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Cooperative effects allow for fascinating characteristics in light-matter interacting systems. Here, we study naturally occurring superradiant coupling in a class of quasi-two-dimensional, layered semiconductor systems. We perform optical…

Mesoscale and Nanoscale Physics · Physics 2018-06-08 C. E. Stevens , T. Stroucken , A. V. Stier , J. Paul , H. Zhang , P. Dey , S. A. Crooker , S. W. Koch , D. Karaiskaj

Localized interlayer excitons (LIXs) in two-dimensional moir\'e superlattices exhibit sharp and dense emission peaks, making them promising as highly tunable single-photon sources. However, the fundamental nature of these LIXs is still…

In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of the Coulomb interaction leads to strongly correlated many-body states, including excitons and trions, that dominate the optical properties.…

$\require{mediawiki-texvc}$ We demonstrate that the low symmetry of armchair lateral heterojunction between transition metal dichalcogenide monolayers allows for the mixing of $\mathbf{K}_+$ and $\mathbf{K}_-$ valleys. From the tight…

Mesoscale and Nanoscale Physics · Physics 2024-08-20 M. V. Durnev , D. S. Smirnov

Monolayer transition-metal dichalcogenide (TMD) semiconductors exhibit strong excitonic effects and hold promise for optical and optoelectronic applications. Yet, electron doping of TMDs leads to the conversion of neutral excitons into…

Interlayer excitons are observed coexisting with intralayer excitons in bi-layer, few-layer, and bulk MoSe2 single crystals by confocal reflection contrast spectroscopy. Quantitative analysis using the Dirac-Bloch-Equations provides…

Materials Science · Physics 2018-06-13 Jason Horng , Tineke Stroucken , Long Zhang , Eunice Y. Paik , Hui Deng , Stephan W. Koch

Lattice reconstruction in twisted transition-metal dichalcogenide (TMD) bilayers gives rise to piezo- and ferroelectric moir\'e potentials for electrons and holes, as well as a modulation of the hybridisation across the bilayer. Here, we…

Mesoscale and Nanoscale Physics · Physics 2021-09-30 S. J. Magorrian , V. V. Enaldiev , V. Zólyomi , Fábio Ferreira , Vladimir I. Fal'ko , David A. Ruiz-Tijerina

We reveal by first-principles calculations that the interlayer binding in a twisted MoS2/MoTe2 heterobilayer decreases with increasing twist angle, due to the increase of the interlayer overlapping degree, a geometric quantity describing…

Materials Science · Physics 2020-10-07 W. T. Geng , V. Wang , J. B. Lin , T. Ohno , J. Nara

Strongly bound excitons confined in two-dimensional (2D) semiconductors are dipoles with a perfect in-plane orientation. In a vertical stack of semiconducting 2D crystals, such in-plane excitonic dipoles are expected to efficiently couple…

We study the refraction effect of electronic wave in hole-doped lateral heterojunctions of metallic and semiconducting transition-metal dichalcogenide monolayers. This effect is theoretically investigated in 2$H$-type MoSe$_2$-NbS$_2$ and…

Mesoscale and Nanoscale Physics · Physics 2019-10-01 Tetsuro Habe

Moir\'e lattices created in two-dimensional heterostructures exhibit rich many-body physics of interacting electrons and excitons and, at the same time, suggest promising optoelectronic applications. Here, we study the cooperative radiance…

Quantum Physics · Physics 2025-05-14 Jan Kumlin , Ajit Srivastava , Thomas Pohl

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 Roland Gillen , Janina Maultzsch

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

Nearly localized moire flat bands in momentum space, arising at particular twist angles, are the key to achieve correlated effects in transition-metal dichalcogenides. Here, we use angle-resolved photoemission spectroscopy (ARPES) to…

The photoluminescence (PL) spectrum of transition metal dichalcogenides (TMDs) shows a multitude of emission peaks below the bright exciton line and not all of them have been explained yet. Here, we study the emission traces of…

Disorder derived from defects or strain in monolayer TMDs can lead to a dramatic change in the physical behavior of the interband excitations, producing inhomogeneous spectral broadening and localization; leading to radiative lifetime…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Sabrine Ayari , Adlen Smiri , Aida Hichri , Sihem Jaziri , Thierry Amand

The possibility of the formation of an electron-hole liquid in the type II heterostructures based on monolayers (bilayers) of transition metal dichalcogenides is considered. It is indicated that additional valleys in the conduction band,…

Mesoscale and Nanoscale Physics · Physics 2022-06-22 Pavel V. Ratnikov

Heterostructures (HSs) formed by the transition-metal dichalcogenides (TMDCs) materials have shown great promise in next-generation optoelectronic and photonic applications. An artificially twisted HS, allows us to manipulate the optical,…

This work presents a first-principles study of the optoelectronic properties of vertically-stacked bilayer heterostructures composed of 2D transition-metal dichalcogenides (TMDs). The calculations are performed using the density-functional…

Materials Science · Physics 2025-01-15 Khushboo Dange , Rachana Yogi , Alok Shukla

WSe$_2$ monolayers with variable doping are an ideal system to study two-dimensional excitonic complexes. Here, we find that the strongest photoluminescence from bright neutral excitons occurs at moderate $p$-doping levels, owing to a rapid…

Mesoscale and Nanoscale Physics · Physics 2020-05-07 Sven Borghardt , Jhih-Sian Tu , Takashi Taniguchi , Kenji Watanabe , Beata E. Kardynal