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We review many-body effects, their microscopic origin, as well as their impact onto thermoelectricity in correlated narrow-gap semiconductors. Members of this class---such as FeSi and FeSb$_2$---display an unusual temperature dependence in…

Strongly Correlated Electrons · Physics 2018-04-11 Jan M. Tomczak

Utilizing the non-coherent quantum transport formalism, we investigate thermoelectric performance across dissipative superlattice configurations in the linear regime of operation. Using the {\it{dissipative}} non-equilibrium Green's…

Mesoscale and Nanoscale Physics · Physics 2020-12-30 Pankaj Priyadarshi , Bhaskaran Muralidharan

In search of new prospects for thermoelectric materials, using ab-initio calculations and semi-classical Boltzmann theory, we have systematically investigated the electronic structure and transport properties of 18-valence electron count…

Computational Physics · Physics 2017-12-20 Mohd Zeeshan , Harish K. Singh , Jeroen van den Brink , Hem C. Kandpal

Bi2Te3 based thermoelectric devices typically use a nickel layer as a diffusion barrier to block the diffusion of solder or copper atoms from the electrode into the thermoelectric material. Previous studies have shown degradation in the…

Materials Science · Physics 2012-12-05 Kevin C. Lukas , Weishu Liu , Zhifeng Ren , Cyril P. Opeil

The thermoelectric response of 80-nm-thick strained HgTe films of a three-dimensional topological insulator (3D TI) has been studied experimentally. An ambipolar thermopower is observed where the Fermi energy moves from conducting to the…

Mesoscale and Nanoscale Physics · Physics 2021-12-14 G. M. Gusev , Z. D. Kvon , A. D. Levin , N. N. Mikhailov

Buildings are responsible for a considerable fraction of the energy wasted globally every year, and as a result, excess carbon emissions. While heat is lost directly in colder months and climates, resulting in increased heating loads, in…

The binary compound SnSe exhibits record high thermoelectric performance, largely because of its very low thermal conductivity. The origin of the strong phonon anharmonicity leading to the low thermal conductivity of SnSe is investigated…

Materials Science · Physics 2019-11-12 Jiawang Hong , Olivier Delaire

The thermoelectric efficiency of semiconductors is usually considered in the ohmic electronic transport regime, which is achieved through high doping. Here we consider the opposite regime of low doping where the current-voltage…

Materials Science · Physics 2012-10-01 François Léonard

Thermoelectric properties of monolayer indium selenide (InSe) are investigated by using Boltzman transport theory and first-principles calculations as a function of Fermi energy and crystal orientation. We find that the maximum power factor…

Materials Science · Physics 2017-09-05 Nguyen T. Hung , Ahmad R. T. Nugraha , R. Saito

In this work, we report the structural, magnetic and electrical and thermal transport properties of the Heusler-type alloy Ru2NbAl. From the detailed analysis of magnetization data, we infer the presence of superparamagnetically interacting…

Strongly Correlated Electrons · Physics 2018-11-21 Sanchayita Mondal , Chandan Mazumdar , R. Ranganathan , Eric Alleno , P. C. Sreeparvathy , V. Kanchana , G. Vaitheeswaran

We present an ab initio study of the structural and electronic transport properties of tetrahedrite, Cu$_{12}$Sb$_4$S$_{13}$, in its high-temperature phase. We show how this complex compound can be seen as the outcome of an ordered…

Materials Science · Physics 2020-07-07 Cono di Paola , Francesco Macheda , Savio Laricchia , Cedric Weber , Nicola Bonini

Thermoelectric materials convert heat into electricity through thermally driven charge transport in solids, or vice versa for cooling. To be competitive with conventional energy-generation technologies, a thermoelectric material must…

We report transport studies on (Bi,Sb)2Te3 topological insulator thin films with tunable electronic band structure. We find a doping and temperature regime in which the Hall coefficient is negative indicative of electron-type carriers,…

Thermoelectric technology is an alternate way to efficiently utilize the energy by converting waste heat into electricity. Thermoelectric requires material with low thermal conductivity to improves its thermoelectric performance. In this…

Materials Science · Physics 2021-01-22 Rajmohan Muthaiah , Jivtesh Garg

By combining the electronic structures obtained from first principles calculations with Boltzmann transport theory we have investigated the electronic, magnetic and transport properties of Co$_{2}$MnGe Heusler compound. The density of…

Materials Science · Physics 2014-06-16 Sonu Sharma , Sudhir K. Pandey

Thermoelectric materials convert a temperature gradient into a voltage. This phenomenon is relatively well understood for inorganic materials, but much less so for organic semiconductors (OSs). These materials present a challenge because…

The atomic variations of electronic wavefunctions at the surface and electron scattering near a defect have been detected unprecedentedly by tracing thermoelectric voltages given a temperature bias [Cho et al., Nature Mater. 12, 913…

Mesoscale and Nanoscale Physics · Physics 2014-04-02 Eui-Sup Lee , Sanghee Cho , Ho-Ki Lyeo , Yong-Hyun Kim

First principles studies were performed in order to find out the possibility of inducing half-metallicity in Heusler Compound CoFeMnSb, by means of alloying it with 3d-transition metal elements. Proper alloying element is selected through…

Materials Science · Physics 2019-05-15 Upendra Kumar , P. V. Sreenivasa Reddy , Satadeep Bhattacharjee , Seung-Cheol Lee

Nanostructured composites and nanowire arrays of traditional thermoelectrics like Bi, Bi(1-x)Sb(x) and Bi(2)Te(3) have metallic Rashba surface spin-orbit bands featuring high mobilities rivaling that of the bulk for which topological…

Materials Science · Physics 2015-05-30 T. E. Huber , K. Owusu , S. Johnson , A. Nikolaeva L. Konopko , R. C. Johnson , M. J. Graf

Thermoelectric films and periodic structures have particularly intriguing electrical and thermal transport features due to their low dimensionality. As a result, they have piqued the attention of researchers from across the spectrum of…

Materials Science · Physics 2024-02-23 Nagaraj Nandihalli