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We present a spin-free, size-extensive, and size-consistent coupled cluster method based on a generalised normal ordered exponential ansatz. This approach is a natural generalisation of single-reference coupled cluster theory for arbitrary…

Chemical Physics · Physics 2025-07-21 Nicholas Lee , David P. Tew

A general-order open-shell coupled-cluster method based on spatial orbitals is formulated. The method is an extension of the partial-spin adaptation (PSA) scheme from Janssen and Schaefer (Theor. Chim. Acta, 79, 1-42, 1991). By increasing…

Chemical Physics · Physics 2024-03-18 Cong Wang

In this paper, we report on a correctly scaling novel coupled cluster singles and doubles (CCSD) implementation for arbitrary high-spin open-shell states. The chosen cluster operator is completely spin-free, i.e. employs spatial…

Chemical Physics · Physics 2022-02-23 Nils Herrmann , Michael Hanrath

We present a new high-order coupled cluster method (CCM) formalism for the ground states of lattice quantum spin systems for general spin quantum number, $s$. This new ``general-$s$'' formalism is found to be highly suitable for a…

Strongly Correlated Electrons · Physics 2010-05-07 D. J. J. Farnell , R. F. Bishop , K. A. Gernoth

A general method is described for finding algebraic expressions for matrix elements of any one- and two-particle operator for an arbitrary number of subshells in an atomic configuration, requiring neither coefficients of fractional…

Atomic Physics · Physics 2009-11-10 G. Gaigalas , Z. Rudzikas , C. Froese Fischer

We report a spin-free formulation of the multireference (MR) driven similarity renormalization group (DSRG) by employing the ensemble normal ordering of Mukherjee and Kutzelnigg [W. Kutzelnigg and D. Mukherjee, J. Chem. Phys. 107, 432…

Chemical Physics · Physics 2021-10-04 Chenyang Li , Francesco A. Evangelista

We present a near-linear scaling formulation of the explicitly-correlated coupled-cluster singles and doubles with perturbative triples method (CCSD(T)$_{\overline{\text{F12}}}$) for high-spin states of open-shell species. The approach is…

Chemical Physics · Physics 2024-07-30 Ashutosh Kumar , Frank Neese , Edward F. Valeev

We extend our assessment of the potential of perturbative coupled cluster (CC) expansions for a test set of open-shell atoms and organic radicals to the description of quadruple excitations. Namely, the second- through sixth-order models of…

Chemical Physics · Physics 2016-05-17 Janus J. Eriksen , Devin A. Matthews , Poul Jørgensen , Jürgen Gauss

This is a continuation of the previous work (arXiv:2403.10128). Additional aspects such as linear combinations of projections and hash-table canonicalizations are described. Implementations of the general-order partial-spin adaptation (PSA)…

Chemical Physics · Physics 2025-01-02 Cong Wang

In this paper, we present a method for calculation of spin groups elements for known pseudo-orthogonal group elements with respect to the corresponding two-sheeted coverings. We present our results using the Clifford algebra formalism in…

Mathematical Physics · Physics 2025-04-29 D. S. Shirokov

We show that the Tensor Renormalization Group (TRG) method can be applied to O(N) spin models, principal chiral models and pure gauge theories (Z2, U(1) and SU(2)) on (hyper) cubic lattices. We explain that contrarily to some common belief,…

High Energy Physics - Lattice · Physics 2014-12-02 Yannick Meurice , Alan Denbleyker , Yuzhi Liu , Tao Xiang , Zhiyuan Xie , Ji-Feng Yu , Judah Unmuth-Yockey , Haiyuan Zou

Properly spin-adapted coupled-cluster theory for general open-shell configurations remains an active area of research in electronic structure theory. In this contribution we examine Lindgren's normal-ordered exponential ansatz to correlate…

Chemical Physics · Physics 2024-10-02 Alexander Gunasekera , Nicholas Lee , David P. Tew

In topological quantum computation the geometric details of a particle trajectory are irrelevant; only the topology matters. Taking this one step further, we consider a model of computation that disregards even the topology of the particle…

Quantum Physics · Physics 2011-06-03 Stephen P. Jordan

Exact diagonalization and other numerical studies of quantum spin systems are notoriously limited by the exponential growth of the Hilbert space dimension with system size. A common and well-known practice to reduce this increasing…

Strongly Correlated Electrons · Physics 2019-04-10 T. Heitmann , J. Schnack

We apply the microscopic coupled-cluster method (CCM) to the spin-$1\over2$ $XXZ$ models on both the one-dimensional chain and the two-dimensional square lattice. Based on a systematic approximation scheme of the CCM developed by us…

Condensed Matter · Physics 2017-08-24 R. F. Bishop , R. G. Hale , Y. Xian

We develop the BRST approach for all massless integer and half-integer higher spins in 4D Minkowski space, using the two component spinor nota- tion and develop the Lagrangian formulation for supersymmetric higher spin models. It is shown…

High Energy Physics - Theory · Physics 2016-01-27 I. L. Buchbinder , K. Koutrolikos

We introduce perturbation and coupled-cluster theories based on a cluster mean-field reference for describing the ground state of strongly-correlated spin systems. In cluster mean-field, the ground state wavefunction is written as a simple…

We describe how Computational Group Theory provides tools for manipulating tensors in explicit index notation. In special, we present an algorithm that puts tensors with free indices obeying permutation symmetries into the canonical form.…

Mathematical Physics · Physics 2007-05-23 R. Portugal , B. F. Svaiter

We present a tensor-network approach for two-dimensional strong-coupling QCD with staggered quarks at nonzero chemical potential. After integrating out the gauge fields at infinite coupling, the partition function can be written as a full…

High Energy Physics - Lattice · Physics 2022-12-28 Jacques Bloch , Robert Lohmayer

We focus here on a class of fourth-order parabolic equations that can be written as a system of second-order equations by introducing an auxiliary variable. We design a novel second-order fully discrete mixed finite element method to…

Numerical Analysis · Mathematics 2020-08-28 Sana Keita , Abdelaziz Beljadid , Yves Bourgault
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