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Recent developments of the sources of intense and ultrashort X-ray pulses stimulate theoretical studies of phenomena occurring on ultrafast timescales. In the present study, spin-flip dynamics in transition metal complexes triggered by…

Chemical Physics · Physics 2020-08-26 Vladislav Kochetov , Huihui Wang , Sergey I. Bokarev

Recent developments in attosecond spectroscopy yield access to the correlated motion of electrons on their intrinsic time scales. Spin-flip dynamics is usually considered in the context of valence electronic states, where spin-orbit…

Atomic and Molecular Clusters · Physics 2017-08-02 H. Wang , S. I. Bokarev , S. G. Aziz , O. Kühn

Recent advances in attosecond physics provide access to the correlated motion of valence and core electrons on their intrinsic timescales. For valence excitations, processes related to the electron spin are usually driven by nuclear motion.…

Chemical Physics · Physics 2017-01-18 Huihui Wang , Sergey I. Bokarev , Saadullah G. Aziz , O. Kühn

This article gives an overview on recent theoretical progress in controlling the charge and spin dynamics in low-dimensional electronic systems by means of ultrashort and ultrabroadband electromagnetic pulses. A particular focus is put on…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Andrey S. Moskalenko , Zhen-Gang Zhu , Jamal Berakdar

Theoretical analyses of ultrafast spin dynamics commonly address and discuss simulated phenomena by means of observables, whereas in quantum information theory one often utilizes measures of quantum states. In this Paper we report on…

Mesoscale and Nanoscale Physics · Physics 2023-02-15 Franziska Ziolkowski , Oliver Busch , Ingrid Mertig , Jürgen Henk

Ultrafast electronic dynamics are typically studied using pulsed lasers. We demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique…

Spintronics had a widespread impact over the past decades due to transferring information by spin rather than electric currents. Its further development requires miniaturization and reduction of characteristic timescales of spin dynamics…

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

Ultrafast magnetization dynamics probes the most fundamental properties of magnetic materials, exploring questions about the fundamental interactions responsible for magnetic phenomena. Thermal effects are known to be extremely important…

Materials Science · Physics 2019-08-26 Daniel Meilak , Sarah Jenkins , Rory Pond , Richard F. L. Evans

Damping effects form the core of many emerging concepts for high-speed spintronic applications. Important characteristics such as device switching times and magnetic domain-wall velocities depend critically on the damping rate. While the…

Materials Science · Physics 2020-12-08 Christian Tzschaschel , Takuya Satoh , Manfred Fiebig

We investigate ultrafast vibronic dynamics triggered by intense femtosecond infrared pulses in small molecules. Our study is based on numerical simulations performed with 2D model molecules, and analyzed in the perspective of the renown…

Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

Strongly Correlated Electrons · Physics 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

Optical pulses are routinely used to drive dynamical changes in the properties of solids. In quantum materials, many new phenomena have been discovered, including ultrafast transitions between electronic phases, switching of ferroic orders…

Strongly Correlated Electrons · Physics 2018-05-08 Michele Buzzi , Michael Först , Roman Mankowsky , Andrea Cavalleri

The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…

Chemical Physics · Physics 2017-02-08 W. A. Bryan , C. R. Calvert , R. B. King , J. B. Greenwood , W. R. Newell , I. D. Williams

We explore the dynamics and the steady state of a driven quantum spin coupled to a bath of fermions, which can be realized with a strongly imbalanced mixture of ultracold atoms using currently available experimental tools. Radio-frequency…

Quantum Gases · Physics 2014-01-06 Michael Knap , Dmitry A. Abanin , Eugene Demler

Ultrashort optical pulses are a cornerstone for manipulating electronic and magnetic states in materials on a femtosecond timescale. Conventional models assume that optical excitation primarily modifies the occupation of the electron energy…

Materials Science · Physics 2025-05-12 Sergii Parchenko , Peter M. Oppeneer , Andreas Scherz

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

The field of spintronics involves the study of both spin and charge transport in solid state devices with a view toward increasing their functionality and efficiency. Alternatively, the field of ultrafast magnetism focuses on the use of…

Mesoscale and Nanoscale Physics · Physics 2017-11-07 Yang Yang , R. B. Wilson , Jon Gorchon , Charles-Henri Lambert , Sayeef Salahuddin , Jeffrey Bokor

Using an ultrashort laser pulse we explore {\it ab-initio} the spin dynamics of Gd$_x$(FeCo)$_{1-x}$ at femtosecond time scales. Optical excitations are found to drive charge from Fe majority $d$-states to the unoccupied Gd $f$-minority…

Materials Science · Physics 2022-02-16 J. K. Dewhurst , Sam Shallcross , I. E. Radu , P. Elliott , C. v. Korff Schmising , S. Sharma

Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…

Chemical Physics · Physics 2013-04-26 P. A. Carpeggiani , P. Tzallas , A. Palacios , D. Gray , F. Martín , D. Charalambidis
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