Related papers: Ultrafast dissipative spin-state dynamics triggere…
We review theoretical foundations and some recent progress related to the quest of controlling the motion of charge carriers with intense laser pulses and optical waveforms. The tools and techniques of attosecond science enable detailed…
Intense, few-cycle pulses in the terahertz frequency range have strong potential for schemes of control over vibrational modes in solid-state materials in the electronic ground-state. Here we report an experiment using single cycle…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
We use R-Matrix with Time-dependence (RMT) theory, with spin-orbit effects included, to study krypton irradiated by two time-delayed XUV ultrashort pulses. The first pulse excites the atom to 4s$^{2}$4p$^{5}$5s. The second pulse then…
In the field of femtomagnetism magnetic matter is controlled by ultrafast laser pulses; here we show that coupling phonon excitations of the nuclei to spin and charge leads to femto-phono-magnetism, a powerful route to control magnetic…
In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…
We report entanglement of a single atom's hyperfine spin state with its motional state in a timescale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of +/- 2 hbar k. Using…
Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…
Transport through spin-blockaded quantum dots provides a means for electrical control and detection of nuclear spin dynamics in the host material. Although such experiments have become increasingly popular in recent years, interpretation of…
Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…
We present a model describing the use of ultra-short strong pulses to control the population of the excited level of a two-level quantum system. In particular, we study an off-resonance excitation with a few cycles pulse which presents a…
The discovery of femtosecond laser-induced ultrafast demagnetization in 1996 opened a new field, femtomagnetism, in which magnetic order can be quenched on timescales shorter than a picosecond. This seminal observation revealed that angular…
We study the emission of femtosecond spin current pulses at Fe/Au interfaces. Using optical second harmonic generation we demonstrate the control of pulse shape and duration by varying the emitter thickness and show that it is determined by…
We investigate the spin-resolved electron dynamics in a double quantum dot driven by ultrafast asymmetric electromagnetic pulses. Using a analytical model we show that applying an appropriate pulse sequence allows to control coherently the…
We use a non-equilibrium many-body theory that engages the elements of transient coherence, correlation, and nonlinearity to describe changes in the magnetic and electronic phases of strongly correlated systems induced by femtosecond…
Manipulating spin in antiferromagnetic (AFM) materials has great potential in AFM opto-spintronics. Laser pulses can induce a transient ferromagnetic (FM) state in AFM metallic systems, but have never been proven in two-dimensional (2D) AFM…
Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…
We investigate the problem of two-level atoms driven by an ultrashort pulse train in the frequency domain. At low intensity regime, we obtain a perturbative analytical solution that allows us to discuss the role of the mode number of the…
In quantum systems, coherent superpositions of electronic states evolve on ultrafast timescales (few femtosecond to attosecond, 1 as = 0.001 fs = 10^{-18} s), leading to a time dependent charge density. Here we exploit the first attosecond…
In some applications of quantum control, it is necessary to produce very weak excitation of a quantum system. Such an example is presented by the concept of single-photon generation in cold atomic ensembles or doped solids, e.g. by the DLCZ…