Related papers: Hyperfine interaction with the $^{229}$Th nucleus …
The hyperfine structure of the long-lived $5D_{3/2}$ and $5D_{5/2}$ levels of Ba$^+$ ion is analyzed. A procedure for extracting relatively unexplored nuclear magnetic moments $\Omega$ is presented. The relevant electronic matrix elements…
We explore an unusual nature of chemical bonding of the thorium atom with a ring of six carbon atoms (hexagon) in novel carbon materials. Our ab initio calculations of Th-based metallofullerenes (Th@C60, Th@C20) and Th bound to benzene or…
Motivated by recent experimental advances, including the ongoing development of an optical atomic clock in singly ionised radium, we perform a detailed theoretical characterisation of Ra+ and its lighter analogue, Ba+. Both ions are of…
A new method for obtaining of inverse population between quadrupole sublevels of the ground state $5/2^+(0.0)$ and the isomeric state $3/2^+(7.6$ eV) of the $^{229}$Th nucleus in a dielectric crystal with a large band gap by means of…
The multiconfiguration Dirac-Hartree-Fock method implemented in the Grasp2018 package was employed to calculate the magnetic dipole hyperfine interaction constants and electric field gradients of levels in the ground configuration of the…
Precision measurements of Schiff moments in heavy, deformed nuclei are sensitive probes of beyond Standard Model $T,P$-violation in the hadronic sector. While the most sensitive limits on Schiff moments to date are set with diamagnetic…
The 7.8 eV nuclear isomer transition in 229 Thorium has been suggested as an etalon transition in a new type of optical frequency standard. Here we discuss the construction of a "solid-state nuclear clock" from Thorium nuclei implanted into…
Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…
An experiment to search for the electron electric dipole moment (\eEDM) on the metastable $H^3\Delta_1$ state of ThO molecule was proposed and now in the final stage of preparation by the ACME collaboration [http://www.electronedm.org]. To…
Binding energies of high-L Rydberg states (L^3 7) of Th2+ with n=27-29 were studied using the Resonant Excitation Stark Ionization Spectroscopy (RESIS) method. The core of the Th2+ Rydberg ion is the Fr-like ion Th3+ whose ground state is a…
The 8.4 eV transition in the $^{229}$Th nucleus is the basis for a high-precision nuclear clock with exceptional sensitivity to new physics effects. We have identified several cases in the Th$^+$ ion where electronic excitations closely…
There exist in nature a few nuclear isomers with very low (eV) excitation energies, and the combination of low energy and narrow width makes them possible candidates for laser-based investigations. The best candidate is the lowest-energy…
We consider hyperfine splitting of 1s and, in part, of 2s levels in light hydrogen-like atoms: hydrogen, deuterium, tritium, helium-3 ion, muonium and positronium. We discuss present status of precision theory and experiment for the hfs…
We propose a laser resonance chromatography (LRC) experiment on $^{229}$Th$^{3+}$, with the goal of detecting the ion's electronic ground $5f$ $^2$F$_{5/2}$ state and metastable $7s$ $^2$S$_{1/2}$ state by means of their ion mobilities. To…
We report the relativistic coupled cluster study of the hyperfine structure and effect of the nuclear magnetization distribution (Bohr-Weisskopf effect) in the $6P_{1/2}$, $6P_{3/2}$ and $7S_{1/2}$ states of several Tl isotopes. It is shown…
It is shown that the non-relativistic ground state energy of helium-like and lithium-like ions with static nuclei can be interpolated in full physics range of nuclear charges $Z$ with accuracy of not less than 6 decimal digits (d.d.) or 7-8…
We present relativistic many-body calculations of atomic and molecular Schiff-moment interaction constants including interelectron correlation effects using atomic Gaussian basis sets specifically optimized for the Schiff interaction. Our…
The possibility of refining the energy of the 8.36-eV 229mTh nuclear isomer -- the most likely candidate for the role of a nuclear frequency standard -- by means of resonant optical pumping is discussed. Attention is focused on considering…
Thorium-doped LiCaAlF$_6$ and LiSrAlF$_6$ (Th:LiCAF and Th:LiSAF) are promising crystals for a solid-state nuclear clock based on the 8 eV transition in $^{229}$Th; however, their complex crystal structures complicate understanding the…
The longer-lived excited nuclear states, referred as nuclear isomers, exist due to the hindered decays owing to their peculiar nucleonic structural surroundings. Some of these conditions, being exceptionally rare and limited to achieve,…