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We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

Materials Science · Physics 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

The spatiotemporal response of crystals in x-ray Bragg diffraction resulting from excitation by an ultra-short, laterally confined x-ray pulse is studied theoretically. The theory presents an extension of the analysis in symmetric…

Optics · Physics 2012-10-22 Yuri Shvyd'ko , Ryan Lindberg

Femtosecond laser exposure in the non-ablative regime induces a variety of bulk structural modifications, in which anisotropy may depend on the polarization of the writing beam. In this work, we investigate the correlation between…

Optics · Physics 2016-09-15 Ben McMillen , Yves Bellouard

We have observed the signatures of valence electron rearrangement in photoexcited ammonia using ultrafast hard X-ray scattering. Time-resolved X-ray scattering is a powerful tool for imaging structural dynamics in molecules because of the…

We describe an optical method to directly measure position-dependent thermal diffusivity of reflective single crystal samples across a broad range of temperatures for condensed matter physics research. Two laser beams are used, one as a…

We provide a theoretical analysis for the intermediate scattering function typically measured in depolarized dynamic light scattering experiments. We calculate the field autocorrelation function $g_1^{\rm VH}(Q,t)$ in dependence on the wave…

Soft Condensed Matter · Physics 2015-07-31 Christopher Passow , Borge ten Hagen , Hartmut Löwen , Joachim Wagner

X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…

Strongly Correlated Electrons · Physics 2025-02-11 Daniel Jost , Eder G. Lomeli , Ta Tang , Joshua J. Kas , John J. Rehr , Wei-Sheng Lee , Hong-Chen Jiang , Brian Moritz , Thomas P. Devereaux

Time-resolved mapping of lattice dynamics in real- and momentum-space is essential to understand better several ubiquitous phenomena such as heat transport, displacive phase transition, thermal conductivity, and many more. In this regard,…

Strongly Correlated Electrons · Physics 2021-01-06 Navdeep Rana , Aditya Prasad Roy , Dipanshu Bansal , Gopal Dixit

Molecular iodine was photoexcited by a strong 800 nm laser, driving several channels of multiphoton excitation. The motion following photoexcitation was probed using time-resolved X-ray scattering, which produces a scattering map…

Chemical Physics · Physics 2020-03-25 Philip H. Bucksbaum , Matthew R. Ware , Adi Natan , James P. Cryan , James M. Glownia

We develop a novel technique for modeling of atomic and molecular ionization in superposition of XUV and IR fields with characteristics typical for attosecond streaking and RABBITT experiments. The method is based on solving the…

Atomic Physics · Physics 2016-06-29 Vladislav V. Serov , A. S. Kheifets

The multiple scattering of scalar waves in diffusive media is investigated by means of the radiative transfer equation. This approach, which does not rely on the diffusion approximation, becomes asymptotically exact in the regime of most…

Condensed Matter · Physics 2009-10-28 E. Amic , J. M. Luck , Th. M. Nieuwenhuizen

The scintillation anisotropy effect for proton recoil events has been investigated in five pure organic crystalline materials: anthracene, trans-stilbene, p-terphenyl, bibenzyl, and diphenylacetylene. These measurements include…

Instrumentation and Detectors · Physics 2018-05-04 Patricia Schuster , Patrick Feng , Erik Brubaker

This paper is concerned with the inverse scattering problem for the three-dimensional Maxwell's equations in bi-anisotropic periodic structures. The inverse scattering problem aims to determine the shape of bi-anisotropic periodic…

Numerical Analysis · Mathematics 2020-08-25 Dinh-Liem Nguyen , Trung Truong

X-ray free-electron lasers (XFELs) produce X-ray pulses with high brilliance and short pulse duration. These properties enable structural investigations of biomolecular nanocrystals, and they allow resolving the dynamics of biomolecules…

Chemical Physics · Physics 2022-08-05 Leonie Chatzimagas , Jochen S. Hub

The macroscopic characteristics of a solid, such as its thermal, optical or transport properties are determined by the available microscopic states above its lowest energy level. These slightly higher quantum states are described by…

In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Thomas P. Devereaux , John P. Hill , Jeroen van den Brink

Photochemical reactions on semiconductors are anisotropic, since they occur with different rates on surfaces of different orientation. Understanding the origin of this anisotropy is crucial to engineering more efficient photocatalysts. In…

Materials Science · Physics 2022-05-04 Chiara Ricca , Ulrich Aschauer

Time-resolved X-ray Emission/Absorption Spectroscopy (Tr-XES/XAS) is an informative experimental tool sensitive to electronic dynamics in materials, widely exploited in diverse research fields. Typically, Tr-XES/XAS requires X-ray pulses…

Resonance anomalous surface x-ray scattering (RASXS) technique was applied to electrochemical interface studies. It was used to determine the chemical states of electrochemically formed anodic oxide monolayers on platinum surface. It is…

X-ray laser-induced structural changes in silicon undergoing femtosecond melting have been investigated by using an x-ray pump-x-ray probe technique. The experimental results for different initial sample temperatures reveal that the onset…

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