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The triangular spin lattice of NiBr$_{2}$ is a canonical example of a frustrated helimagnet that shows a temperature-driven phase transition from a collinear commensurate antiferromagnetic structure to an incommensurate spin helix on…

Materials Science · Physics 2019-03-19 S. Babu , K. Prokes , Y. K. Huang , F. Radu , S. K. Mishra

We have discovered a novel candidate for a spin liquid state in a ruthenium oxide composed of dimers of $S = $ 3/2 spins of Ru$^{5+}$,Ba$_3$ZnRu$_2$O$_9$. This compound lacks a long range order down to 37 mK, which is a temperature…

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Recent numerical work (Nature 464, 847 (2010)) indicates the existence of a spin liquid phase (SL) that intervenes between the antiferromagnetic and semimetallic phases of the half filled Hubbard model on a honeycomb lattice. To better…

Strongly Correlated Electrons · Physics 2011-08-18 B. K. Clark , D. A. Abanin , S. L. Sondhi

We report the discovery of a novel gapless quantum spin liquid in the S=1 honeycomb system Cu$_3$LiRu$_2$O$_6$ with Ru$^{4+}$ ($4d^4$) where moments remain dynamic down to 50 mK. Heat capacity measurements show no sign of magnetic ordering…

$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…

We investigate the ground-state and finite-temperature properties of the bond-random $s=1/2$ Heisenberg model on a honeycomb lattice with frustrated nearest- and next-nearest-neighbor antiferromagnetic interactions, $J_1$ and $J_2$, by the…

Strongly Correlated Electrons · Physics 2018-10-24 Kazuki Uematsu , Hikaru Kawamura

We report the signatures of dynamic spin fluctuations in the layered honeycomb Li$_3$Cu$_2$SbO$_6$ compound, with a 3$d$ S = 1/2 $d^9$ Cu$^{2+}$ configuration, through muon spin rotation and relaxation ($\mu$SR) and neutron scattering…

The description and detection of unconventional magnetic states such as spin liquids is a recurring topic in condensed matter physics. While much of the efforts have traditionally been directed at geometrically frustrated antiferromagnets,…

Strongly Correlated Electrons · Physics 2018-05-25 L. Bovo , M. Twengström , O. A. Petrenko , T. Fennell , M. J. P. Gingras , S. T. Bramwell , P. Henelius

We carried out inelastic neutron scattering experiments on a buckled honeycomb lattice antiferromagnet Ba$_{2}$NiTeO$_{6}$ exhibiting a stripe structure at a low temperature. Magnetic excitations are observed in the energy range of $\hbar…

Strongly Correlated Electrons · Physics 2017-10-11 Shinichiro Asai , Minoru Soda , Kazuhiro Kasatani , Toshio Ono , V. Ovidiu Garlea , Barry Winn , Takatsugu Masuda

Quantum fluctuations endow spin systems with surprisingly enriched magnetic phase diagrams. In frustrated magnets, strong quantum fluctuations boosted by either geometrical incompatibility or competitive exchange interactions stabilize…

We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional…

We study a spin model on honeycomb lattice with two types of Heisenberg exchange couplings, $J$ and $\tilde J$, where $J$ is for the conventional spin and and $\tilde J$ for rotated spin. When $\tilde J=0$, this is the conventional…

Strongly Correlated Electrons · Physics 2015-06-04 Yue Yu , Long Liang , Qian Niu , Shaojing Qin

Despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K, the Tb2Ti2O7 pyrochlore magnetic material lacks long range magnetic order down to at least $T^*\approx 50$ mK. It has recently been proposed that the low temperature collective…

Statistical Mechanics · Physics 2009-05-07 Hamid R. Molavian , Michel J. P. Gingras

Spiral spin liquids are correlated states of matter in which a frustrated magnetic system evades order by fluctuating between a set of (nearly) degenerate spin spirals. Here, we investigate the response of spiral spin liquids to quenched…

Strongly Correlated Electrons · Physics 2024-02-29 Pedro M. Cônsoli , Matthias Vojta

The magnetic response of antiferromagnetic CsO2, coming from the p-orbital S=1/2 spins of anionic O2- molecules, is followed by 133Cs nuclear magnetic resonance across the structural phase transition occuring at Ts1=61 K on cooling. Above…

Strongly Correlated Electrons · Physics 2018-04-16 M. Klanjsek , D. Arcon , A. Sans , P. Adler , M. Jansen , C. Felser

Geometric frustration among competing spin exchanges can give rise to novel quantum phases by enhancing fluctuations that drive magnetic systems beyond the classical regime. We investigate the frustrated array of strongly correlated spin…

Anderson proposed structural topology in frustrated magnets hosting novel quantum spin liquids (QSLs). The QSL state is indeed exactly derived by fractionalizing the spin excitation into spinless Majorana fermions in a perfect two…

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…