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We report on the dynamic nuclear polarization of a single charge-tunable self-assembled InAs/GaAs quantum dot in a longitudinal magnetic field of $\sim$0.2T. The hyperfine interaction between the optically oriented electron and nuclei spins…

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

We study experimentally the dependence of dynamic nuclear spin polarization on the power of non-resonant optical excitation in two types of individual neutral semiconductor quantum dots: InGaAs/GaAs and GaAs/AlGaAs. We show that the…

Mesoscale and Nanoscale Physics · Physics 2013-07-10 J. Puebla , E. A. Chekhovich , M. Hopkinson , P. Senellart , A. Lemaitre , M. S. Skolnick , A. I. Tartakovskii

We studied the zero-field dynamic nuclear spin polarization in a single In$_{0.75}$Al$_{0.25}$As/Al$_{0.3}$Ga$_{0.7}$As quantum dot. Even without any external magnetic field, the positive trion excited by the circularly-polarized light…

Mesoscale and Nanoscale Physics · Physics 2017-03-20 Ryosuke Matsusaki , Reina Kaji , Sohta Yamamoto , Hirotaka Sasakura , Satoru Adachi

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. R. Petta , J. M. Taylor , A. C. Johnson , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

Optical and electrical control of the nuclear spin system allows enhancing the sensitivity of NMR applications and spin-based information storage and processing. Dynamic nuclear polarization in semiconductors is commonly achieved in the…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Sallen , S. Kunz , T. Amand , L. Bouet , T. Kuroda , T. Mano , D. Paget , O. Krebs , X. Marie , K. Sakoda , B. Urbaszek

The central-spin problem, in which an electron spin interacts with a nuclear spin bath, is a widely studied model of quantum decoherence. Dynamic nuclear polarization (DNP) occurs in central spin systems when electronic angular momentum is…

We propose a new mechanism for polarizing nuclear spins in quantum dots, based on periodic modulation of the hyperfine coupling by electric driving at the electron spin resonance frequency. Dynamical nuclear polarization results from…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 M. S. Rudner , L. S. Levitov

Repeated injection of spin polarized carriers in a quantum dot leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the first observation of p-shell carrier assisted DNP in…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 C. F. Fong , Y. Ota , E. Harbord , S. Iwamoto , Y. Arakawa

We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

Sharp threshold-like transitions between two stable nuclear spin polarizations are observed in optically pumped individual InGaAs self-assembled quantum dots embedded in a Schottky diode when the bias applied to the diode is tuned. The…

A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic…

Mesoscale and Nanoscale Physics · Physics 2010-09-30 F. Klotz , V. Jovanov , J. Kierig , E. C. Clark , M. Bichler , G. Abstreiter , M. S. Brandt , J. J. Finley , H. Schwager , G. Giedke

The spin dynamics of positively (X$^{+}$) and negatively (X$^{-}$) charged excitons in InP/In$_{0.48}$Ga$_{0.52}$P quantum dots subject to a magnetic field is studied. We find that a characteristic feature of the system under study is the…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 S. V. Nekrasov , I. A. Akimov , Yu. G. Kusrayev , D. R. Yakovlev , M. Bayer

We report on the dynamics of optically induced nuclear spin polarization in individual CdTe/ZnTe quantum dots loaded with one electron by modulation doping. The fine structure of the hot trion (charged exciton $X^-$ with an electron in the…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , A. Brunetti , H. Boukari , L. Besombes

Highly polarized nuclear spins within a semiconductor quantum dot (QD) induce effective magnetic (Overhauser) fields of up to several Tesla acting on the electron spin or up to a few hundred mT for the hole spin. Recently this has been…

Mesoscale and Nanoscale Physics · Physics 2011-11-04 M. N. Makhonin , K. V. Kavokin , P. Senellart , A. Lema^itre , A. J. Ramsay , M. S. Skolnick , A. I. Tartakovskii

We present a comprehensive examination of optical pumping of spins in individual GaAs quantum dots as we change the charge from positive to neutral to negative using a Schottky diode. We observe that photoluminescence polarization memory…

Dynamic nuclear polarization (DNP) is an attractive method for initializing nuclear spins that are strongly coupled to optically active electron spins because it functions at room temperature and does not require strong magnetic fields. In…

We theoretically investigate the controlled dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. Three regimes of long-term dynamics are identified, including the build up of a large difference…

Mesoscale and Nanoscale Physics · Physics 2012-11-07 M. Gullans , J. J. Krich , J. M. Taylor , H. Bluhm , B. I. Halperin , C. M. Marcus , M. Stopa , A. Yacoby , M. D. Lukin

We employ optical pump-probe spectroscopy to investigate the voltage dependence of spontaneous electron and nuclear spin polarizations in hybrid MnAs/n-GaAs and Fe/n-GaAs Schottky diodes. Through the hyperfine interaction, nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. J. Epstein , J. Stephens , M. Hanson , Y. Chye , A. C. Gossard , P. M. Petroff , D. D. Awschalom

We report optical orientation experiments in individual, strain free GaAs quantum dots in AlGaAs grown by droplet epitaxy. Circularly polarized optical excitation yields strong circular polarization of the resulting photoluminescence at 4K.…

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