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The mutual angle formed by the non-collinear polarization axes of two laser pulses is used to control two-photon XUV+IR ionization of noble gas atoms in the process of reconstruction of attosecond bursts by beating of two-photon transitions…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Zhongtao Xu

We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…

Atomic Physics · Physics 2016-06-29 Vladislav V. Serov , A. S. Kheifets

Reconstruction of Attosecond Beating By Interference of Two-photon Transitions (RABBITT) is a technique that can be used to determine the phases of atomic transition elements in photoionization processes. In the traditional RABBITT scheme,…

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) reveals the target atom electronic structure when one of the transitions proceeds from below the ionization threshold. Such an…

Atomic Physics · Physics 2021-09-14 Anatoli Kheifets

One of the most ubiquitous techniques within attosecond science is the so-called Reconstruction of Attosecond Bursts by Interference of Two-Photon Transitions (RABBITT). Originally proposed for the characterization of attosecond pulses, it…

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets

We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal…

Atomic Physics · Physics 2018-08-01 Shunsuke A. Sato , Hannes Hübener , Angel Rubio , Umberto De Giovannini

We employ Reconstruction of Attosecond Beating By Interference of Two-photon Transitions with an advanced energy resolution (rainbow RABBITT) to resolve under-threshold discrete excitations and above-threshold auto-ionizing states in the He…

Atomic Physics · Physics 2025-02-14 Vladislav Serov , Anatoli Kheifets

Angle-resolved (AR) RABBIT measurements offer a high information content measurement scheme, due to the presence of multiple, interfering, ionization channels combined with a phase-sensitive observable in the form of angle and time-resolved…

Quantum Physics · Physics 2017-09-05 Paul Hockett

Attosecond measurements reveal new physical insights in photo ionization dynamics from atoms, molecules and condensed matter. However, on such time scales even small timing jitter can significantly reduce the time resolution in pump-probe…

Optics · Physics 2020-05-20 Constantin Krüger , Jaco Fuchs , Laura Cattaneo , Ursula Keller

We introduce circular under-threshold RABBITT (cuRABBITT) as a new interferometric method to probe discrete electronic excitations in atoms with attosecond resolution. By combining circularly polarized attosecond pulses with broadband…

We explore how the spectral phase of atto\-second pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an…

Atomic Physics · Physics 2025-06-12 J. Jakob , C. Bauer , M. -J. Ilhan , D. Bharti , C. Ott , T. Pfeifer , K. Bartschat , A. Harth

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) can become resonant with a discrete atomic level either in the intermediate or the final continuous states. Experimental observations of…

Atomic Physics · Physics 2021-09-01 Anatoli S. Kheifets

Reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) is a powerful photoelectron spectroscopy, offering direct access to internal dynamics of the target. It is being increasingly applied to molecular…

Chemical Physics · Physics 2023-04-10 Serguei Patchkovskii , Jakub Benda , Dominik Ertel , David Busto

A relativistic transient absorption theory is derived, implemented and validated within the dipole approximation based on the time-dependent Dirac equation. Time-dependent simulations have been performed using the Dirac equation and the…

Atomic Physics · Physics 2020-10-14 Felipe Zapata , Jimmy Vinbladh , Eva Lindroth , Jan Marcus Dahlström

We report on the simulation results for the angular resolution of an electromagnetic (EM) sampling calorimeter with photons in the range of 100~MeV to 2~GeV. The simulation model of the EM calorimeter consists of alternating layers of a…

Instrumentation and Detectors · Physics 2023-04-26 Junlee Kim , Eun-Joo Kim , YoungJun Kim , JungKeun Ahn , GeiYoub Lim

We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of…

Atomic Physics · Physics 2016-03-02 Álvaro Jiménez Galán , Fernando Martín , Luca Argenti

The RABBITT setup is theoretically studied for various combinations of XUV and IR field components polarization: 'linear+linear', `linear+circular' with crossed propagation directions, and `circular+circular' with parallel propagation…

Atomic Physics · Physics 2024-10-29 Maria M. Popova , Sergei N. Yudin , Alexei N. Grum-Grzhimailo , Elena V. Gryzlova
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