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We systemically investigate the nature of Ce 4f electrons in structurally layered heavy-fermion compounds CcmMnIn3m+2n (with M =Co, Rh, Ir, and Pt, m=l, 2, n=0 - 2), at low temperature using on-resonance angle-resolved photoemission…

We show that crystal-field calculations for $C_1$ point-group symmetry are possible, and that such calculations can be performed with sufficient accuracy to have substantial utility for rare-earth based quantum information applications. In…

Contrary to the well known spin qubits, rare-earth qubits are characterized by a strong influence of crystal field due to large spin-orbit coupling. At low temperature and in the presence of resonance microwaves, it is the magnetic moment…

Strongly Correlated Electrons · Physics 2009-11-26 Sylvain Bertaina , J. H. Shim , S. Gambarelli , B. Z. Malkin , B. Barbara

CeRh$_2$As$_2$ is a new multiphase superconductor with strong suggestions for an additional itinerant multipolar ordered phase. The modeling of the low temperature properties of this heavy fermion compound requires a quartet Ce$^{3+}$…

We use high resolution angle-resolved photoemission spectroscopy (ARPES) and electronic structure calculations to study the electronic properties of rare-earth monoantimonides RSb (R = Y, Ce, Gd, Dy, Ho, Tm, Lu). The experimentally measured…

Materials Science · Physics 2017-07-20 Yun Wu , Yongbin Lee , Tai Kong , Daixiang Mou , Rui Jiang , Lunan Huang , S. L. Bud'ko , P. C. Canfield , Adam Kaminski

In this article we present high-resolution angle-resolved photoemission (ARPES) spectra of the heavy-fermion superconductor URu$_2$Si$_2$. Measurements as a function of both excitation energy and temperature allow us to disentangle a…

The delafossite family of compounds with a triangular lattice of rare earth ions has been recently proposed as a candidate host for quantum spin liquid (QSL) states. To realize QSLs, the crystal-electric-field (CEF) ground state of the rare…

Strongly Correlated Electrons · Physics 2020-07-20 Shang Gao , Fan Xiao , Kazuya Kamazawa , Kazuhiko Ikeuchi , Daniel Biner , Karl Krämer , Christian Rüegg , Taka-hisa Arima

It is a long-standing important issue in heavy fermion physics whether $f$-electrons are itinerant or localized when the magnetic order occurs. Here we report the {\it in situ} scanning tunneling microscopy observation of the electronic…

Rare-earth (RE) based compounds and alloys are of great interest both for their fundamental physical properties and for applications. In order to tailor the required compounds for a specific task, one must be able to predict the energy…

Condensed Matter · Physics 2007-05-23 Nicola Magnani

Crystal-field (CF) effects on the rare-earth (RE) ions in ferrimagnetic intermetallics NdCo$_5$ and TbCo$_5$ are evaluated using an ab initio density functional + dynamical mean-field theory approach in conjunction with a quasi-atomic…

Materials Science · Physics 2020-06-23 L. V. Pourovskii , J. Boust , R. Ballou , G. Gomez Eslava , D. Givord

Electronic structures of a charge-density-wave CDW system CeTe_2-xSb_x (x=0, 0.05) have been investigated by employing angle-resolved photoemission spectroscopy (ARPES). The observed Fermi surface (FS) agrees very well with the calculated…

Strongly Correlated Electrons · Physics 2011-09-05 J. -S. Kang , D. H. Kim , H. J. Lee , J. H. Hwang , Han-Koo Lee , H. -D. Kim , B. H. Min , K. E. Lee , Y. S. Kwon , J. W. Kim , Kyoo Kim , B. H. Kim , B. I. Min

We address the fundamental question of crossover from localized to itinerant state of a paradigmatic heavy fermionmaterial CeIrIn5. The temperature evolution of the one electron spectra and the optical conductivity is predicted from first…

Strongly Correlated Electrons · Physics 2009-11-13 J. H. Shim , K. Haule , G. Kotliar

We use angle-resolved photoemission spectroscopy (ARPES) to image the emergence of substaintial dispersion anomalies in the electronic renormalization of the actinide compound UCoGa$_5$ which was presumed to belong to a conventional Fermi…

Strongly Correlated Electrons · Physics 2013-01-30 Tanmoy Das , Tomasz Durakiewicz , Jian-Xin Zhu , John J. Joyce , John L. Sarrao , Matthias J. Graf

We report on the results of a high-resolution angle-resolved photoemission (ARPES) study on the ordered surface alloy CePt5. The temperature dependence of the spectra show the formation of the coherent low-energy heavy-fermion band near the…

Strongly Correlated Electrons · Physics 2015-05-27 M. Klein , A. Nuber , H. Schwab , N. Tobita , M. Higashiguchi , J. Jiang , S. Fukuda , K. Tanaka , K. Shimada , M. Mulazzi , F. F. Assaad , F. Reinert

The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

Strongly Correlated Electrons · Physics 2009-11-11 Annamaria Kiss , Yoshio Kuramoto

We report the ground-state symmetry of the Ce $4f$ states in the heavy fermion superconductor CeNi$_{2}$Ge$_{2}$, yielding anisotropic $cf$-hybridization between the Ce $4f$ states and conducting electrons. By analyzing linear dichroism in…

Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

We present a high-resolution photoemission study on the strongly correlated Ce-compounds CeCu_6, CeCu_2Si_2, CeRu_2Si_2, CeNi_2Ge_2, and CeSi_2. Using a normalization procedure based on a division by the Fermi-Dirac distribution we get…

Strongly Correlated Electrons · Physics 2007-08-03 D. Ehm , S. H"ufner , F. Reinert , J. Kroha , P. W"olfle , O. Stockert , C. Geibel , H. von L"ohneysen

The electronic structure of ThRu2Si2 was studied by angle-resolved photoelectron spectroscopy (ARPES) with incident photon energies of hn=655-745 eV. Detailed band structure and the three-dimensional shapes of Fermi surfaces were derived…

Among numerous hypotheses, recently proposed to explain superconductivity in iron-based superconductors [1-9], many consider Fermi surface (FS) nesting [2, 4, 8, 10] and dimensionality [4, 9] as important contributors. Precise determination…

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