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Experiments on one- and two-photon laser excitation of 232Th+ ions in a radiofrequency ion trap are reported. As the first excitation step, the strongest resonance line at 402 nm from the 6d^2 7s J=3/2 ground state to the 6d7s7p J=5/2 state…

We report electromagnetically induced transparency for the D1 and D2 lines in $^{6}$Li in both a vapour cell and an atomic beam. Electromagnetically induced transparency is created using co-propagating mutually coherent laser beams with a…

Atomic Physics · Physics 2009-11-11 J. Fuchs , G. J. Duffy , W. J. Rowlands , A. M. Akulshin

The presence of electron energy loss (EELS) peak is proposed theoretically in molybdenum disulfide (MoS2) nanosheets. Using density functional theory simulations and calculations, one EELS peak is identified in the visible energy range, for…

We investigated the two-dimensional electron momentum distributions of atomic negative ions in an intense laser field by solving the time-dependent Schrodinger equation (TDSE) and using the first- and 2nd-order strong-field approximations…

Atomic Physics · Physics 2009-11-13 XiaoXin Zhou , Zhangjin Chen , Toru Morishita , Anh-Thu Le , C. D. Lin

State-specific complete active space self-consistent field (SS-CASSCF) theory has emerged as a promising route to accurately predict electronically excited energy surfaces away from molecular equilibria. However, its accuracy and…

Chemical Physics · Physics 2024-02-21 Sandra Saade , Hugh G. A. Burton

The electronic properties of two-dimensional (2D) materials depend sensitively on the underlying atomic arrangement down to the monolayer level. Here we present a novel strategy for the determination of the band gap and complex dielectric…

Understanding the optical properties of color centers in silicon carbide is essential for their use in quantum technologies, such as single-photon emission and spin-based qubits. In this work, first-principles calculations were employed…

How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various…

Chemical Physics · Physics 2022-01-05 JunWoo Kim , Jonggu Jeon , Tai Hyun Yoon , Minhaeng Cho

We observe ultralong-range blue-shifted Cs$_{2}$ molecular states near $ns_{1/2}$ Rydberg states in an optical dipole trap, where $31\leq n\leq34$. The accidental near degeneracy of $(n-4)l$ and $ns$ Rydberg states for $l>2$ in Cs, due to…

Atomic Physics · Physics 2015-06-05 J. Tallant , S. T. Rittenhouse , D. Booth , H. R. Sadeghpour , J. P. Shaffer

A novel method for fast information retrieval from a probe storage device is considered. It is shown that information can be stored and retrieved using the optical diffraction patterns obtained by the illumination of a large array of…

Information Theory · Computer Science 2015-05-27 Joost van Honschoten , Henri de Jong , Wabe W. Koelmans , Thomas P. Parnell , Oleg V. Zaboronski

Strong resonant elastic light scattering (RELS) from the donor-bound exciton transition in GaAs (1.514eV) occurs at neutral donors in the ground (1S) state, but not at neutral donors in excited hydrogenic states. When 1.6 THz radiation is…

Quantum Physics · Physics 2007-05-23 D. G. Allen , C. R. Stanley , M. S. Sherwin

Among the many potential applications of topological insulator materials, their broad potential for the development of novel tunable plasmonics at THz and mid-infrared frequencies for quantum computing, terahertz detectors, and spintronic…

Mesoscale and Nanoscale Physics · Physics 2023-05-09 Helena La , Abel Brokkelkamp , Stijn van der Lippe , Jaco ter Hoeve , Juan Rojo , Sonia Conesa-Boj

We demonstrate the DC-Kerr effect in PECVD Silicon-rich Nitride (SRN) and use it to demonstrate a third order nonlinear susceptibility, \c{hi}^((3)), as high as (6 +/- 0.58)x10-19 m2/v2. We employ spectral shift versus applied voltage…

Optics · Physics 2021-09-08 Alex Friedman , Hani Nejadriahi , Rajat Sharma , Yeshaiahu Fainman

In atomically thin semiconductors based on transition metal dichalcogenides, photoexcitation can be used to generate high densities of electron-hole pairs. Due to optical nonlinearities, which originate from Pauli blocking and many-body…

Mesoscale and Nanoscale Physics · Physics 2020-12-15 Daniel Erben , Alexander Steinhoff , Michael Lorke , Frank Jahnke

Observation of internal quantum dynamics relies on correlations between the system being observed and the measurement apparatus. We propose using the center-of-mass (c.m.) degrees of freedom of atoms and molecules as a "built-in" monitoring…

Atomic Physics · Physics 2020-07-01 A. W. Bray , U. Eichmann , S. Patchkovskii

We use time-resolved momentum microscopy at a free-electron laser (FEL) and extend orbital tomography into the time domain to image the electronic wave functions of excited molecular orbitals. This technique provides unprecedented insight…

High degrees of intensity correlation between two independent lasers were observed after propagation through a rubidium vapor cell in which they generate Electromagnetically Induced Transparency (EIT). As the optical field intensities are…

Quantum Physics · Physics 2016-08-14 L. S. Cruz , D. Felinto , J. G. Aguirre Gómez , M. Martinelli , P. Valente , A. Lezama , P. Nussenzveig

Laser excitation has emerged as an effective tool for probing microscopic interactions and manipulating phases of matter. Among charge density wave (CDW) materials, 1T-TaS2 has garnered significant attention due to its diverse stacking…

Materials Science · Physics 2025-02-26 Jin Zhang , Yang Yang , Jia Zhang , Mengxue Guan , Jiyu Xu , Kun Yang , Xinghua Shi , Sheng Meng

Coherent diffraction imaging (CDI) allows the retrieval of the structure of an isolated object, such as a macromolecule, from its diffraction pattern. CDI requires the fulfilment of two conditions: the imaging radiation must be coherent and…

Optics · Physics 2018-11-16 Tatiana Latychevskaia , Hans-Werner Fink

Ultra-thin two-dimensional (2D) materials have gained significant attention for making next-generation optoelectronic devices. Here, we report a large-area heterojunction photodetector fabricated using a liquid metal-printed 2D…