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We performed Raman spectroscopy measurements under temperature changes from 10 K up to 850 K to probe the phonon-spin coupling in Y$_2$NiMnO$_6$. The spin-phonon coupling was observed as a softening of the stretching mode, indicating this…

Spin-phonon coupling effects, as reflected in phonon frequency shifts between ferromagnetic (FM) and G-type antiferromagnetic (AFM) configurations in cubic CaMnO$_3$, SrMnO$_3$, BaMnO$_3$, LaCrO$_3$, LaFeO$_3$ and La$_2$(CrFe)O$_6$, are…

Strongly Correlated Electrons · Physics 2012-11-20 Jiawang Hong , Alessandro Stroppa , Jorge Íñiguez , Silvia Picozzi , David Vanderbilt

Low-dimensional frustrated magnetic square networks feature a variety of unconventional phases with novel emergent excitations. Often these excitations are intertwined and manifest into intriguing phenomena, an area that has remained…

Materials Science · Physics 2024-01-10 Shalini Badola , Aprajita Joshi , Akriti Singh , Surajit Saha

The temperature dependence of phonon excitations and the presence of spin phonon coupling in polycrystalline Pr2NiMnO6 samples were studied using micro-Raman spectroscopy and magnetometry. Magnetic properties show a single…

Materials Science · Physics 2011-01-17 K. D. Truong , M. P. Singh , S. Jandl , P. Fournier

In this paper we investigated the influence of the rare-earth ionic radii on the spin-phonon coupling in RE2NiMnO6 double perovskites by Raman spectroscopy. Spin-phonon in dense Nd2NiMnO6 and Gd2NiMnO6 ceramics were investigated by Raman…

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

The structural, electronic and magnetic properties of anti-site disordered Sm$ _{2} $NiMnO$ _{6} $ double perovskite has been studied. RE$_{2}$NiMnO$_{6}$ (RE: rare-earth) ordered double perovskite is commonly believed to show two distinct…

Materials Science · Physics 2025-07-28 S. Majumder , M. Tripathi , P. Rajput , S. N. Jha , R. J. Choudhary , D. M. Phase

Electronic structure near Fermi level of Pr2CoFeO6 (at 300 K) was investigated by X-ray photoemission spectroscopy (XPS) technique. All three cations, i.e., Pr, Co and Fe were found to be trivalent in nature. XPS analysis also suggested the…

Strongly Correlated Electrons · Physics 2019-05-22 Arkadeb Pal , Surajit Ghosh , Amish G. Joshi , P. K. Gupta , P. Prakash , Amitabh Das , A. K. Ghosh , Sandip Chatterjee

In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman and dielectric spectroscopic study. Pr$_2$CoMnO$_6$ is a manganite compound , it undergoes a paramagnetic to…

Strongly Correlated Electrons · Physics 2021-04-13 Ilyas Noor Bhatti , Imtiaz Noor Bhatti

We present Raman spectroscopy results backed by first-principles calculations and investigate the nature of possible spin-phonon coupling (SPC) in a Gd-doped Y$_2$CoMnO$_6$ (YGCMO) double perovskite oxide. The influence of Gd substitution,…

Materials Science · Physics 2025-08-20 Anasua Khan , Debdatta Banerjee , Divya Rawat , T. K Nath , Ajay Soni , Swastika Chatterjee , A. Taraphder

Using first-principles density functional calculations, we study the electronic and magnetic properties of ferromagnetic insulating double-perovskite compound La2NiMnO6, which has been reported to exhibit interesting magnetic field…

Materials Science · Physics 2008-05-09 Hena Das , Umesh V. Waghmare , T. Saha-Dasgupta , D. D. Sarma

We report the detection of paramagnetic resonance in the double perovskite La2NiMnO6 at room temperature for microwave magnetic fields with frequencies, f = 1 GHz to 5 GHz, using two cavity-less methods. We use an indirect impedance method…

Materials Science · Physics 2020-10-28 Ushnish Chaudhuri , Debendra Prasad Panda , A. Sundaresan , R. Mahendiran

Using Raman spectroscopy, we investigate the lattice phonons, magnetic excitations, and magneto-elastic coupling in the distorted triangular-lattice Heisenberg antiferromagnet alpha-SrCr2O4, which develops helical magnetic order below 43 K.…

Sr$_{2}$NiIrO$_{6}$ would be a ferromagnetic (FM) insulator in terms of the common superexchange mechanism between the first nearest neighboring (1NN) magnetic ions Ni$^{2+}$ ($t_{2g}^{6}e_{g}^{2}$) and Ir$^{6+}$ ($t_{2g}^{3}$). However,…

Strongly Correlated Electrons · Physics 2014-12-23 Xuedong Ou , Zhengwei Li , Fengren Fan , Hongbo Wang , Hua Wu

We report structural, magnetic, and Raman studies of the disordered double perovskite GdSrCoMnO$_{6}$~(GSCM). DC magnetization shows a ferromagnetic transition at $T_{C} \approx 153$~K. The inverse susceptibility exhibits a downturn above…

We report the structural, magnetic and thermodynamic properties of the double perovskite compound La2CuIrO6 from X-ray, neutron diffraction, neutron depolarization, dc magnetization, ac susceptibility, specific heat, muon-spin-relaxation…

Multifunctional properties in quantum systems require the interaction between different degrees of freedom. As such, spin-phonon coupling emerges as an ideal mechanism to tune multiferroicity, magnetism, and magnetoelectric response. In…

The strong exchange interaction between 3$d$-4$f$ magnetic sublattice in rare-earth perovskites introduces a variety of complex magnetic states hosting fascinating electronic ground states with exotic properties. Especially when it comes to…

The observation of strongly coupled lattice and spin dynamics in altermagnet CoF$_2$ is reported. On the background of the expected spin-phonon interaction leading to renormalization of all phonons at the Neel temperature an additional…

Materials Science · Physics 2024-05-14 M. A. Prosnikov , M. Bal , R. V. Pisarev , P. C. M. Christianen , A. M. Kalashnikova

The quadruple Calcium manganite (CaMn7O12) is a multiferroic material that exhibits a giant magnetically-induced ferroelectric polarization which makes it very interesting for magnetoelectric applications. Here, we report the Raman…

Strongly Correlated Electrons · Physics 2019-01-16 C. Toulouse , C. Martin , M-A. Measson , Y. Gallais , A. Sacuto , M. Cazayous
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