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Antiferromagnetic materials with strong spin-phonon coupling have the potential for spintronic applications. Here, we report the structural, magnetic, and vibrational properties of 12R-BaTi0.4Mn0.6O3. Temperature-dependent magnetization…

Materials Science · Physics 2021-10-27 Bommareddy Poojitha , Anjali Rathore , Surajit Saha

We investigate the structural, magnetic and spin-state transitions, and magnetocaloric properties of Sr$_{2-x}$La$_x$CoNbO$_6$ ($x=$ 0--1) double perovskites. The structural transition from tetragonal to monoclinic phase at $x$ $\geqslant$…

Materials Science · Physics 2020-04-21 Ajay Kumar , R. S. Dhaka

The magnetism of the double perovskite compounds \SLFCOx\ ($x$ = 0, 1, 2) are contrasted using magnetization, neutron diffraction and electron paramagnetic resonance with the support from density functional theory calculations. \LFCO\ is…

Antiferromagnetic antiperovskites, of the form Mn$_3B$N ($B$ = Ni, Cu, Zn, Sn, Ir, and Pt), have shown an outstanding behavior in which, giant negative thermal expansion and chiral magnetic structures are intertwined. As such, aiming to…

Materials Science · Physics 2022-09-07 L. Florez-Gomez , W. Ibarra-Hernandez , A. C. Garcia-Castro

We performed a Raman scattering study of thin films of LiTi$_2$O$_4$ spinel oxide superconductor. We detected four out of five Raman active modes, with frequencies in good accordance with our first-principles calculations. Three T$_{2g}$…

Superconductivity · Physics 2017-09-13 D. Chen , Y. -L. Jia , T. -T. Zhang , Z. Fang , K. Jin , P. Richard , H. Ding

The interplay of the electron-phonon interaction and of the double and super exchange magnetic effects is analyzed in the $La_{1-x}Ca_xMnO_3$ perovskites with $0<x<0.5$. By using an analytical variational scheme that allows to treat the…

Strongly Correlated Electrons · Physics 2009-10-31 V. Cataudella , G. De Filippis , G. Iadonisi

We study experimentally and theoretically the electronic and magnetic properties of two insulating double perovskites that show similar atomic and electronic structure, but different magnetic properties. In magnetization measurements,…

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

Strongly Correlated Electrons · Physics 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

We present a fully analytical model of hybridization between magnon, and phonons observed experimentally in magneto-Raman scattering in van der Waals (vdW) antiferromagnets (AFM). Here, the representative material, FePS3, has been shown to…

Mesoscale and Nanoscale Physics · Physics 2025-01-03 Somsubhra Ghosh , Mainak Palit , Sujan Maity , Subhadeep Datta

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

We present results based on local spin density calculations of a computational search for half-metallic (HM) antiferromagnetic (AFM) materials within the class of double perovskite structure oxides LaM'M''O3 that incorporate open shell 3d…

Materials Science · Physics 2009-10-30 Warren E. Pickett

Sr$_{2}$FeMoO$_6$ is a double perovskite compound, known for its high temperature behavior. Combining different magnetic and spectroscopic tools, we show that this compound can be driven to rare example of antiferromagnetic metallic state…

We present optical measurements of phononic excitations in La$_{2/3}$Ca$_{1/3}$MnO$_{3}$ (LCMO) and La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ (LSMO) thin films covering the full temperature range from the metallic ferromagnetic to the insulating…

Strongly Correlated Electrons · Physics 2010-05-24 Ch. Hartinger , F. Mayr , A. Loidl , T. Kopp

Based on the theoretical exploration of electronic structures, we propose that the ordered double perovskites LaAVRuO$_6$ and LaVO$_3$/ARuO$_3$ (001) superlattice (A = Ca, Sr and Ba) are strong candidates for half-metallic (HM)…

Strongly Correlated Electrons · Physics 2016-08-31 J. H. Park , S. K. Kwon , B. I. Min

We report detailed Raman spectroscopic and magnetic susceptibility studies on the spin-driven ferroelectric compounds Mn4Nb2O9 (MNO) and Mn4Ta2O9 (MTO). Both systems exhibit strong spin-phonon coupling below the short-range magnetic…

Materials Science · Physics 2026-02-09 Rajesh Jana , Alka Garg , Rekha Rao , Thomas Meier

Using density-functional theory calculations, we investigated the electronic structure and magnetic exchange interactions of the ordered 3d-5d double perovskite Sr2FeOsO6, which has recently drawn attention for interesting antiferromagnetic…

Materials Science · Physics 2014-07-24 Sudipta Kanungo , Binghai Yan , Martin Jansen , Claudia Felser

We explore the role of interfacial antiferromagnetic interaction in coupled soft and hard ferromagnetic layers to ascribe the complex variety of magneto-transport phenomena observed in $La_{0.7}Sr_{0.3}MnO_3/SrRuO_3$ (LSMO/SRO)…

Strongly Correlated Electrons · Physics 2023-06-28 Sandip Halder , Subrat K. Das , Kalpataru Pradhan

We report on the structural evolution, spin phonon interactions, and magnetoelastic effects in bulk LaFeO3 perovskite across its antiferromagnetic transition. We found that while the lattice constants exhibit slight deviations at the Neel…

The Griffiths phase-like features and the spin-phonon coupling effects observed in Tb$_2$NiMnO$_6$ are reported. The double perovskite compound crystallizes in monoclinic $P2_1/n$ space group and exhibits a magnetic phase transition at $T_c…

Strongly Correlated Electrons · Physics 2015-06-03 Harikrishnan S. Nair , Diptikanta Swain , Hariharan N. , Shilpa Adiga , Chandrabhas Narayana , Suja Elizabeth

We investigate the antiferromagnetic insulating state of the recently discovered double perovskites Sr$_2$XOsO$_6$ (X$=$Sc, Mg) by using ab-initio calculations (based on Density Functional Theory and Dynamical Mean-Field Theory) to…

Strongly Correlated Electrons · Physics 2016-11-22 Gianluca Giovannetti