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With their brilliance and temporal structure, X-ray free-electron laser can unveil atomic-scale details of ultrafast phenomena. Recent progress in split-and-delay optics (SDO), which produces two X-ray pulses with time-delays, offers bright…

Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…

Atomic Physics · Physics 2019-05-15 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Arbitrary manipulation of the temporal and spectral properties of X-ray pulses at free-electron lasers (FELs) would revolutionize many experimental applications. At the Linac Coherent Light Source at Stanford National Accelerator…

The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome…

Optics · Physics 2021-02-15 Stefano M. Cavaletto , Daniel Keefer , Shaul Mukamel

X-ray Free-Electron Lasers (XFELs) deliver X-ray pulses with a coherent flux that is approximately eight orders of magnitude greater than that available from a modern third generation synchrotron source. The power density in an XFEL pulse…

Low-collisionality plasma in a magnetic field generically develops anisotropy in its distribution function with respect to the magnetic field direction. Motivated by the application to radiation from accretion flows and jets, we explore the…

High Energy Astrophysical Phenomena · Physics 2023-09-20 Alisa Galishnikova , Alexander Philippov , Eliot Quataert

Dynamics of optically-excited plasmonic nanoparticles are presently understood as a series of sequential scattering events, involving thermalization processes after pulsed optical excitation. One important step is the initiation of…

Textures in images can often be well modeled using self-similar processes while they may at the same time display anisotropy. The present contribution thus aims at studying jointly selfsimilarity and anisotropy by focusing on a specific…

Data Analysis, Statistics and Probability · Physics 2015-06-16 S. G. Roux , M. Clausel , B. Vedel , S. Jaffard , P. Abry

Exciton plasmon polaritons have gained increasing interests over recent years due to their versatile properties emerging by the underlying light-matter coupling and making them potential candidates for new photonic applications. We have…

In single particle coherent x-ray diffraction imaging experiments, performed at x-ray free-electron lasers (XFELs), samples are exposed to intense x-ray pulses to obtain single-shot diffraction patterns. The high intensity induces…

Atomic and Molecular Clusters · Physics 2013-01-29 U. Lorenz , N. M. Kabachnik , E. Weckert , I. A. Vartanyants

We propose a technique, to be used for time-resolved pump-probe experiments, for timing an x-ray free electron laser (XFEL) to a high-power conventional laser with femtosecond accuracy. Our method takes advantage of the same electron bunch…

Accelerator Physics · Physics 2009-11-13 Gianluca Geloni , Evgeni Saldin , Evgeni Schneidmiller , Mikhail Yurkov

We have conducted a series of scattering experiments at the uranium M4 absorption edge on low-symmetry uranium compounds (U2N3 and U3O8) produced as epitaxial films. At weak and forbidden reflections, we find a resonant signal, independent…

Strongly Correlated Electrons · Physics 2024-10-02 E. Lawrence Bright , E. N. Ovchinnikova , L. M. Harding , D. G. Porter , R. Springell , V. E. Dmitrienko , R. Caciuffo , G. H. Lander

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

Recent developments of the pump-probe thermoreflectance methods (such as the beam-offset and elliptical-beam approaches of the time-domain and frequency-domain thermoreflectance techniques) enabled measurements of the thermal conductivities…

Applied Physics · Physics 2020-09-02 Puqing Jiang , Heng Ban

X-ray polarimetry has great scientific potential and new experiments, such as X-Calibur, PoGOLite, XIPE, and GEMS, will not only be orders of magnitude more sensitive than previous missions, but also provide the capability to measure…

Instrumentation and Methods for Astrophysics · Physics 2015-03-03 Fabian Kislat , Matthias Beilicke , Qingzhen Guo , Anna Zajczyk , Henric Krawczynski

Polarized emission carries captivating information and can help understand various elementary processes involving collisions within the plasma as well as in radiative transitions. In this work, we investigate the spatio-temporal dependence…

Plasma Physics · Physics 2023-10-23 Geethika B. R. , Jinto Thomas , Milaan Patel , Renjith Kumar R. , Hem Chandra Joshi

Measuring the time structure of the storage ring on the sample spot inside the experimental hutch is a foundational step during the time-resolved experiments using the pulsed synchrotron X-rays with the time structure defined by the storage…

Instrumentation and Detectors · Physics 2014-10-08 Zhang Zhaohong , Jiang Zheng , Xue Song , Zheng Lifang

Advances in our ability to understand and utilize the world around us have always relied on the development of advanced tools for probing and manipulating materials properties. X-ray matter interactions played a critical role in the…

Materials Science · Physics 2021-08-13 Mariano Trigo , Mark P. M. Dean , David A. Reis
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