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Recent theoretical study has shown that the hexagonal YCo$_5$ is dynamically unstable and distorts into a stable orthorhombic structure. In this study, we show theoretically that the orthorhombic phase is energetically more stable than the…

Materials Science · Physics 2023-07-25 Guangzong Xing , Yoshio Miura , Terumasa Tadano

Synchrotron X-ray diffraction and Raman spectroscopy have been used to study chemical reactions of molecular hydrogen (H2) with sulfur (S) at high pressures. We find theoretically predicted Cccm and Im-3m H3S to be the reaction products at…

Superconductivity · Physics 2017-04-19 Alexander F. Goncharov , Sergey S. Lobanov , Vitali B. Prakapenka , Eran Greenberg

Phase transitions and symmetry are intimately linked. Melting of ice, for example, restores translation invariance. The mysterious hidden order (HO) phase of URu$_2$Si$_2$ has, despite relentless research efforts, kept its symmetry breaking…

Strongly Correlated Electrons · Physics 2019-01-10 J. Choi , O. Ivashko , N. Dennler , D. Aoki , K. von Arx , S. Gerber , O. Gutowski , M. H. Fischer , J. Strempfer , M. v. Zimmermann , J. Chang

The molecular phase of hydrogen converts to the atomic metallic phase at high pressures estimated usually as 300 - 500 GPa. We analyze the decay of metallic phase as the pressure is relieved below the transition one. The metallic state is…

Other Condensed Matter · Physics 2018-01-03 S. N. Burmistrov , L. B. Dubovskii

The electrical conductivity and Raman spectroscopy measurements have been performed on MoS$_2$ at high pressures up to 90 GPa and variable temperatures down to 5 K. We find that the temperature dependence of the resistance in a metallic…

Materials Science · Physics 2018-06-27 Zi-Yu Cao , Jia-Wei Hu , Alexander F. Goncharov , Xiao-Jia Chen

A hexagonal structure of solid molecular hydrogen with $P6_122$ symmetry is calculated to be more stable below about 200 GPa than the monoclinic $C2/c$ structure identified previously as the best candidate for phase III. We find that the…

Materials Science · Physics 2016-11-01 Bartomeu Monserrat , Richard J. Needs , Eugene Gregoryanz , Chris J. Pickard

The structure of solid oxygen has been studied at pressures from 50 to 140~GPa using static structure search methods and molecular dynamics simulations with density functional theory and a hybrid exchange functional. Several crystalline…

Materials Science · Physics 2023-09-26 Sabri F. Elatresh , V. Askarpour , S. A. Bonev

Pressure-induced superconductivity and structural phase transitions in phosphorous (P) are studied by resistivity measurements under pressures up to 170 GPa and fully $ab-initio$ crystal structure and superconductivity calculations up to…

Based on evolutionary crystal structure searches in combination with ab initio calculations, we predict an unusual structural phase of the superconducting LaH$_{10}$ that is stable from about 250 GPa to 425 GPa pressure. This new phase…

Superconductivity · Physics 2021-11-17 Ashok K. Verma , P. Modak , Fabian Schrodi , Alex Aperis , Peter M. Oppeneer

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

Materials Science · Physics 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

We investigated the evolution of ferromagnetism in layered Fe$_3$GeTe$_2$ flakes under different pressures and temperatures using in situ magnetic circular dichroism (MCD) spectroscopy. We found that the rectangle shape of hysteretic loop…

Mesoscale and Nanoscale Physics · Physics 2020-05-08 Heshen Wang , Runzhang Xu , Cai Liu , Le Wang , Zhan Zhang , Huimin Su , Shanmin Wang , Yusheng Zhao , Zhaojun Liu , Dapeng Yu , Jia-Wei Mei , Xiaolong Zou , Jun-Feng Dai

We investigate the structural and magnetic phase transitions in EuTi1-xNbxO3 with synchrotron powder X-ray diffraction (XRD), resonant ultrasound spectroscopy (RUS), and magnetization measurements. Upon Nb-doping, the Pm-3m to I4/mcm…

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

Transition metal dihalides (MX$_2$, M= transition metal, X= halide) have attracted much attention recently due to their intriguing low-dimensional magnetic properties. Particular focus has been placed in this family in the context of…

Materials Science · Physics 2024-04-26 Soumen Bag , Jesse Kapeghian , Onur Erten , Antia S. Botana

The effect of electron doping on the structural, transport, and magnetic properties of Mn (IV) - rich Ca1-xYxMnO3 (x < 0.2) samples have been investigated using neutron diffraction, neutron depolarization, magnetization and resistivity…

Materials Science · Physics 2016-02-09 Neetika Sharma , A. Das , C. L. Prajapat , Amit Kumar , M. R. Singh

Neutron diffraction studies of antiferromagnetic MnO confined to MCM-41 type matrices with channel diameters 24-87 A demonstrate a continuous magnetic phase transition in contrast to a discontinuous first order transition in the bulk. The…

Strongly Correlated Electrons · Physics 2009-11-11 I. V. Golosovsky , I. Mirebeau , V. P. Sakhnenko , D. A. Kurdyukov , Y. A. Kumzerov

Computational searches for structures of solid oxygen under pressures in the multi TPa range have been carried out using density-functional-theory methods. We find that molecular oxygen persists to about 1.9 TPa at which it transforms into…

Materials Science · Physics 2012-07-06 Jian Sun , Miguel Martinez-Canales , Dennis D. Klug , Chris J. Pickard , Richard J. Needs

We studied the crystal structure of TiOCl up to pressures of $p$=25~GPa at room temperature by x-ray powder diffraction measurements. Two pressure-induced structural phase transitions are observed: At $p_{c1}$$\approx$15~GPa emerges an…

Strongly Correlated Electrons · Physics 2015-05-20 J. Ebad-Allah , A. Schönleber , S. van Smaalen , M. Hanfland , M. Klemm , S. Horn , S. Glawion , M. Sing , R. Claessen , C. A. Kuntscher

The electron and phonon spectra, as well as the density of electron and phonon states of the stable orthorhombic structure of hydrogen sulfide (SH2) at pressures 100-180 GPa have been calculated. It is found that the set of parallel planes…

Superconductivity · Physics 2015-07-22 Nikolay Degtyarenko , Evgeny Mazur

We report the temperature dependent x-ray powder diffraction of the quaternary compound NdOFeAs (also called NdFeAsO) in the range between 300 K and 95 K. We have detected the structural phase transition from the tetragonal phase, with…

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