Related papers: Coherent multidimensional spectroscopy of dilute g…
This thesis describes capacitance and tunneling experiments performed on two-dimensional electron gas (2DEG) and quantum dot systems. It develops a system of equations that allow determination, by means of capacitance measurements, of the…
Two-dimensional electronic spectroscopy (2DES) has enabled significant discoveries in both biological and synthetic energy-transducing systems. Although deriving chemical information from 2DES is a complex task, machine learning (ML) offers…
Electrostatic confinement in semiconductors provides a flexible platform for the emulation of interacting electrons in a two-dimensional lattice, including in the presence of gauge fields. This combination offers the potential to realize a…
Multidimensional spectroscopy has a long history originating from nuclear magnetic resonance, and has now found widespread application at infrared and optical frequencies as well. However, the energy scales of traditional multidimensional…
Simulating the irreversible quantum dynamics of exciton and electron transfer problems poses a nontrivial challenge. Because the irreversibility of the system dynamics is a result of quantum thermal activation and dissipation caused by the…
Ultracold dilute gases provide ideal settings for measurements of atomic structure. Helium has an internal structure sufficiently simple to permit highly accurate predictions of its resonances and transition rates. Precise laser…
In quantum computation, it is of paramount importance to locate the parameter space where maximal coherence can be preserved in the qubit system. In recent years environment-induced decoherence based the quantum Brownian motion (QBM) models…
This work presents novel discrete event-based simulation algorithms based on the Quantized State System (QSS) numerical methods. QSS provides attractive features for particle transportation processes, in particular a very efficient handling…
Among very low disorder systems of condensed matter, the high mobility two-dimensional electron gas confined in gallium arsenide/aluminum gallium arsenide heterostructures holds a privileged position as platform for the discovery of new…
The multi-mode anharmonic Brownian motion model provides a universal framework for simulating molecular vibrations in condensed phases. When vibrational energy surpasses thermal excitation, quantum effects become significant, necessitating…
A highly conductive metallic gas that is quantum mechanically confined at a solid-state interface is an ideal platform to explore nontrivial electronic states that are otherwise inaccessible in bulk materials. Although two-dimensional…
The advent of bottom-up atomic manipulation heralded a new horizon for attainable information density, as it allowed a bit of information to be represented by a single atom. The discrete spacing between atoms in condensed matter has thus…
This article provides a review of recent work in the field of helium nanodroplet spectroscopy with emphasis on the dynamical aspects of the interactions between molecules in helium as well as their interaction with this unique quantum…
Controlling atom-photon interactions in engineered environments is central to quantum optics and emerging quantum technologies. Non-Hermitian (NH) photonic baths, where dissipation fundamentally reshapes spectral and dynamical properties,…
Ultracold atom gases provide model systems in which many-body quantum physics phenomena can be studied. Recent experiments on Fermi gases have realized a phase transition to a Fermi superfluid state with strong interparticle interactions.…
Is it possible to infer the time evolving quantum state of a multichromophoric system from a sequence of two-dimensional electronic spectra (2D-ES) as a function of waiting time? Here we provide a positive answer for a tractable model…
Dissipation is unavoidable in quantum systems. It usually induces decoherences and changes quantum correlations. To access the information of strongly correlated quantum matters, one has to overcome or suppress dissipation to extract out…
This article provides an overview, primarily from an experimental perspective, of recent progress and future prospects in using helium to realize a range of quantum materials of generic interest, by "top-down" and "bottom-up"…
Electronic energy transfer in photosynthesis occurs over a range of time scales and under a variety of intermolecular coupling conditions. Recent work has shown that electronic coupling between chromophores can lead to coherent oscillations…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…