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We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from…

Atomic Physics · Physics 2026-01-30 R. Esteban Goetz , Anh-Thu Le

The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…

Atomic Physics · Physics 2021-11-24 Kunlong Liu , Yibo Hu , Qingbin Zhang , Peixiang Lu

Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…

Atomic Physics · Physics 2022-03-29 Lei Geng , Hao Liang , K. Krajewska , Liang-You Peng , Qihuang Gong

We present a theoretical study of transient absorption and reshaping of extreme ultraviolet (XUV) pulses by helium atoms dressed with a moderately strong infrared (IR) laser field. We formulate the atomic response using both the…

Atomic Physics · Physics 2013-03-25 Mette B. Gaarde , Christian Buth , Jennifer L. Tate , Kenneth J. Schafer

Light-matter entanglement plays a fundamental role in many applications of quantum information science. Thus, finding processes where it can be observed is an important task. Here, we address this matter by theoretically investigating the…

We address the influence of the molecular orbital geometry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules for different molecular species,…

Atomic Physics · Physics 2015-05-28 T. Shaaran , B. B. Augstein , C. Figueira de Morisson Faria

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We observe energy-dependent angle-resolved diffraction patterns in protons from strong-field dissociation of the molecular hydrogen ion H$_2^+$. The interference is a characteristic of dissociation around a laser-induced conical…

Atomic and Molecular Clusters · Physics 2016-04-11 Adi Natan , Matthew R Ware , Vaibhav S. Prabhudesai , Uri Lev , Barry D. Bruner , Oded Heber , Philip H Bucksbaum

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

Although it seems that obtaining quantum properties of light from classical calculations is a self-contradictory claim, it is shown here that a unified mechanism governs the three distinct measurements of high harmonic generation spectra…

Quantum Physics · Physics 2024-09-18 Nimrod Moiseyev

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

An ab initio theory is devised for the x-ray photoabsorption cross section of atoms in the field of a moderately intense optical laser (800nm, 10^13 W/cm^2). The laser dresses the core-excited atomic states, which introduces a dependence of…

Atomic Physics · Physics 2013-03-25 Christian Buth , Robin Santra

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

The single ionization of noble gas atoms by the combined action of XUV attopulses and an infrared laser field is theoretically investigated by means of a non-perturbative model that under certain approximations gives closed-form expressions…

Atomic Physics · Physics 2015-12-21 D. I. R. Boll , O. A. Fojón

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…

Atomic Physics · Physics 2020-08-26 Lorenz Drescher , Marc J. J. Vrakking , Jochen Mikosch

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

We investigate the role of hyperfine structure in resonant-dipole interactions between two atoms cotrapped in an optical tweezer. Two-body loss rates from light-assisted collisions (LACs) are measured across the $^{87}$Rb hyperfine spectrum…

Atomic Physics · Physics 2025-01-14 Steven K. Pampel , Matteo Marinelli , Mark O. Brown , José P. D'Incao , Cindy A. Regal

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…