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The photoinduced switching of Fe(II)-based spin-crossover complexes from singlet to quintet takes place at ultrafast time scales. This a priori spin-forbidden transition triggered numerous time-resolved experiments of solvated samples to…

We propose a new pulse sequence for dynamical averaging of the dipole-dipole interactions and inhomogeneities of the magnetic fields in the nuclear spin system. The sequence contains a short cycle of the periodic resonant pulse excitation…

Quantum Physics · Physics 2015-03-05 S. A. Moiseev , V. A. Skrebnev

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…

Optics · Physics 2024-01-02 Xiaoyu Mi , Ming Zhang , Zheng Li

We show that ultrashort pulses can be focused, in a particular instant, to a spot size given by the wavelength associated with its spectral width. For attosecond pulses this spot size is within the nanometer scale. Then we show that a…

Quantum Physics · Physics 2016-08-31 Patrick Maurer , J. Ignacio Cirac , Oriol Romero-Isart

Superradiant phase transition represents an important quantum phenomenon that shows the collective excitations based on the coupling between atoms and cavity modes. The spin-orbit coupling is another quantum effect which induced from the…

Quantum Gases · Physics 2021-05-26 Ying Lei , Shaoliang Zhang

Ultrashort spin current pulses have a great potential of becoming the carriers of information in future ultrafast spintronics. They present the outstanding property of an extremely compressed time profile, which can allow for the building…

Materials Science · Physics 2018-03-28 Marco Battiato

Understanding the nature of magnetic interactions in ultra-small magnetic ensembles and their intrinsic properties is vital to uncover the dynamics therein. In this study we reveal the spin dynamics of hexagonally arranged Fe atoms on…

Mesoscale and Nanoscale Physics · Physics 2018-08-21 Tamene R. Dasa , Valeri S. Stepanyuk

We consider strongly interacting systems of effective spins, subject to dissipative spin-flip processes associated with optical pumping. We predict the existence of novel magnetic phases in the steady-state of this system, which emerge due…

Quantum Gases · Physics 2013-06-21 Tony E. Lee , Sarang Gopalakrishnan , Mikhail D. Lukin

We present a new class of control pulses designed to transfer co-located ensembles without relying on frequency selectivity, thereby allowing much faster state-transitions. A geometric approach allows us to construct sequences which are…

Atomic Physics · Physics 2026-04-23 K. L. Wood , W. A. Terrano

Different energy shifts for majority and minority electrons occur. Thus, for example in case of (laser) excited ferromagnetic metals majority and minority electrons may respond differently in time during closing the exchange splitting. Spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-27 M. Avignon , K. H. Bennemann

Ultrafast phenomena on a femtosecond timescale are commonly examined by pump-probe experiments. This implies multiple measurements where the sample under investigation is pumped with a short light pulse and then probed with a second pulse…

The last decade has witnessed a rapid advancement in laser technology, enabling the direct monitoring and control of electronic motion on its natural attosecond to sub-femtosecond timescales. Ultrafast processes are conventionally studied…

Chemical Physics · Physics 2026-05-27 Torsha Moitra

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

We consider the full driven quantum dynamics of a qubit realized as spin of electron in a one-dimensional double quantum dot with spin-orbit coupling. The driving perturbation is taken in the form of a single half-period pulse of electric…

Mesoscale and Nanoscale Physics · Physics 2010-09-28 D. V. Khomitsky , E. Ya. Sherman

We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Stefano Chesi , W. A. Coish

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

We study the dynamics of an electron spin in a graphene quantum dot, which is interacting with a bath of less than ten nuclear spins via the anisotropic hyperfine interaction. Due to substantial progress in the fabrication of graphene…

Mesoscale and Nanoscale Physics · Physics 2014-01-09 Moritz Fuchs , John Schliemann , Björn Trauzettel

We report a study on the ultrafast coherent population oscillations (UCPO) in two level atoms induced by the frequency modulated few-cycle optical pulse train. The phenomenon of UCPO is investigated by numerically solving the optical Bloch…

Optics · Physics 2013-05-30 Parvendra Kumar , Amarendra K. Sarma

We investigate the interaction of femtosecond laser pulses with spins including relativistic corrections. The time-ordered magneto-optical signals corresponding to a pump-probe configuration are calculated in the case of one electron…

Strongly Correlated Electrons · Physics 2012-01-04 Hélène Vonesch , Jean-Yves Bigot