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Related papers: Interlayer excitons in MoSe$_2$/WSe$_2$ heterostru…

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Excitons in bilayer transition metal dichalcogenides (2L-TMDs) are Coulomb-bound electron/hole pairs that can be viewed as broadly tunable analogs of atomic or molecular systems. Here, we study the properties of 2L-TMD excitons under strong…

Mesoscale and Nanoscale Physics · Physics 2023-03-20 S. Kovalchuk , K. Greben , A. Kumar , S. Pessel , K. Watanabe , T. Taniguchi , D. Christiansen , M. Selig , A. Knorr , K. I. Bolotin

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…

Transition metal dichalcogenide (TMD) bilayers with an interlayer twist exhibit a moire super-period, whose effects can manifest in both structural and electronic properties. Atomic displacements can lead to reconstruction into domains of…

Materials Science · Physics 2025-10-23 Madeleine Phillips , C. Stephen Hellberg

Monolayer WSe$_2$ hosts a series of exciton Rydberg states denoted by the principal quantum number n = 1, 2, 3, etc. While most research focuses on their absorption properties, their optical emission is also important but much less studied.…

Materials Science · Physics 2019-05-22 Erfu Liu , Jeremiah van Baren , Takashi Taniguchi , Kenji Watanabe , Yia-Chung Chang , Chun Hung Lui

MA2Z4 monolayers form a new class of hexagonal non-centrosymmetric materials hosting extraordinary spin-valley physics. While only two compounds (MoSi2N4 and WSi2N4) were recently synthesized, theory predicts interesting (opto)electronic…

The interaction of intralayer and interlayer excitons is studied in a two-dimensional semiconductor, homobilayer MoS$_2$. It is shown that the measured optical susceptibility reveals both the magnitude and the sign of the coupling…

Moir\'e heterostructures are rapidly emerging as a tunable platform to study correlated electronic phenomena. Discovery of exotic quantum phases in moir\'e systems requires novel probes of charge and spin order. Unlike detection schemes…

Mesoscale and Nanoscale Physics · Physics 2021-11-19 Weijie Li , Luka M. Devenica , Jin Zhang , Yang Zhang , Xin Lu , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

We demonstrate the possibility of engineering the optical properties of transition metal dichalcogenide heterobilayers when one of the constitutive layers has a Janus structure. This has important consequences for the charge separation…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Engin Torun , Fulvio Paleari , Milorad V. Milosevic , Ludger Wirtz , Cem Sevik

In this work, we present a mathematical model for the Wannier-Mott exciton in monolayers of transition metal dichalcogenides such as $WS_2$, $WSe_2$, $MoS_2$, $MoSe_2$ that estimates the radiation lifetime in the effective mass…

Mesoscale and Nanoscale Physics · Physics 2025-06-06 Rohit Ramesh Nimje , Swati G , Ashutosh Mahajan

Strong Coulomb interactions can drive electrons to crystallize into a Wigner lattice. Achieving the bosonic analogue - a crystal of excitons - has remained elusive due to their short lifetimes and weaker interactions. Here, we report the…

We present first-principles calculations of the optical response of monolayer molybdenum disulfide employing the GW-Bethe Salpeter equation (GW-BSE) approach including self-energy, excitonic, and electron-phonon effects. We show that…

Materials Science · Physics 2014-06-30 Diana Y. Qiu , Felipe H. da Jornada , Steven G. Louie

For quantum technologies based on single excitons and spins, the deterministic placement and control of a single exciton is a long-standing goal. MoSe2-WSe2 heterostructures host spatially indirect interlayer excitons (IXs) which exhibit…

Monolayer transition-metal dichalcogenides, such as WSe$_2$, are direct gap, multi-valley semiconductors. Long-range electron-hole exchange interactions mix the valleys, yielding dispersion relations for massive ($\propto Q^2$) as well as…

Mesoscale and Nanoscale Physics · Physics 2025-08-20 A. Delhomme , T. Amit , P. Ji , C. Faugeras , S. Refaely-Abramson , J. J. Finley , A. V. Stier

We investigate the spin-valley physics (SVP) in MoSe$_2$/WSe$_2$ heterobilayers under external electric field (EF) and changes of the interlayer distance (ID). We analyze the spin ($S_z$) and orbital ($L_z$) degrees of freedom, and the…

Mesoscale and Nanoscale Physics · Physics 2023-04-11 Paulo E. Faria Junior , Jaroslav Fabian

A Bose-Einstein condensate is the ground state of a dilute gas of bosons, such as atoms cooled to temperatures close to absolute zero. With much smaller mass, excitons (bound electron-hole pairs) are expected to condense at significantly…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Zefang Wang , Daniel A. Rhodes , Kenji Watanabe , Takashi Taniguchi , James C. Hone , Jie Shan , Kin Fai Mak

Excitons dominate the optics of atomically-thin transition metal dichalcogenides and 2D van der Waals heterostructures. Interlayer 2D excitons, with an electron and a hole residing in different layers, form rapidly in heterostructures…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 M. G. Burdanova , M. Liu , M. Staniforth , Y. Zheng , R. Xiang , S. Chiashi , A. Anisimov , E. I. Kauppinen , S. Maruyama , J. Lloyd-Hughes

Transition-metal dichalcogenide heterostructures exhibit moir\'e patterns that spatially modulate the electronic structure across the material's plane. For certain material pairs, this modulation acts as a potential landscape with deep,…

Mesoscale and Nanoscale Physics · Physics 2021-03-12 David A. Ruiz-Tijerina , Isaac Soltero , Francisco Mireles

Moir\'{e} excitons (MXs) are electron-hole pairs localised by the periodic (moir\'{e}) potential forming in two-dimensional heterostructures (HSs). MXs can be exploited, $e.g.$, for creating nanoscale-ordered quantum emitters and achieving…

Interlayer excitons in van der Waals heterostructures offer rich collective phases, prospective optoelectronic applications, and versatile tunability, where control by electronic means is particularly relevant and practical. Here, in the…

Mesoscale and Nanoscale Physics · Physics 2025-02-20 Cem Sevik , Engin Torun , Milorad V. Milosevic , Fulvio Paleari

Exciton condensates (EC) are macroscopic coherent states arising from condensation of electron-hole pairs. Bilayer heterostructures, consisting of two-dimensional electron and hole layers separated by a tunnel barrier, provide a versatile…

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