English
Related papers

Related papers: Hyperfine interaction with the $^{229}$Th nucleus …

200 papers

The hyperfine structure of the long-lived $5D_{3/2}$ and $5D_{5/2}$ levels of Ba$^+$ ion is analyzed. A procedure for extracting relatively unexplored nuclear magnetic moments $\Omega$ is presented. The relevant electronic matrix elements…

Atomic Physics · Physics 2009-11-13 K. Beloy , A. Derevianko , V. A. Dzuba , G. T. Howell , B. B. Blinov , E. N. Fortson

We explore an unusual nature of chemical bonding of the thorium atom with a ring of six carbon atoms (hexagon) in novel carbon materials. Our ab initio calculations of Th-based metallofullerenes (Th@C60, Th@C20) and Th bound to benzene or…

Materials Science · Physics 2020-12-02 A. V. Bibikov , A. V. Nikolaev , E. V. Tkalya

Motivated by recent experimental advances, including the ongoing development of an optical atomic clock in singly ionised radium, we perform a detailed theoretical characterisation of Ra+ and its lighter analogue, Ba+. Both ions are of…

Atomic Physics · Physics 2025-09-30 Robin B. Cserveny , Benjamin M. Roberts

A new method for obtaining of inverse population between quadrupole sublevels of the ground state $5/2^+(0.0)$ and the isomeric state $3/2^+(7.6$ eV) of the $^{229}$Th nucleus in a dielectric crystal with a large band gap by means of…

Nuclear Theory · Physics 2013-08-07 E V Tkalya , L P Yatsenko

The multiconfiguration Dirac-Hartree-Fock method implemented in the Grasp2018 package was employed to calculate the magnetic dipole hyperfine interaction constants and electric field gradients of levels in the ground configuration of the…

Atomic Physics · Physics 2025-03-26 Jiguang Li , Jacek Bieroń , Michel Godefroid , Per Jönsson

Precision measurements of Schiff moments in heavy, deformed nuclei are sensitive probes of beyond Standard Model $T,P$-violation in the hadronic sector. While the most sensitive limits on Schiff moments to date are set with diamagnetic…

Atomic Physics · Physics 2021-01-15 Phelan Yu , Nicholas R. Hutzler

The 7.8 eV nuclear isomer transition in 229 Thorium has been suggested as an etalon transition in a new type of optical frequency standard. Here we discuss the construction of a "solid-state nuclear clock" from Thorium nuclei implanted into…

Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…

An experiment to search for the electron electric dipole moment (\eEDM) on the metastable $H^3\Delta_1$ state of ThO molecule was proposed and now in the final stage of preparation by the ACME collaboration [http://www.electronedm.org]. To…

Chemical Physics · Physics 2013-12-13 L. V. Skripnikov , A. N. Petrov , A. V. Titov

Binding energies of high-L Rydberg states (L^3 7) of Th2+ with n=27-29 were studied using the Resonant Excitation Stark Ionization Spectroscopy (RESIS) method. The core of the Th2+ Rydberg ion is the Fr-like ion Th3+ whose ground state is a…

Atomic Physics · Physics 2011-06-07 J. A. Keele , M. E. Hanni , S. L. Woods , S. R. Lundeen , C. W. Fehrenbach

The 8.4 eV transition in the $^{229}$Th nucleus is the basis for a high-precision nuclear clock with exceptional sensitivity to new physics effects. We have identified several cases in the Th$^+$ ion where electronic excitations closely…

Atomic Physics · Physics 2025-04-29 V. A. Dzuba , V. V. Flambaum

There exist in nature a few nuclear isomers with very low (eV) excitation energies, and the combination of low energy and narrow width makes them possible candidates for laser-based investigations. The best candidate is the lowest-energy…

Nuclear Theory · Physics 2008-11-26 A. C. Hayes , J. L. Friar

We consider hyperfine splitting of 1s and, in part, of 2s levels in light hydrogen-like atoms: hydrogen, deuterium, tritium, helium-3 ion, muonium and positronium. We discuss present status of precision theory and experiment for the hfs…

High Energy Physics - Phenomenology · Physics 2014-11-17 Savely G. Karshenboim , Vladimir G. Ivanov

We propose a laser resonance chromatography (LRC) experiment on $^{229}$Th$^{3+}$, with the goal of detecting the ion's electronic ground $5f$ $^2$F$_{5/2}$ state and metastable $7s$ $^2$S$_{1/2}$ state by means of their ion mobilities. To…

We report the relativistic coupled cluster study of the hyperfine structure and effect of the nuclear magnetization distribution (Bohr-Weisskopf effect) in the $6P_{1/2}$, $6P_{3/2}$ and $7S_{1/2}$ states of several Tl isotopes. It is shown…

Atomic Physics · Physics 2019-03-08 S. D. Prosnyak , D. E. Maison , L. V. Skripnikov

It is shown that the non-relativistic ground state energy of helium-like and lithium-like ions with static nuclei can be interpolated in full physics range of nuclear charges $Z$ with accuracy of not less than 6 decimal digits (d.d.) or 7-8…

Atomic Physics · Physics 2017-11-27 Alexander V. Turbiner , Juan C. Lopez Vieyra , Horacio Olivares Pilon

We present relativistic many-body calculations of atomic and molecular Schiff-moment interaction constants including interelectron correlation effects using atomic Gaussian basis sets specifically optimized for the Schiff interaction. Our…

Atomic Physics · Physics 2022-09-14 Mickaël Hubert , Timo Fleig

The possibility of refining the energy of the 8.36-eV 229mTh nuclear isomer -- the most likely candidate for the role of a nuclear frequency standard -- by means of resonant optical pumping is discussed. Attention is focused on considering…

Nuclear Theory · Physics 2024-03-26 F. F. Karpeshin

Thorium-doped LiCaAlF$_6$ and LiSrAlF$_6$ (Th:LiCAF and Th:LiSAF) are promising crystals for a solid-state nuclear clock based on the 8 eV transition in $^{229}$Th; however, their complex crystal structures complicate understanding the…

Materials Science · Physics 2026-01-13 Martin Pimon , Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy , Andreas Grüneis

The longer-lived excited nuclear states, referred as nuclear isomers, exist due to the hindered decays owing to their peculiar nucleonic structural surroundings. Some of these conditions, being exceptionally rare and limited to achieve,…

Nuclear Theory · Physics 2024-02-07 Bhoomika Maheshwari , Ashok Kumar Jain