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The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

We present out-of-plane dielectric and magnetodielectric measurements of single crystallines $\alpha$-RuCl$_3$ with various degrees of stack faults. A frequency dependent, but field independent, dielectric anomaly appears at…

The 2D layered insulator $\alpha$-RuCl$_3$ is a candidate material for a quantum spin-liquid state, which may be realized when a magnetic field suppresses the antiferromagnetic order present at low temperature. Oscillations in the field…

Strongly Correlated Electrons · Physics 2023-02-10 Étienne Lefrançois , Jordan Baglo , Quentin Barthélemy , Subin Kim , Young-June Kim , Louis Taillefer

Material realization of the non-Abelian Kitaev spin liquid phase - an example of Ising topological order (ITO) - has been the subject of intense research in recent years. The $4d$ honeycomb Mott insulator $\alpha$-RuCl$_3$ has emerged as a…

Strongly Correlated Electrons · Physics 2021-02-26 Jacob S. Gordon , Hae-Young Kee

The recently proposed multiferroic state of the charge-transfer salt {\kappa}-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl [P. Lunkenheimer et al., Nature Mater., vol. 11, pp. 755-758, Sept. 2012] has been studied by dc-conductivity, magnetic…

Strongly Correlated Electrons · Physics 2018-07-04 M. Lang , P. Lunkenheimer , J. Müller , A. Loidl , B. Hartmann , N. H. Hoang , E. Gati , H. Schubert , J. A. Schlueter

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

Magnetic dc susceptibility between 1.5 and 800 K, ac susceptibility and magnetization, thermodynamic properties, temperature dependence of radio and audio-wave dielectric constants and conductivity, contact-free dielectric constants at…

Materials Science · Physics 2010-07-22 Jun Lu , A. Günther , F. Schrettle , F. Mayr , S. Krohns , P. Lunkenheimer , A. Pimenov , V. D. Travkin , A. A. Mukhin , A. Loidl

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Strongly Correlated Electrons · Physics 2016-09-21 A. Koitzsch , C. Habenicht , E. Mueller , M. Knupfer , B. Buechner , H. Kandpal , J. van den Brink , D. Nowak , A. Isaeva , Th. Doert

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

Strongly Correlated Electrons · Physics 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

We report magnetic and thermodynamic properties of single crystal $\alpha$-RuCl$_3$, in which the Ru$^{3+}$ ($4d^5$) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2015-04-27 J. A. Sears , M. Songvilay , K. W. Plumb , J. P. Clancy , Y. Qiu , Y. Zhao , D. Parshall , Young-June Kim

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

The Mott insulator $\alpha$-RuCl$_3$ has generated great interest in the community due to its possible field-induced Kitaev quantum spin liquid state. Despite enormous effort spent trying to obtain the form of the low energy Hamiltonian,…

We discuss the implications that new magnetocaloric, thermal expansion and magnetostriction data in $\alpha$-RuCl$_{3}$ single crystals have on its temperature-field phase diagram and uncover the magnetic-field dependence of an apparent…

Thermodynamics of the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ is studied for different directions of in-plane magnetic field using measurements of the magnetic Gr\"uneisen parameter $\Gamma_B$ and specific heat $C$. We identify two…

Strongly Correlated Electrons · Physics 2021-03-03 S. Bachus , D. A. S. Kaib , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valentí , P. Gegenwart

The dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ can be tuned into a metallic and superconducting state upon applying pressure of 1.5 kbar and more. We have performed dielectric spectroscopy measurements (7 kHz to 5 MHz) on…

Strongly Correlated Electrons · Physics 2021-03-17 R. Rösslhuber , A. Pustogow , E. Uykur , A. Böhme , A. Löhle , R. Hübner , J. Schlueter , Y. Tan , V. Dobrosavljević , M. Dressel

We report a rather high dependence of the dielectric permittivity on the magnetic field in La2/3Ca1/3MnO3. The variation is maximum at around 270 K, little above the Curie temperature, TC, and it reaches a 30% under only 0.5 T. We attribute…

Strongly Correlated Electrons · Physics 2009-11-11 J. Rivas , J. Mira , B. Rivas-Murias , A. Fondado , J. Dec , W. Kleemann , M. A. Senaris Rodriguez

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

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