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Related papers: Defect-induced oxygen adsorption on graphene films

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We study the low temperature properties of a single layer of parahydrogen adsorbed on graphene, by means of Quantum Monte Carlo simulations. The computed phase diagram is very similar to that of helium on the same substrate, featuring…

Mesoscale and Nanoscale Physics · Physics 2018-05-02 Marisa Dusseault , Massimo Boninsegni

We have carried out ab initio electronic structure calculations on graphane (hydrogenated graphene) with single and double vacancy defects. Our analysis of the density of states reveal that such vacancies induce the mid gap states and…

Materials Science · Physics 2010-02-11 Bhalchandra S. Pujari , D. G. Kanhere

In cold astrophysical environments, some molecules are observed in the gas phase whereas they should have been depleted, frozen on dust grains. In order to solve this problem, astrochemists have proposed that a fraction of molecules…

Chemical Physics · Physics 2016-03-02 Minissale Marco , Dulieu François

Understanding the reactivity of carbon surfaces is crucial for the development of advanced functional materials. In this study, we systematically investigate the reactivity of graphene surfaces with the Stone-Wales (SW) defect using Density…

Materials Science · Physics 2023-08-11 Aleksandar Z. Jovanović , Ana S. Dobrota , Natalia V. Skorodumova , Igor A. Pašti

We investigate the microscopic processes leading to graphene growth by the chemical vapor deposition of propane in the argon atmosphere at the SiC surface. Experimentally, it is known that the presence of argon fastens the dehydrogenation…

Materials Science · Physics 2017-09-13 Malgorzata Wierzbowska , Adam Dominiak , Kamil Tokar

The mechanical integrity of composite materials depends primarily on the interface strength and the defect density of the reinforcement which is the provider of enhanced strength and stiffness. In the case of graphene/ polymer…

The chemical reactivity of graphene under ultraviolet (UV) light irradiation is investigated under positive and negative gate electric fields. Graphene edges are selectively etched when negative gate voltages are applied, while the…

Materials Science · Physics 2013-11-15 Nobuhiko Mitoma , Ryo Nouchi

Graphene forms from a relatively dense, tightly-bound C-adatom gas, when elemental C is deposited on or segregates to the Ru(0001) surface. Nonlinearity of the graphene growth rate with C adatom density suggests that growth proceeds by…

Materials Science · Physics 2010-12-14 E. Loginova , N. C. Bartelt , P. J. Feibelman , K. F. McCarty

The physical processes occurring in the presence of disorder: point defects, grain boundaries, etc. may have detrimental effects on the electronic properties of graphene. Here we present an approach to reveal the grain structure of graphene…

In order to realize applications of hydrogen-adsorbed graphene, a main issue is how to control hydrogen adsorption/desorption at room temperature. In this study, we demonstrate the possibility to tune hydrogen adsorption on graphene by…

Mesoscale and Nanoscale Physics · Physics 2019-05-07 Yuya Murata , Arrigo Calzolari , Stefan Heun

Electron paramagnetic resonance (EPR) study of air-physisorbed defective carbon nano-onions evidences in favor of microwave assisted formation of weakly-bound paramagnetic complexes comprising negatively-charged O2- ions and edge carbon…

Mesoscale and Nanoscale Physics · Physics 2016-06-10 D. W. Boukhvalov , V. Yu. Osipov , A. I. Shames , K. Takai , T. Hayashi , T. Enoki

Reduced graphene oxide (rGO) is a bulk-processable quasi-amorphous 2D material with broad spectral coverage and fast electronic response. rGO sheets are suspended in a polymer matrix and sequentially photoreduced while measuring the…

Materials Science · Physics 2023-06-19 Alden N. Bradley , Spencer G. Thorp , Gina Mayonado , Edward Elliott , Matt W. Graham

Using micro-Raman spectroscopy and scanning tunneling microscopy, we study the relationship between structural distortion and electrical hole doping of graphene on a silicon dioxide substrate. The observed upshift of the Raman G band…

Materials Science · Physics 2012-01-23 Sunmin Ryu , Li Liu , Stephane Berciaud , Young-Jun Yu , Haitao Liu , Philip Kim , George W. Flynn , Louis E. Brus

We showed how a structural modification of graphene, which gives a carbon allotrope graphyne, can induce an energy gap at the K point of the Brillouin zone. Upon adsorption on metallic surfaces, the same mechanism is responsible for the…

Mesoscale and Nanoscale Physics · Physics 2014-10-16 P. Lazic , Z. Crljen

Atomic oxygen adsorption on the Mo(112) surface has been investigated by means of first-principles total energy calculations. Among the variety of possible adsorption sites it was found that the bridge sites between two Mo atoms of the…

Materials Science · Physics 2007-05-23 Adam Kiejna , R. M. Nieminen

Graphene is expected to be rather insensitive to ionizing particle radiation. We demonstrate that single layers of exfoliated graphene sustain significant damage from irradiation with slow highly charged ions. We have investigated the ion…

Materials Science · Physics 2013-10-24 J. Hopster , R. Kozubek , B. Ban-d'Etat , S. Guillous , H. Lebius , M. Schleberger

The results of DFT supercell calculations of oxygen behavior upon the UN (001) and (110) surfaces as well as at the tilt grain boundary are presented. Oxygen adsorption, migration, incorporation into the surface N vacancies on (001) and…

Materials Science · Physics 2015-06-12 D. Bocharov , D. Gryaznov , Yu. F. Zhukovskii , E. A. Kotomin

Using magnetization measurements, we show that point defects in graphene - fluorine adatoms and irradiation defects (vacancies) - carry magnetic moments with spin 1/2. Both types of defects lead to notable paramagnetism but no magnetic…

Mesoscale and Nanoscale Physics · Physics 2012-05-23 R. R. Nair , M. Sepioni , I-Ling Tsai , O. Lehtinen , J. Keinonen , A. V. Krasheninnikov , T. Thomson , A. K. Geim , I. V. Grigorieva

Plasma surface modification was used to fabricate graphene on the top of insulating diamond-like carbon films. It is shown that by a combination of pulsed argon plasma treatment and thermal annealing at 350\degreeC is possible to achieve…

Materials Science · Physics 2012-07-05 Savcho Tinchev

A single-crystal sheet of graphene is synthesized on the low-symmetry substrate Ir(110) by thermal decomposition of C$_2$H$_4$ at 1500 K. Using scanning tunneling microscopy, low-energy electron diffraction, angle-resolved photoemission…

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