo Peng

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

Materials Science · Physics 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

Recently, two-dimensional (2D) bilayer magnetic systems have been widely studied. Their interlayer magnetic interactions play a vital role in the magnetic properties. In this paper, we theoretically studied the interlayer magnetic…

Materials Science · Physics 2025-09-10 Wenqi Yang , Xinlong Yang , Menglei Li , Lin Hu , Fawei Zheng

The emergence of two-dimensional (2D) magnetic crystals and moir\'e engineering has opened the door for devising new magnetic ground states via competing interactions in moir\'e superlattices. Although a suite of interesting phenomena,…

Chromium trihalides, CrX$_3$ (with X = Cl, Br, I), are a family of layered magnetic materials that can be easily exfoliated to provide ferromagnetic monolayers. When two layers are stacked together to form a bilayer the interlayer exchange…

Materials Science · Physics 2020-12-30 Marco Gibertini

Two-dimensional(2D) multiferroic materials hold significant promise for advancing the miniaturization and integration of nanodevices. In this study, we demonstrate that 2D bilayer ScI2, which exhibits ferromagnetic(FM) ordering within each…

Materials Science · Physics 2026-03-03 Yaxin Pan , Chongze Wang , Shuyuan Liu , Fengzhu Ren , Chang Liu , Bing Wang , Jun-Hyung Cho

The atomic thickness of two-dimensional (2D) materials provides a unique opportunity to control material properties and engineer new functionalities by electrostatic doping. Electrostatic doping has been demonstrated to tune the electrical…

Materials Science · Physics 2018-08-01 Shengwei Jiang , Lizhong Li , Zefang Wang , Kin Fai Mak , Jie Shan

A monolayer of CrI$_3$ is a two-dimensional crystal that in its equilibrium configuration is a ferromagnetic semiconductor, however, two coupled layers can be ferromagnetic or antiferromagnetic depending on the stacking. We study the…

Mesoscale and Nanoscale Physics · Physics 2020-04-07 Andrea Leon , J. W. González , J. Mejía-López , F. Crasto de Lima , E. Suárez Morell

The manipulation of two-dimensional (2D) magnetic order is of significant importance to facilitate future 2D magnets for low-power and high-speed spintronic devices. Van der Waals stacking engineering makes promises for controllable…

Motivated by the potential of atomically-thin magnets towards tunable high-frequency magnonics, we detail the spin-wave dispersion of bilayer CrI$_3$. We demonstrate that the magnonic behavior of the bilayer strongly depends on its stacking…

Materials Science · Physics 2023-03-01 M. Soenen , C. Bacaksiz , R. M. Menezes , M. V. Milosevic
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