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We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

Dynamic Nuclear Polarization (DNP) is to date the most effective technique to increase the nuclear polarization up to a factor $100,000$ opening disruptive perspectives for medical applications. In DNP, the nuclear spins are driven to an -…

Strongly Correlated Electrons · Physics 2015-08-26 Andrea De Luca , Alberto Rosso

We report on the resonant optical pumping of the |\pm1> spin states of a single Mn dopant in an InAs/GaAs quantum dot embedded itself in a charge tuneable device. The experiment relies on a "W" scheme of transitions reached when a suitable…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Emmanuel Baudin , Emile Benjamin , Aristide Lemaître , Olivier Krebs

We present an experimental study of the Dynamic Nuclear Polarization (DNP) of \si{} nuclei in silicon crystals of natural abundance doped with As in the temperature range 0.1-1 K and in strong magnetic field of 4.6 T. This ensures very high…

Mesoscale and Nanoscale Physics · Physics 2020-06-24 J. Jarvinen , D. Zvezdov , J. Ahokas , S. Sheludyakov , L. Lehtonen , S. Vasiliev , L. Vlasenko , Y. Ishikawa , Y. Fujii

For spin-based quantum computation in semiconductors, dephasing of electron spins by a fluctuating background of nuclear spins is a main obstacle. Here we show that this nuclear background can be precisely controlled in generic quantum dots…

Mesoscale and Nanoscale Physics · Physics 2019-06-19 Sergej Markmann , Christian Reichl , Werner Wegscheider , Gian Salis

We measure the statistical polarization of quadrupolar nuclear spins in a sub-micrometer (0.6 um^3) particle of GaAs using magnetic resonance force microscopy. The crystalline sample is cut out of a GaAs wafer and attached to a…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 Fei Xue , D. P. Weber , P. Peddibhotla , M. Poggio

Coherent two-level systems, or qubits, based on electron spins in GaAs quantum dots are strongly coupled to the nuclear spins of the host lattice via the hyperfine interaction. Realizing nuclear spin control would likely improve electron…

Mesoscale and Nanoscale Physics · Physics 2010-06-15 D. J. Reilly , J. M. Taylor , J. R. Petta , C. M. Marcus , M. P. Hanson , A. C. Gossard

Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving…

Sizable nuclear spin polarization is pumped in individual InP/GaInP dots in a wide range of external magnetic fields B_ext=0-5T by circularly polarized optical excitation. We observe nuclear polarization of up to ~40% at Bext=1.5T and…

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

The role of nuclear spin fluctuations in the dynamic polarization of nuclear spins by electrons is investigated in (In,Ga)As quantum dots. The photoluminescence polarization under circularly polarized optical pumping in transverse magnetic…

Spin-blockaded quantum dots provide a unique setting for studying nuclear-spin dynamics in a nanoscale system. Despite recent experimental progress, observing phase-sensitive phenomena in nuclear spin dynamics remains challenging. Here we…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 M. S. Rudner , I. Neder , L. S. Levitov , B. I. Halperin

In systems with spin-momentum locking, such as the surface states of three-dimensional topological insulators, a charge current is spin-polarized and spin-flip interactions between electron and nuclear spins can transfer this polarization…

Mesoscale and Nanoscale Physics · Physics 2025-06-18 Sofie Kölling , İnanç Adagideli , Alexander Brinkman

We have studied the current through a carbon nanotube quantum dot with one ferromagnetic and one normal-metal lead. For the values of gate voltage at which the normal lead is resonant with the single available non-degenerate energy level on…

Mesoscale and Nanoscale Physics · Physics 2008-08-20 Christopher A. Merchant , Nina Markovic

Conduction electrons are used to optically polarize, detect and manipulate nuclear spin in a (110) GaAs quantum well. Using optical Larmor magnetometry, we find that nuclear spin can be polarized along or against the applied magnetic field,…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 G. Salis , D. T. Fuchs , J. M. Kikkawa , D. D. Awschalom , Y. Ohno , H. Ohno

The periodic optical orientation of electron spins in (In,Ga)As/GaAs quantum dots leads to the formation of electron spin precession modes about an external magnetic field which are resonant with the pumping periodicity. As the electron…

Mesoscale and Nanoscale Physics · Physics 2019-08-15 E. Evers , V. V. Belykh , N. E. Kopteva , I. A. Yugova , A. Greilich , D. R. Yakovlev , D. Reuter , A. D. Wieck , M. Bayer

We report manifestly nonlinear dependence of quantum dot nuclear spin polarization on applied magnetic fields. Resonant absorption and emission of circularly polarized radiation pumps the resident quantum dot electron spin, which in turn…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. Maletinsky , C. W. Lai , A. Badolato , A. Imamoglu

Multielectron semiconductor quantum dots (QDs) provide a novel platform to study the role of Coulomb correlations in finite quantum systems and their impact on many-body energy spectra. An example is the formation of interaction-driven,…

A new method for local dynamic nuclear polarization is demonstrated in a GaAs/AlGaAs heterostructure at the Landau level filling factor $\nu=3$. Using a narrow channel sample, where the width varies stepwise along the electron flow, we find…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yosuke Komori , Tohru Okamoto

We theoretically study the nuclear spin dynamics driven by electron transport and hyperfine interaction in an electrically-defined double quantum dot (DQD) in the Pauli-blockade regime. We derive a master-equation-based framework and show…

Mesoscale and Nanoscale Physics · Physics 2014-06-03 Martin J. A. Schuetz , Eric M. Kessler , Lieven M. K. Vandersypen , J. Ignacio Cirac , Geza Giedke
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